相关论文: Diffusiophoresis, Batchelor scale and effective P\…
Mixing a passive scalar field by stirring can be measured in a variety of ways including tracer particle dispersion, via the flux-gradient relationship, or by suppression of scalar concentration variations in the presence of inhomogeneous…
Monte Carlo simulations in the grand canonical ensemble were used to obtain critical parameters and conditions leading to microphase separation for block copolymers with solvophilic and solvophobic segments. Solvent selectivity was…
We study many-particle diffusion in 2D colloidal suspensions with full hydrodynamic interactions through a novel mesoscopic simulation technique. We focus on the behaviour of the effective scaled tracer and collective diffusion coefficients…
Mixing at the microfluidic scale is challenging due to the low Reynolds numbers and often high P\'eclet numbers. Without turbulence, mixing relies solely on diffusion, resulting in slow and inefficient mixing. We demonstrate enhanced mixing…
Double-diffusive convection refers to mixing where the effects of thermal and composition gradients compete to determine the stability of a fluid. In addition to the familiar fast convective instability, such fluids exhibit the slow, direct…
A migration of charged particles relative to a solvent, caused by a gradient of salt concentration and termed a diffusiophoresis, is of much interest being exploited in many fields. Existing theories deal with diffusiophoresis of passive…
To understand the performance of popular density-functional theory (DFT) exchange-correlation (xc) functionals in simulations of liquid water, water monomers and dimers were extracted from a PBE simulation of liquid water and examined with…
In this work, we numerically investigate the impact of two-dimensional solute gradients on the distribution of colloidal particles, i.e., colloidal banding, induced via diffusiophoresis. The solute gradients are generated by spatially…
Lagrangian particle-tracking methods are particularly suitable to study solute transport in velocity fields displaying chaotic advection. They can accurately resolve stretching and folding processes, the increase in the solute-solvent…
Mixing of miscible liquids is an essential process in multiple industrial settings, usually with the intent to homogenize the product. This seemingly simple process is in fact a complex hydrodynamic problem that has a direct impact on the…
We study how varying the P \'eclet number (Pe) affects the steady state sedimentation of colloidal particles that interact through short-ranged attractions. By employing a hybrid molecular dynamics simulation method we demonstrate that the…
We theoretically and numerically investigate the instabilities driven by diffusiophoretic flow, caused by a solutal concentration gradient along a reacting surface. The important control parameter is the Peclet number Pe, which quantifies…
Solute-surface interactions have garnered considerable interest in recent years as a novel control mechanism for driving unique fluid dynamics and particle transport with potential applications in fields such as biomedicine, the development…
We quantitatively study the interaction between diffusion and mixing in both the continuous, and discrete time setting. In discrete time, we consider a mixing dynamical system interposed with diffusion. In continuous time, we consider the…
The current view about the mixing of heat and salt in the ocean is that it should be parameterised by means of a rotated diffusion tensor based on mixing directions parallel and perpendicular to the local neutral vector. However, the…
We investigate the mixing properties of scalars stirred by spatially smooth, divergence-free flows and maintained by a steady source-sink distribution. We focus on the spatial variation of the scalar field, described by the {\it dissipation…
We reveal an unreported physical mechanism that enables the pre-concentration, sorting and characterization of charged polystyrene nanobeads and liposomes dispersed in a continuous flow within a straight micron-sized channel. Initially, a…
A standard model for the study of scalar dispersion through advection and molecular diffusion is a two-dimensional periodic flow with closed streamlines inside periodic cells. Over long time scales, the dispersion of a scalar in this flow…
Intermolecular correlations in liquid water at ambient conditions have generally been characterized through short range density fluctuations described through the atomic pair distribution functions (PDF). Recent numerical and experimental…
Current theories of diffusiophoresis in porous media are limited to a porous medium saturated with a valence symmetric electrolyte. A predictive model for diffusiophoresis in porous media saturated with a valence asymmetric electrolyte, or…