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Long-lived quantum speedup serves as a fundamental component for quantum algorithms. The quantum walk is identified as an ideal scheme to realize the long-lived quantum speedup. However, one finds that the duration of quantum speedup is…

光学 · 物理学 2019-05-22 Jun Ren , Tian Chen , Xiangdong Zhang

Recent findings suggest that processes such as the electronic energy transfer through the photosynthetic antenna display quantal features, aspects known from the dynamics of charge carriers along polymer backbones. Hence, in modeling energy…

量子物理 · 物理学 2015-05-13 Elena Agliari , Oliver Muelken , Alexander Blumen

Escaping from a complex maze, by exploring different paths with several decision-making branches in order to reach the exit, has always been a very challenging and fascinating task. Wave field and quantum objects may explore a complex…

The theoretical and experimental study of energy transfer in photosynthesis has revealed an interesting transport regime, which lies at the borderline between classical transport dynamics and quantum-mechanical interference effects.…

生物物理 · 物理学 2014-02-13 Tobias Kramer , Christoph Kreisbeck

The dynamics of the excitation energy transfer (EET) in photosynthetic complexes is an interesting question both from the perspective of fundamental understanding and the research in artificial photosynthesis. Challenges persist in…

化学物理 · 物理学 2024-06-25 Amartya Bose , Peter L. Walters

Long-lived exciton coherences have been recently observed in photosynthetic complexes via ultrafast spectroscopy, opening exciting possibilities for the study and design of coherent exciton transport. Yet, ambiguity in the spectroscopic…

A non-trivial interplay between quantum coherence and dissipative environment-driven dynamics is becoming increasingly recognised as key for efficient energy transport in photosynthetic pigment-protein complexes, and converting these…

量子物理 · 物理学 2013-03-19 M. del Rey , A. W. Chin , S. F. Huelga , M. B. Plenio

Quantum walks (QWs) represent pillars of quantum dynamics and information processing. They provide a powerful framework for simulating quantum transport, designing search algorithms, and enabling universal quantum computation. Several…

量子物理 · 物理学 2026-01-30 E. Stefanutti , J. Philipps , J. Buetow , A. Guidara , M. Nuvoli , A. Chiuri , L. Sansoni

Near-unity energy transfer efficiency has been widely observed in natural photosynthetic complexes. This phenomenon has attracted broad interest from different fields, such as physics, biology, chemistry and material science, as it may…

We consider the quantum mechanical transport of (coherent) excitons on small-world networks (SWN). The SWN are build from a one-dimensional ring of N nodes by randomly introducing B additional bonds between them. The exciton dynamics is…

量子物理 · 物理学 2009-11-13 Oliver Muelken , Volker Pernice , Alexander Blumen

Photosynthetic proteins have evolved over billions of years so as to undergo optimal energy transfer to the sites of charge separation. Based on spectroscopically detected quantum coherences, it has been suggested that this energy transfer…

化学物理 · 物理学 2016-07-13 David Paleček , Petra Edlund , Sebastian Westenhoff , Donatas Zigmantas

The question of how quantum coherence facilitates energy transfer has been intensively debated in the scientific community. Since natural and artificial light-harvesting units operate under the stationary condition, we address this question…

化学物理 · 物理学 2020-07-22 Pei-Yun Yang , Jianshu Cao

Photosynthetic antenna complexes achieve high quantum efficiency through exciton transport in coupled pigment networks. Conventional Frenkel-exciton models treat each chromophore as a structureless site and neglect internal electronic…

光学 · 物理学 2026-04-01 Jingyu Liu , Tao-Yuan Du

The high quantum efficiency of photosynthetic complexes has inspired researchers to explore new routes to utilize this process for photovoltaic devices. Quantum coherence has been demonstrated to play a crucial role within this process.…

化学物理 · 物理学 2015-06-23 Yiteng Zhang , Sangchul Oh , Fahhad H. Alharbi , Greg Engel , Sabre Kais

Transport phenomena in photosynthetic systems have attracted a great deal of attention due to their potential role in devising novel photovoltaic materials. In particular, energy transport in light-harvesting complexes is considered quite…

Excitonic transport in photosynthesis exhibits a wide range of time scales. Absorption and initial relaxation takes place over tens of femtoseconds. Excitonic lifetimes are on the order of a nanosecond. Hopping rates, energy differences…

量子物理 · 物理学 2011-11-22 Seth Lloyd , Masoud Mohseni , Alireza Shabani , Herschel Rabitz

Quantum walks have a host of applications, ranging from quantum computing to the simulation of biological systems. We present an intrinsically stable, deterministic implementation of discrete quantum walks with single photons in space. The…

量子物理 · 物理学 2010-04-21 M. A. Broome , A. Fedrizzi , B. P. Lanyon , I. Kassal , A. Aspuru-Guzik , A. G. White

Using methods of condensed matter and statistical physics, we examine the transport of excitons through the Fenna-Matthews-Olson (FMO) complex from a receiving antenna to a reaction center. Writing the equations of motion for the exciton…

生物物理 · 物理学 2016-02-23 Lev Mourokh , Franco Nori

The quantum dynamics of transport networks in the presence of noisy environments have recently received renewed attention with the discovery of long-lived coherences in different photosynthetic complexes. This experimental evidence has…

生物物理 · 物理学 2015-06-04 A. W. Chin , S. F. Huelga , M. B. Plenio

We propose a driven optical cavity quantum electrodynamics (QED) set up aimed at directly probing energy transport dynamics in photosynthetic biomolecules. We show that detailed information concerning energy transfer paths and…