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A simple model is presented to calculate the potential of mean force between a polyion and a multivalent counterion inside a polyelectrolite solution. We find that under certain conditions the electrostatic interactions can lead to a strong…

统计力学 · 物理学 2009-11-11 Jürgen F. Stilck , Yan Levin

In this paper we demonstrate a quantitative way to measure the membrane potential of live cells by dielectric spectroscopy. We also show that the values of the membrane potential obtained using our technique are in good agreement with those…

软凝聚态物质 · 物理学 2009-09-15 Corina Bot , Camelia Prodan

We examine the interactions between polyelectrolytes (PEs) and uncharged substrates at conditions corresponding to a dielectric discontinuity between the aqueous solution and the substrate. To this end, we vary the relevant system…

软凝聚态物质 · 物理学 2024-12-03 Hossein Vahid , Alberto Scacchi , Maria Sammalkorpi , Tapio Ala-Nissila

We investigate the thermodynamic properties of a polyelectrolyte solution in a presence of {\it multivalent} salts. The polyions are modeled as rigid cylinders with the charge distributed uniformly along the major axis. The solution,…

凝聚态物理 · 物理学 2015-06-25 Paulo S. Kuhn , Yan Levin , Marcia C. Barbosa

By using a method, previously established to calculate electromagnetic fields, we compute the force of light upon a metallic particle. This procedure is based on both Maxwell's Stress Tensor and the Couple Dipole Method. With these tools,…

光学 · 物理学 2009-11-10 P. C. Chaumet , M. Nieto-Vesperinas

Counterion distribution around an isolated flexible polyelectrolyte in the presence of a divalent salt is evaluated using the adsorption model [M. Muthukumar, J. Chem. Phys. {\bf 120}, 9343 (2004)] that considers Bjerrum length, salt…

软凝聚态物质 · 物理学 2008-12-29 Arindam Kundagrami , M. Muthukumar

This chapter deals with charged polymers (polyelectrolytes) in solution and at surfaces. The behavior of polyelectrolytes is markedly different from that of neutral polymers. In bulk solutions, i.e. disregarding the surface effect, there…

软凝聚态物质 · 物理学 2009-09-25 Roland R. Netz , David Andelman

This study uses advanced numerical methods to estimate the mean force potential (PMF) between charged, polarizable colloidal particles in dense electrolytes. We observe that when the Debye screening length, $\lambda_{\mathrm{D}}$, is below…

软凝聚态物质 · 物理学 2025-02-10 Emily Krucker-Velasquez , Martin Z. Bazant , Alfredo Alexander-Katz , James W. Swan

Polyelectrolytes under confinement are crucial for energy storage and for understanding biomolecular functions. Using molecular dynamics simulations, we analyze a polyelectrolyte solution confined between two oppositely charged planar…

统计力学 · 物理学 2019-06-05 Debarshee Bagchi , Trung Dac Nguyen , Monica Olvera de la Cruz

The exact wave functions, which describe the states of an electron, bound in the image potential, and the magnetic field, which is perpendicular to surface of a metal, are obtained. The correction terms to the energy of an electron in the…

量子物理 · 物理学 2015-02-24 P. A. Golovinski , M. A. Preobrazhenskiy

The in-plane polarizational stopping power of heavy-ion diclusters in a two-dimensional strongly coupled electron liquid is studied. Analytical expressions for the stopping power of both fast and slow projectiles are derived. To go beyond…

强关联电子 · 物理学 2007-10-17 D. Ballester , A. M. Fuentes , I. M. Tkachenko

Stretching dynamics of polymers in microfluidics is of particular interest for polymer scientists. As a charged polymer, a polyelectrolyte can be deformed from its coiled equilibrium configuration to an extended chain by applying uniform or…

软凝聚态物质 · 物理学 2014-11-18 Farnoush Farahpour , Fathollah Varnik , Mohammad Reza Ejtehadi

We utilize the self-consistent field theory to explore the mechanical and electrical properties of charged surfaces immersed in polyelectrolyte solutions that could be potentially useful for electrochemical applications. Our research…

软凝聚态物质 · 物理学 2023-08-25 Yu. A. Budkov , N. N. Kalikin

Recent molecular simulation and integral equation results alkali-halide ion pair potentials-of-mean-force in water are discussed. Dielectric model calculations are implemented to check that these models produce that characteristic structure…

chem-ph · 物理学 2008-02-03 Lawrence R. Pratt , Gerhard Hummer , Angel E. Garcia

The association between polyelectrolytes (PEs) of the same size but opposite charge is systematically studied in terms of the potential of mean force (PMF) along their center-of-mass reaction coordinate via coarse-grained, implicit-solvent,…

软凝聚态物质 · 物理学 2017-06-05 Xiao Xu , Matej Kanduč , Jianzhong Wu , Joachim Dzubiella

We explore, using the recently developed efficient Monte Carlo simulation method, the interaction of an anionic polyelectrolyte solution with a like-charged dielectric surface. In addition to polyions, the solution also contains salt with…

软凝聚态物质 · 物理学 2018-01-12 Alexandre P. dos Santos , Matheus Girotto , Yan Levin

In this work we theoretically study the differential capacitance of an aqueous electrolyte in contact with a planar electrode, using classical Density Functional Theory, and show how this measurable quantity can be used as a probe to better…

软凝聚态物质 · 物理学 2021-09-16 Peter Cats , René van Roij

An overview of the latest theoretical developments and results on electromagnetic and weak probes in relativistic heavy-ion collisions is presented. The possibilities to use electromagnetic probes, i.e., photons and dileptons, as a…

高能物理 - 唯象学 · 物理学 2021-02-03 Ralf-Arno Tripolt

Mobile charge in an electrolytic solution can in principle be represented as the divergence of ionic polarization. After adding explicit solvent polarization a finite volume of electrolyte can then be treated as a composite non-uniform…

软凝聚态物质 · 物理学 2021-03-03 Michiel Sprik

The inelastic scattering of electrons is one route to study the vibrational and electronic properties of materials. Such experiments, also called electron energy-loss spectroscopy, are particularly useful for the investigation of the…

材料科学 · 物理学 2014-06-24 Friedrich Roth , Andreas König , Jörg Fink , Bernd Büchner , Martin Knupfer
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