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We report on the first detailed beam test attesting the fundamental principle behind the development of high-current-efficiency ultrafast electron microscope systems where a radio-frequency cavity is incorporated as a condenser lens in the…

材料科学 · 物理学 2024-01-03 Xiaoyi Sun , Joseph William , Sachin Sharma , Shriraj Kunjir , Dan Morris , Shen Zhao , Chong-Yu Ruan

Time-resolved optical spectroscopy (TR-OS) has emerged as a fundamental spectroscopic tool for probing complex materials, to both investigate ground-state-related properties and trigger phase transitions among different states with peculiar…

Optical frequency combs paved the way for fast and compact multi-component optical chemical analysis due to their broadband spectra. Dual-comb spectrometers embody this technology, but their design requires a pair of matched combs, adding…

光学 · 物理学 2025-09-25 Ina Heckelmann , Davide Pinto , Uwe Schmitt , Mattias Beck , Jérôme Faist

X-ray photoelectron diffraction is a powerful tool for determining the structure of clean and adsorbate-covered surfaces. Extending the technique into the ultrafast time domain will open the door to studies as diverse as the direct…

We investigate coherent phonon oscillations of BaFe$_2$As$_2$ using optical pump-probe spectroscopy. Time-resolved optical reflectivity shows periodic modulations due to $A_{1g}$ coherent phonon of $c$-axis arsenic vibrations. Optical probe…

We report on the impulsive generation of coherent optical phonons in CdTe0.68Se0.32 nanocrystallites embedded in a glass matrix. Pump probe experiments using femtosecond laser pulses were performed by tuning the laser central energy to…

介观与纳米尺度物理 · 物理学 2009-11-10 A. V. Bragas , C. Aku-Leh , S. Costantino , Alka Ingale , J. Zhao , R. Merlin

We describe a setup for time- and angle-resolved photoemission spectroscopy with wavelength-tunable excitation and extreme ultraviolet probe. It is enabled by using the 10 kHz twin Ti:sapphire amplifiers seeded by the common Ti:sapphire…

材料科学 · 物理学 2025-02-11 Takeshi Suzuki , Yigui Zhong , Kecheng Liu , Teruto Kanai , Jiro Itatani , Kozo Okazaki

Spintronics is postulated on the possibility to employ the magnetic degree of freedom of electrons for computation and couple it to charges. In this view, the combination of the high-frequency of spin manipulations offered by…

Ultrafast optical pump-probe spectroscopy is used to track carrier dynamics in the large magnetoresistance material WTe$_{2}$. Our experiments reveal a fast relaxation process occurring on a sub-picosecond time scale that is caused by…

We present a widefield two-dimensional electronic spectroscopy microscope (2DESM) that integrates multidimensional coherent spectroscopy with optical imaging, enabling femtosecond temporal and micrometer spatial resolution. The broadband…

Coherent optical phonons in bulk solid system play a crucial role in understanding and designing light-matter interactions and can be detected by the transient-reflectivity measurement. In this paper, we demonstrate spectrally resolved…

Coherent phonons describe the collective, ultrafast motion of atoms and play a central role in light-induced structural dynamics. Here, we employ terahertz scanning tunneling microscopy (THz-STM) to excite and detect coherent phonons in…

Raman scattering spectroscopy is widely used as an analytical technique in various fields, but its measurement process tends to be slow due to the low scattering cross-section. In the last decade, various broadband coherent Raman scattering…

光学 · 物理学 2025-05-06 Takuma Nakamura , Kazuki Hashimoto , Takuro Ideguchi

Time-resolved Raman spectroscopy has been applied to probe the anharmonic coupling and electron-phonon interaction of optical phonons in graphite. From the decay of the transient anti-Stokes scattering of the G-mode following ultrafast…

材料科学 · 物理学 2015-05-14 Hugen Yan , Daohua Song

We present and numerically investigate a high-quality factor (high-Q) meta-atom with Fano resonance. Numerical simulations indicate that the designed meta-atom has a single sharp Fano resonance in the 1350-1750 1/cm range. Moreover, the…

光学 · 物理学 2026-05-11 S. Hadi Badri , M. M. Gilarlue , Sanam Saeidnahaei , Jong Su Kim

Fast and broadband spectrum sensing is an essential component in cognitive radio systems, intelligent transportation systems, electronic warfare systems, etc. However, traditional electronic-based solutions have a trade-off among the…

光学 · 物理学 2024-09-25 Taixia Shi , Chi Jiang , Chulun Lin , Fangyi Yang , Yiqing Liu , Fangzheng Zhang , Yang Chen

The functionalities of a wide range of optical and opto-electronic devices are based on resonance effects and active tuning of the amplitude and wavelength response is often essential. Plasmonic nanostructures are an efficient way to create…

Controlling nonequilibrium responses in optically driven quantum materials is essential for advancing applications in energy conversion, ultrafast electronics, and quantum computation. Nonlinear optical spectroscopy serves as a powerful…

Frequency- and time-domain Brillouin scattering spectroscopy are powerful tools to read out the mechanical properties of complex systems in material and life sciences. Indeed, coherent acoustic phonons in the time-domain method offer…

光学 · 物理学 2023-01-06 Ayumu Ishijima , Shinga Okabe , Ichiro Sakuma , Keiichi Nakagawa

We directly measure by femtosecond time-resolved x-ray diffraction the E$_g$ symmetry coherent phonon excited in bismuth by strong optical excitation. The magnitude of the E$_g$ mode observed is 0.2 pm peak-to-peak, compared against the 2.7…

材料科学 · 物理学 2015-06-12 S. L. Johnson , P. Beaud , E. Möhr-Vorobeva , A. Caviezel , G. Ingold , C. J. Milne