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相关论文: Evolution of structure and magnetism across the me…

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Tuning of spin-orbit coupling and electron correlation effects in pyrochlore iridates is considered for many interesting phenomena. We have investigated the temperature evolution of structural, magnetic and electronic properties in doped…

强关联电子 · 物理学 2019-05-07 Harish Kumar , A. K. Pramanik

Combining density functional theory (DFT) and embedded dynamical mean-field theory (DMFT) methods, we study the metal-insulator transition in $R_2$Ir$_2$O$_7$ ($R$=Y, Eu, Sm, Nd, Pr, and Bi) and the topological nature of the insulating…

强关联电子 · 物理学 2017-01-18 Hongbin Zhang , Kristjan Haule , David Vanderbilt

In this study, we performed powder neutron diffraction and inelastic scattering measurements of frustrated pyrochlore Nd$_2$Ir$_2$O$_7$, which exhibits a metal-insulator transition at a temperature $T_{\rm MI}$ of 33 K. The diffraction…

强关联电子 · 物理学 2012-02-29 K. Tomiyasu , K. Matsuhira , K. Iwasa , M. Watahiki , S. Takagi , M. Wakeshima , Y. Hinatsu , M. Yokoyama , K. Ohoyama , K. Yamada

The interplay between spin-orbit coupling (SOC) and electron correlation ($U$) is considered for many exotic phenomena in iridium oxides. We have investigated the evolution of structural, magnetic and electronic properties in pyrochlore…

强关联电子 · 物理学 2017-03-08 Harish Kumar , R. S. Dhaka , A. K. Pramanik

In this study, we employ bulk electronic properties characterization and x-ray scattering/spectroscopy techniques to map the structural, magnetic and electronic properties of (Eu$_{1-x}$Ca$_{x}$)$_{2}$Ir$_{2}$O$_{7}$ as a function of…

强关联电子 · 物理学 2021-08-03 E. Zoghlin , Z. Porter , S. Britner , S. Husremovic , Y. Choi , D. Haskel , G. Laurita , S. D. Wilson

We report study of magnetization, resistivity, magnetoresistance and specific heat of the pyrochlore Iridate (Eu1-xNdx)2Ir2O7 with x=0.0, 0.5 and 1.0, where spin orbit coupling, electronic correlation, magnetic frustration and Kondo…

强关联电子 · 物理学 2020-12-02 Sampad Mondal , M. Modak , B. Maji , M. K. Ray , S. Mandal , Swapan K. Mandal , M. Sardar , S. Banerjee

The electronic structures of the metallic and insulating phases of the alloy series Ca(2-x)Sr(x)RuO4 (0 <= x <= 2) are calculated using LDA, LDA+U and Dynamical Mean-Field Approximation methods. In the end members the groundstate…

强关联电子 · 物理学 2009-09-25 V. I. Anisimov , I. A. Nekrasov , D. E. Kondakov , T. M. Rice , M. Sigrist

We address the concomitant metal-insulator transition (MIT) and antiferromagnetic ordering in the novel pyrochlore iridate Eu2Ir2O7 by combining x-ray absorption spectroscopy, x-ray and neutron diffractions and density functional theory…

We study structurally-triggered metal-insulator transition in CaCu$_3$Fe$_4$O$_{12}$ by means of local density approximation (LDA) +$U$ and LDA+dynamical mean-field theory (DMFT). The ferrimagnetic insulating phase is essentially the same…

强关联电子 · 物理学 2024-09-30 Atsushi Hariki , Tatsuya Yamaguchi , Mathias Winder , Jan Kuneš

The $f$-$d$ magnetic exchange interaction is considered to be a key ingredient for many exotic topological phases in pyrochlore iridates. Here, we have investigated the evolution of structural, magnetic and electronic properties in doped…

强关联电子 · 物理学 2020-02-07 Harish Kumar , K. C. Kharkwal , Kranti Kumar , K. Asokan , A. Banerjee , A. K. Pramanik

We report structural, magnetic, transport and thermal properties of single-crystal Ca2Ru1-xIrxO4 (0 < x< 0.65). Ca2RuO4 is a structurally-driven Mott insulator with a metal-insulator transition at TMI = 357 K, which is well separated from…

强关联电子 · 物理学 2016-04-26 S. J. Yuan , J. Terzic , J. C. Wang , S. Aswartham , W. H. Song , F. Ye , G. Cao

In 5d transition metal oxides such as the iridates, novel properties arise from the interplay of electron correlations and spin-orbit interactions. We investigate the electronic structure of the pyrochlore iridates, (such as…

强关联电子 · 物理学 2015-05-19 Xiangang Wan , Ari Turner , Ashvin Vishwanath , Sergey Y. Savrasov

We have explored the critical metal-insulator phenomena for pyrochlore-type $R_2$Ir$_2$O$_7$, in which electron correlation strength and magnetic configuration are systematically controlled by varying the average rare-earth ionic radius…

强关联电子 · 物理学 2015-10-28 K. Ueda , J. Fujioka , C. Terakura , Y. Tokura

We have studied the effect of nonmagnetic Ti substitution Eu2(Ir1-xTix)2O7 with the help of electrical transport and magnetic measurement. The minor structural modification enhances the orbital overlapping and favours its electrical…

强关联电子 · 物理学 2024-07-09 Sampad Mondal , B. Maji , M. Modak , Swapan K. Mandal , S. Banerjee

We present an angle-resolved photoemission study of the electronic structure of the three-dimensional pyrochlore iridate Nd2Ir2O7 through its magnetic metal-insulator transition. Our data reveal that metallic Nd2Ir2O7 has a quadratic band,…

Cd2Os2O7 crystallizes in the pyrochlore structure and undergoes a metal-insulator transition (MIT) near 226 K. We have characterized the MIT in Cd2Os2O7 using X-ray diffraction, resistivity at ambient and high pressure, specific heat,…

A2Ir2O7 iridates were proven to crystallise in the geometrically frustrated pyrochlore structure, which remains stable upon rare-earth cation substitution, temperature variation, and external pressure application. However, the change of…

强关联电子 · 物理学 2024-08-05 Daniel Staško , Petr Proschek , Jiří Prchal , Milan Klicpera

We have investigated the effect of Cu substitution in Eu2(Ir1-xCux)2O7 with the help of magnetic and transport property measurements. XPS measurement reveals that each Cu2+ converts Ir4+ to double amount of Ir5+ ions. The metal-insulator…

强关联电子 · 物理学 2022-04-20 Sampad Mondal , M. Modak , B. Maji , Swapan K. Mandal , B. Ghosh , Surajit Saha , M. Sardar , S. Banerjee

The effect of isoelectronic substitution within single crystals of (Sr1-xCax)2-yIrO4+z is explored. The nominal n=1 Ruddlesden-Popper phase with y=0, z=0 remains stable from x=0 until x=0.11, where the antiferromagnet spin-orbit Mott…

材料科学 · 物理学 2016-11-23 Xiang Chen , Stephen D. Wilson

Carrier doping to the Mott insulator is essential to produce highly correlated metals with emergent properties. Pyrochlore ruthenates, Pr$_{2}$Ru$_{2}$O$_{7}$ (Ru-$4d$ electron number, $n=4$) and Ca$_{2}$Ru$_{2}$O$_{7}$ ($n=3$), are a Mott…

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