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We present numerically exact results for the quantum coherent energy transfer in the Fenna-Matthews-Olson molecular aggregate under realistic physiological conditions, including vibrational fluctuations of the protein and the pigments for…

介观与纳米尺度物理 · 物理学 2011-12-06 Peter Nalbach , Daniel Braun , Michael Thorwart

High-energy physics simulations traditionally rely on classical Monte Carlo methods to model complex particle interactions, often incurring significant computational costs. In this paper, we introduce a novel quantum-enhanced simulation…

量子物理 · 物理学 2025-02-28 Euimin Lee , Sangmin Lee , Shiho Kim

This paper reviews recent advances in continuous-time quantum walks (CTQW) and their application to transport in various systems. The introduction gives a brief survey of the historical background of CTQW. After a short outline of the…

量子物理 · 物理学 2015-05-27 Oliver Muelken , Alexander Blumen

A single photon source is a key enabling technology in device-independent quantum communication, quantum simulation for instance boson sampling, linear optics-based and measurement-based quantum computing. These applications involve many…

Photon storage with 250 ps rise time of the readout optical signal was implemented with indirect excitons in coupled quantum well nanostructures (CQW). The storage and release of photons was controlled by the gate voltage pulse. The…

介观与纳米尺度物理 · 物理学 2010-03-19 A. G. Winbow , L. V. Butov , A. C. Gossard

We have developed a full quantum microscopic theory to analyze the time evolution of transversal and longitudinal components of an exciton-single photon system coupled to bulk acoustic phonons. These components are subjected to two decay…

量子物理 · 物理学 2009-11-13 Kunihiro Kojima , Akihisa Tomita

Recent developments in nanoscale experimental techniques made it possible to utilize single molecule junctions as devices for electronics and energy transfer with quantum coherence playing an important role in their thermoelectric…

介观与纳米尺度物理 · 物理学 2018-03-12 Feng Chen , Yi Gao , Michael Galperin

Recent ultrafast optical experiments show that excitons in large biological light-harvesting complexes are coupled to molecular vibration modes. These high-frequency vibrations will not only affect the optical response, but also drive the…

量子物理 · 物理学 2015-02-12 Arend G. Dijkstra , Chen Wang , Jianshu Cao , Graham R. Fleming

Photosynthesis has been a long-standing research interest due to its fundamental importance. Recently, studies on photosynthesis processes also have inspired attention from a thermodynamical aspect when considering photosynthetic…

化学物理 · 物理学 2016-11-03 Hong-Bin Chen , Pin-Yi Chiu , Yueh-Nan Chen

We prove analytical results showing that decoherence can be useful for mixing time in a continuous-time quantum walk on finite cycles. This complements the numerical observations by Kendon and Tregenna (Physical Review A 67 (2003), 042315)…

量子物理 · 物理学 2007-05-23 Leonid Fedichkin , Dmitry Solenov , Christino Tamon

The charge photogeneration process in organic molecules is investigated by a quantum heat engine model, in which two molecules are modeled by a two-spin system sandwiched between two bosonic baths at their own temperatures. The two baths…

介观与纳米尺度物理 · 物理学 2015-01-22 Yao Yao

Engineering and harnessing coherent excitonic transport in organic nanostructures has recently been suggested as a promising way towards improving man-made light harvesting materials. However, realising and testing the dissipative…

量子物理 · 物理学 2018-06-19 A. W. Chin , E. Mangaud , O. Atabek , M. Desouter-Lecomte

In a Quantum Walk (QW) the "walker" follows all possible paths at once through the principle of quantum superposition, differentiating itself from classical random walks where one random path is taken at a time. This facilitates the…

We study a large number of physically-plausible arrangements of chromophores, generated via a computational method involving stochastic real-space transformations of a naturally occurring `reference' structure, illustrating our methodology…

化学物理 · 物理学 2017-05-23 George C. Knee , Patrick Rowe , Luke D. Smith , Alessandro Troisi , Animesh Datta

We show by general arguments that networks whose density of states contains few highly degenerate eigenvalues result in inefficient performances of continuous-time quantum walks (CTQW) over these networks, while systems whose eigenvalues…

量子物理 · 物理学 2007-10-19 Oliver Muelken

Many disordered systems show a superdiffusive dynamics, intermediate between the diffusive one, typical of a classical stochastic process, and the so called ballistic behaviour, which is generally expected for the spreading in a quantum…

Energy transfer between chromophores in photosynthesis proceeds with near unity quantum efficiency. Understanding the precise mechanisms of these processes is made difficult by the complexity of the electronic structure and interactions…

化学物理 · 物理学 2015-03-03 Gethin H. Richards , Krystyna E. Wilk , Paul M. G. Curmi , Jeffrey A. Davis

Non-Markovian and non-equilibrium phonon effects are believed to be key ingredients in the energy transfer in photosynthetic complexes, especially in complexes which exhibit a regime of intermediate exciton-phonon coupling. In this work, we…

量子物理 · 物理学 2011-07-08 Patrick Rebentrost , Alán Aspuru-Guzik

We present an introduction to coined quantum walks on regular graphs, which have been developed in the past few years as an alternative to quantum Fourier transforms for underpinning algorithms for quantum computation. We then describe our…

量子物理 · 物理学 2018-03-28 Viv Kendon , Ben Tregenna

Revealing the role of quantum entanglement in charge-transport in the Photosystem II reaction center (PSII RC) is of great significance. In this work, we theoretically demonstrate that the robust quantum entanglement provides regulatory…

化学物理 · 物理学 2025-01-14 Ling-Fang Li , Shun-Cai Zhao , Lu-Xin Xu