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We describe how a local non-equilibrium nuclear polarisation can be generated and detected by electrical means in a semiconductor quantum point contact device. We show that measurements of the nuclear spin relaxation rate will provide clear…

介观与纳米尺度物理 · 物理学 2008-06-26 N. R. Cooper , V. Tripathi

While the breakdown of the perturbation expansion for the many-electron problem has several formal consequences, here we unveil its physical effect: Flipping the sign of the effective electronic interaction in specific scattering channels.…

强关联电子 · 物理学 2020-11-06 M. Reitner , P. Chalupa , L. Del Re , D. Springer , S. Ciuchi , G. Sangiovanni , A. Toschi

We calculate the non-linear tunneling current through a molecule with two electron-accepting orbitals which interact with an intramolecular vibration. We investigate the interplay between Coulomb blockade and non-equilibrium…

介观与纳米尺度物理 · 物理学 2007-05-23 Katja C. Nowack , Maarten R. Wegewijs

As promising quantum sensors, nitrogen-vacancy (NV) centers in diamond have been widely used in frontier studies in condensed matter physics, material sciences, and life sciences. In practical applications, weak laser excitation is…

We report on the observation of coherent molecular vibrations launched by the breaking of a molecular bond. The methyl radical, which is produced by $267\,\mathrm{nm}$ photodissociation of methyl iodide, is excited to high levels in its…

Vibrational nonequilibrium effects in charge transport through single-molecule junctions are investigated. Focusing on molecular bridges with multiple electronic states, it is shown that electronic-vibrational coupling triggers a variety of…

介观与纳米尺度物理 · 物理学 2011-03-15 R. Härtle , C. Benesch , M. Thoss

We investigate vibrational properties and lattice distortion of negatively charged nitrogen-vacancy (NV) center in diamond. Using the first-principles electronic structure calculations, we show that the presence of NV center leads to…

材料科学 · 物理学 2015-05-27 Jianhua Zhang , Cai-Zhuang Wang , Z. Z. Zhu , V. V. Dobrovitski

The "atomic saw method" uses the passage of dislocations in two-dimensional (2D) quantum-well superlattices to create periodic slipping layers and one-dimensional (1D) quantum wire superlattices. The effects of this space structuring of the…

无序系统与神经网络 · 物理学 2007-08-14 T. Ferrus , B. Goutiers , L. Ressier , J. P. Peyrade , J. A. Porto , J. Sanchez-dehesa

We study theoretically the effects of heating on the magnetic flux moving in superconductors with a periodic array of pinning sites (PAPS). The voltage-current characteristic (VI-curve) of superconductors with a PAPS includes a region with…

超导电性 · 物理学 2008-04-14 V. R. Misko , S. Savel'ev , A. L. Rakhmanov , Franco Nori

Carbon nanotube junctions are predicted to exhibit negative differential resistance, with very high peak-to-valley current ratios even at room temperature. We treat both nanotube p-n junctions and undoped metal-nanotube-metal junctions,…

凝聚态物理 · 物理学 2009-10-31 F. Leonard , J. Tersoff

Ultrafast laser excitation can trigger multiplex coherent dynamics in molecules. Here, we report attosecond transient absorption experiments addressing simultaneous probing of electronic and vibrational dynamics in a prototype molecule,…

Strong light-matter interaction in cavity environments is emerging as a promising approach to control chemical reactions in a non-intrusive and efficient manner. The underlying mechanism that distinguishes between steering, accelerating, or…

量子物理 · 物理学 2022-12-20 Christian Schäfer , Johannes Flick , Enrico Ronca , Prineha Narang , Angel Rubio

The quantum nonlinear dimer consisting of an electron shuttling between the two sites and in weak interaction with vibrations, is studied numerically under the application of a DC electric field. A field-induced resonance phenomenon between…

其他凝聚态物理 · 物理学 2011-11-04 M. Tiwari , D. V. Seletskiy , V. M. Kenkre

We present a perturbation approach rooted in time-dependent density-functional theory to calculate electron hole (eh)-pair excitation spectra during the non-adiabatic vibrational damping of adsorbates on metal surfaces. Our analysis for the…

化学物理 · 物理学 2017-11-22 Simon P. Rittmeyer , Jörg Meyer , Karsten Reuter

Gunn (or Gunn-Hilsum) Effect and its associated negative differential resistivity (NDR) emanates from transfer of electrons between two different energy bands in a semiconductor. If applying a voltage (electric field) transfers electrons…

介观与纳米尺度物理 · 物理学 2018-05-01 Daryoush Shiri , Amit Verma , Reza Nekovei , Andreas Isacsson , C. R. Selvakumar , M. P. Anantram

The interplay between uniaxial strain and charging effects in zigzag graphene nanoribbons (ZGNR) is investigated by using non-equilibrium Green's function formalism. The I-V characteristic curves and especially negative differential…

介观与纳米尺度物理 · 物理学 2019-12-05 Maliheh Azadparvar , Hosein Cheraghchi

Optically active quantum defects in solids, such as the nitrogen vacancy (NV) center in diamond, are a leading modality for micron-scale and nanoscale (ultralow-mass) nuclear magnetic resonance (NMR) spectroscopy and imaging under ambient…

We investigate chemical bond formation and conductance in a molecular C60-junction under finite bias voltage using first-principles calculations based on density functional theory and nonequilibrium Green's functions (DFT-NEGF). At the…

介观与纳米尺度物理 · 物理学 2013-02-04 Søren Ulstrup , Thomas Frederiksen , Mads Brandbyge

We present a qualitative model for a fundamental process in molecular electronics: the change in conductance upon bond breaking. In our model a diatomic molecule is attached to spin-polarized contacts. Employing a Hubbard Hamiltonian,…

材料科学 · 物理学 2008-06-24 Ali Goker , Francois Goyer , Matthias Ernzerhof

Two dimensional electron gases in narrow GaAs quantum wells show huge longitudinal resistance (HLR) values at certain fractional filling factors. Applying an RF field with frequencies corresponding to the nuclear spin splittings of {69}Ga,…

介观与纳米尺度物理 · 物理学 2009-10-31 S. Kronmueller , W. Dietsche , K. v. Klitzing , G. Denninger , W. Wegscheider , M. Bichler