相关论文: Enantio-discrimination via light deflection effect
We present an optical "enantio-selective switch", that, in two steps, turns a ("racemic") mixture of left-handed and right-handed chiral molecules into the enantiomerically pure state of interest. The optical switch is composed of an…
Circular dichroism spectroscopy is an essential technique for understanding molecular structure and magnetic materials, but spatial resolution is limited by the wavelength of light, and sensitivity sufficient for single-molecule…
Here we highlight enantioselective optical gradient forces present in 3D structured optical vortex tweezing systems. One chiral force originates from the circular polarization of the light, while remarkably the other is independent of the…
We have investigated multiple scattering of light in systems subject to magneto-chiral (MC) effects. Our medium consists of magneto-optically active dipoles placed in a chiral geometry under the influence of an external magnetic field. We…
We show that the photoelectron angular distributions produced by elliptical and cross-polarized two-color laser fields interacting with randomly oriented chiral molecules decompose into four irreducible representations of the $D_{2h}$ point…
We present a semi-classical theory for light deflection by a coherent $\Lambda$-type three-level atomic medium in an inhomogeneous magnetic field or an inhomogeneous control laser. When the atomic energy levels (or the Rabi coupling by the…
Molecular chirality detection and enantiomer discrimination are very important issues for many areas of science and technology, prompting intensive investigations via optical methods. However, these methods are hindered by the intrinsically…
Shaping single-mode operation in high-power fibres requires a precise knowledge of the gain-medium optical properties. This requires accurate measurements of the refractive index differences ($\Delta$n) between the core and the cladding of…
We study the coherent propagation of light whose dynamics is governed by the effective Schr\"{o}dinger equation derived in a magneto-optically-manipulated atomic ensemble with a four-level tripod configuration for electromagnetically…
The practical applications of chiral discrimination are usually limited by the weak chiral response of enantiomers and the high complexity of detection methods. Here, we propose to use the C lines (i.e., lines of polarization singularities)…
This paper presents a algebraic analysis of electromagnetic chirality-induced negative refractive index in a four-level atomic medium. According to analyze mathematically its argument of the complex refractive index for one circular…
We explore the spatial enantioseparation of gaseous chiral molecules for the cyclic three-level systems coupled with three electromagnetic fields. Due to molecular rotations, the specific requirements of the polarization directions of the…
Chirality, the absence of mirror symmetry, is a fundamental molecular property with far-reaching consequences from chemistry to biology. Yet enantiosensitive optical responses are very weak. Here, we introduce a theoretical framework in…
Synthetic chiral light enables ultrafast and highly efficient imaging of molecular chirality. Unlike standard circularly polarized light, the handedness of synthetic chiral light does not rely on the spatial structure of the light field: it…
We propose a chiral imaging modality based on optical chirality engineering, fluorescence-detected circular dichroism and structured illumination microscopy. In this method, the optical chirality of the illumination is structured and the…
The search of chiral magnetic effect (CME) in heavy-ion collisions has attracted long-term attentions. Multiple observables have been proposed but all suffer from obstacles due to large background contaminations. In this Letter, we…
We suggest a scheme of electromagnetic chirality-induced negative refraction utilizing magneto-electric cross coupling in a four-level atomic system. The negative refraction can be achieved with the two chirality coefficients having the…
Chirality is ubiquitous in nature and of fundamental importance in science. The present work focuses on understanding the conditions required to modify the chirality during ultrafast electronic motion by bringing enantiomers…
Chiral molecules show differences in their chemical and optical properties due to different spatial arrangements of the atoms in the two enantiomers. A common way to optically differentiate them is to detect the disparity in the absorption…
Mirror symmetry is among the most fundamental concepts of physics and its spontaneous breaking at the molecular level allows chiral molecules to exist in two enantiomers that are mirror images of each other. The majority of chiro-optical…