相关论文: Higher-order photon correlation as a tool to study…
We present a fully three-dimensional study of the multiexciton optical response of vertically coupled GaN-based quantum dots via a direct-diagonalization approach. The proposed analysis is crucial in understanding the fundamental properties…
Multi-exciton correlations shape the photo-induced response of nanostructured materials, particularly when interactions are enhanced by light confinement. Here multidimensional coherent spectroscopy is used to quantify biexciton and…
Two-dimensional (2D) semiconducting materials are promising building blocks for optoelectronic applications, many of which require efficient dissociation of excitons into free electrons and holes. However, the strongly bound excitons…
In semiconductor nanostructures, optical excitation typically creates bound electron-hole states, such as excitons, trions, and larger complexes. Their relative motion is described by the Wannier equation, which is valid only for spatially…
Two-dimensional magnetic semiconductors provide a unique materials platform in which long-range magnetic order coexists with strongly bound excitons. Because excitonic states and magnetic moments originate from the same electronic orbitals…
Atomically thin semiconductors exhibit tunable exciton resonances that can be harnessed for dynamic manipulation of visible light in ultra-compact metadevices. However, the rapid nonradiative decay and dephasing of excitons at room…
We address spin properties and spin dynamics of carriers and charged excitons in CdSe/CdS colloidal nanoplatelets with thick shells. Magneto-optical studies are performed by time-resolved and polarization-resolved photoluminescence,…
Harnessing the optoelectronic response of organic semiconductors requires a thorough understanding of the fundamental light-matter interaction that is dominated by the excitation of correlated electron-hole pairs, i.e. excitons. The nature…
Colloidal semiconductor nanoplatelets (NPLs) with electronic structure as quantum wells have recently emerged as exciting materials for optoelectronic applications. Here we investigate how morphology affects important photoluminescence (PL)…
Tailoring and enhancing the interaction between light and matter is of great importance for both fundamental researches and future photonic and optoelectronic applications. Due to their high exciton oscillator strength and large exciton…
Polariton emission from optical cavities integrated with various luminophores has been extensively studied recently due to the wide variety of possible applications in photonics, particularly promising in terms of fabrication of…
Excitons and their correlated complexes underpin the rich photophysics of quantum-confined semiconductors. Among these, biexcitons -- bound states of two electrons and two holes -- provide a sensitive probe of Coulomb correlations,…
We show that the nonlinear optical response probed by two-dimensional coherent spectroscopy (2DCS) can discriminate between excitonic and lattice driven order. In the excitonic regime of a realistic model of Ta$_2$NiSe$_5$, the third order…
Harnessing quantum correlations between photons is an emerging frontier in optical spectroscopy, yet experimental demonstrations have largely remained limited to molecular systems at room temperature. Here, we investigate heralded emission…
The correlated Stoke antiStokes (SaS) scattering plays a crucial role in quantum information processing, such as heralded light sources, Fock state dynamics, and write read protocol for quantum memory. However, several reported materials…
Colloidal core/shell InP/ZnSe quantum dots (QDs), recently produced using an improved synthesis method, have a great potential in life-science applications as well as in integrated quantum photonics and quantum information processing as…
Quantum dots acting as single photon emitters in the blue-green range are fabricated and characterized at cryogenic temperature. They consist in CdSe dots inserted in (Zn,Mg)Se nanowires with a thick shell. Photoluminescence spectra, decay…
We derive a rigorous theory of the interaction between photons and spatially extended excitons confined in quantum dots in inhomogeneous photonic materials. We show that, beyond the dipole approximation, the radiative decay rate is…
Excitons are widely found in semiconductors. In contrast to inorganic-based semiconductors, where the presence of excitons may need special morphonology, like low-dimensional layer structure, the excitons prevailingly exist in molecular…
The exciton spin dynamics and polarization properties of the related emission are investigated in colloidal CdSe/CdS dot-in-rod (DiR) and spherical core/shell nanocrystal (NC) ensembles by magneto-optical photoluminescence (PL) spectroscopy…