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Metal-insulator transitions involve a mix of charge, spin, and structural degrees of freedom, and when strongly-correlated, can underlay the emergence of exotic quantum states. Mott insulators induced by the opening of a Coulomb gap are an…

强关联电子 · 物理学 2021-05-14 Yejun Feng , Yishu Wang , D. M. Silevitch , S. E. Cooper , D. Mandrus , Patrick A. Lee , T. F. Rosenbaum

Our single crystal study of the magneto-thermal and transport properties of the pyrochlore iridate Eu2Ir2O7 reveals a continuous phase transition from a paramagnetic metal to an antiferromagnetic insulator for a sample with stoichiometry…

强关联电子 · 物理学 2015-06-04 Jun J. Ishikawa , Eoin C. T. O'Farrell , Satoru Nakatsuji

Structural, magnetization and heat capacity studies were performed on Ce$_2$(Pd$_{1-x}$Ni$_x$)$_2$Sn ($0 \leq x \leq 1$) alloys. The substitution of Pd atoms by isoelectronic Ni leads to a change in the crystallographic structure from…

强关联电子 · 物理学 2011-03-02 J. G. Sereni , G. Schmerber , A. Braghta , B. Chevalier , J. P. Kappler

We propose a new mechanism for the paramagnetic metal-insulator transition in the layered perovskite Ca$_{2-x}$Sr$_{x}$RuO$_{4}$ (0<x<0.2). The LDA+U approach including spin-orbit coupling is used to calculate the electronic structures. In…

强关联电子 · 物理学 2015-05-28 Guo-Qiang Liu

Neutron scattering, magnetometry, and muon spin rotation ($\mu$SR) measurements were performed to investigate the magnetic order and spin dynamics across the ferromagnet-to-paramagnet transition in the hole-doped Mott insulator…

强关联电子 · 物理学 2025-02-19 S. Hameed , I. Khayr , J. Joe , G. Q. Zhao , Y. Cai , K. M. Kojima , S. Chi , T. J. Williams , M. Matsuda , Y. J. Uemura , M. Greven

Turning a pristine Mott insulator into a correlated metal by chemical doping is a common procedure in strongly correlated materials physics, e.g. underlying the phenomenology of high-$T_c$ cuprates. The ruthenate bilayer compound…

强关联电子 · 物理学 2020-09-29 Frank Lechermann , Qiang Han , Andrew J. Millis

Magnetic fluctuations in transition metal oxides are a subject of intensive research because of the key role they are expected to play in the transition from the Mott insulator to the unconventional metallic phase of these materials, and…

强关联电子 · 物理学 2016-01-06 J. Gunasekera , L. Harriger , A. Dahal , T. Heitmann , G. Vignale , D. K. Singh

Pyrochlore oxides with chemical formula of A2B2O7 exhibit a diverse range of electronic properties as a representative family of quantum materials. These properties mostly stem from strong electron correlations at the transition metal B…

强关联电子 · 物理学 2025-04-25 Yoshinori Tokura , Yukitoshi Motome , Kentaro Ueda

Multilayer (TiO$_2$)$_m$/(VO$_2$)$_n$ nanostructures ($d^1$ - $d^0$ interfaces with no polar discontinuity) show a metal-insulator transition with respect to the VO$_2$ layer thickness in first principles calculations. For $n$ $\geq$ 5…

强关联电子 · 物理学 2015-05-14 Victor Pardo , Warren E. Pickett

Infrared reflectance measurements were made on the single crystal pyrochlore Cd$_{2}$Os$_{2}$O$_{7}$ in order to examine the transformations of the electronic structure and crystal lattice across the boundary of the metal insulator…

强关联电子 · 物理学 2009-11-07 W. J. Padilla , D. N. Basov , D. Mandrus

The doping induced insulator-metal transition in $La_{1-x}Sr_{x}TiO_{3}$ is studied using the ab-initio LDA+DMFT method. Combining the LDA bandstructure for the actual, distorted structure found recently with multi-orbital DMFT to treat…

强关联电子 · 物理学 2016-08-31 L. Craco , M. S. Laad , S. Leoni , E. Müller-Hartmann

TM-doped IrTe2(TM=Mn, Fe, Co, Ni) compounds were synthesized by solid state reaction. Single crystal x-ray diffraction experiments indicate that part of the doped TM ions (TM=Fe, Co, and Ni) substitute for Ir, and the rest intercalate into…

超导电性 · 物理学 2013-10-18 J. -Q. Yan , B. Saparov , A. S. Sefat , H. Yang , H. B. Cao , H. D. Zhou , B. C. Sales , D. G. Mandrus

The pyrochlore lattice involves corner sharing tetrahedra and the resulting geometric frustration is believed to suppress any antiferromagnetic order for Mott insulators on this structure. There are nevertheless short-range correlations…

强关联电子 · 物理学 2016-10-19 Nyayabanta Swain , Rajarshi Tiwari , Pinaki Majumdar

We report on the study of insulator-to-metal transition in post-perovskite compound CaIrO3. It is discovered that a gradual chemical substitution of calcium by yttrium leads to the onset of strong metallic behavior in this compound. This…

强关联电子 · 物理学 2015-06-19 J. Gunasekera , Y. Chen , J. W. Kremenak , P. F. Miceli , D. K. Singh

Sr2IrO4 exhibits a novel insulating state assisted by spin-orbit interactions. A series of polycrystalline samples of Sr2-xIrO4 have been synthesized. It is found that deep Sr-vacancies of Sr2-xIrO4 greatly reduce the rotation of IrO6…

强关联电子 · 物理学 2016-11-01 Xuanyong Sun , S. L. Liu , Haiyun Wang , Bin Li , Jie Cheng , Z. H. Wang

We show that the pressure-temperature phase diagram of the Mott insulator Ca$_{2}$RuO$_{4}$ features a metal-insulator transition at 0.5GPa: at 300K from paramagnetic insulator to paramagnetic quasi-two-dimensional metal; at $T \leq$ 12K…

We have investigated magneto-transport properties in a single crystal of pyrochore-type Nd2Ir2O7. The metallic conduction is observed on the antiferromagnetic domain walls of the all-in all-out type Ir-5d moment ordered insulating bulk…

材料科学 · 物理学 2016-10-31 K. Ueda , J. Fujioka , B. -J. Yang , J. Shiogai , A. Tsukazaki , S. Nakamura , S. Awaji , N. Nagaosa , Y. Tokura

We present resistivity, magnetization, and zero field muon spin relaxation ($\mu$SR) data for the pyrochlore iridate materials Nd$_{2-x}$Ca$_{x}$Ir$_{2}$O$_{7}$ ($x = 0, 0.06$, and $0.10$) and Sm$_2$Ir$_2$O$_7$. While…

Metal-insulator transitions in pyrochlore iridates (A2Ir2O7) are believed to occur due to subtle interplay of spin-orbit coupling, geometric frustration, and electron interactions. In particular, the nature of magnetic ordering of iridium…

强关联电子 · 物理学 2014-07-29 Eric Kin-Ho Lee , Subhro Bhattacharjee , Yong Baek Kim

The cubic symmetry of pyrochlore iridium oxides R2Ir2O7 (R = Nd, Eu, and Pr) has been investigated by high resolution X-ray diffraction experiments down to 4 K,in order to clarify the relationship between the metal-insulator transition…

强关联电子 · 物理学 2014-12-12 Hiroshi Takatsu , Kunihiko Watanabe , Kazuki Goto , Hiroaki Kadowaki