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Raman scattering in the three-dimensional Dirac semimetal Cd3As2 shows an intricate interplay of electronic and phonon degrees of freedom. We observe resonant phonon scattering due to interband transitions, an anomalous anharmonicity of…

材料科学 · 物理学 2017-07-05 A. Sharafeev , V. Gnezdilov , R. Sankar , F. C. Chou , P. Lemmens

We have used a combination of linear response time-domain THz spectroscopy (TDTS) and high-field non-linear THz spectroscopy to separately probe the electronic momentum and energy relaxation rates respectively of the Dirac semimetal…

A theory of hot electron cooling power due to polar optical phonons $P_{\rm op}$ is developed in three-dimensional Dirac semimetal($3$DDS) Cd$_3$As$_2$ taking account of hot phonon effect. Hot phonon distribution $N_q$ and $P_{\rm op}$ are…

介观与纳米尺度物理 · 物理学 2018-07-04 Shrishail S. Kubakaddi , Tutul Biswas

Dirac semimetal PdTe2 single-crystal temperature-dependent ultrafast carrier and phonon dynamics were studied using ultrafast optical pump-probe spectroscopy. Two distinct carrier and coherent phonons relaxation processes were identified in…

A theoretical model is presented for the phonon limited mobility of the Dirac-Fermion gas in a three-dimensional (3D) Dirac semimetal Cd$_3$As$_2$ considering scattering from both the acoustic and the optical phonons. Screening effects are…

材料科学 · 物理学 2019-08-01 S S Kubakaddi

Phonon measurements in the A15-type superconductors were complicated in the past because of the unavailability of large single crystals for inelastic neutron scattering, e.g., in the case of Nb$_3$Sn, or unfavorable neutron scattering…

超导电性 · 物理学 2019-04-19 A. Sauer , D. A. Zocco , A. H. Said , R. Heid , A. Böhmer , F. Weber

Inelastic x-ray scattering and $ab$-$initio$ calculation are applied to investigate the lattice dynamics and electron-phonon coupling of the ternary silicide superconductor CaAlSi ($P/bar{6}m2$). A soft c-axis polarized mode is clearly…

超导电性 · 物理学 2009-11-13 S. Kuroiwa , A. Q. R. Baron , T. Muranaka , R. Heid , K. -P. Bohnen , J. Akimitsu

The relaxation dynamics of photoexcited quasiparticles of three-dimensional (3D) Dirac semimetals are vital towards their application in high performance electronic and optoelectronic devices. In this work, the relaxation dynamics of…

光学 · 物理学 2018-10-03 Wei Lu , Jiwei Ling , Faxian Xiu , Dong Sun

Fundamental understanding of thermal transport in compounds with ultra-low thermal conductivity remains challenging, primarily due to the limitations of conventional lattice dynamics and heat transport models. In this study, we investigate…

材料科学 · 物理学 2023-11-13 Jiongzhi Zheng , Changpeng Lin , Chongjia Lin , Baoling Huang , Ruiqiang Guo , Geoffroy Hautier

Using finite temperature Raman spectroscopy, we investigate the electron-phonon interactions (EPI) and phonon-phonon scattering dynamics in the Dirac semimetal Cd3As2 in different fre quency regimes. Strong softening of the Raman shifts…

强关联电子 · 物理学 2025-03-04 Debasmita Swain , Akash Dey , Anushree Roy , Kush Saha , Sitikantha D. Das

Model materials are precious test cases for elementary theories and provide building blocks for the understanding of more complex cases. Here, we describe the lattice dynamics of the structural phase transition in francisite…

We use variable-temperature x-ray thermal diffuse scattering and inelastic scattering to investigate the lattice dynamics in single crystals of multiferroic CaMn7O12 which undergo a series of orbital and magnetic transitions at low…

强关联电子 · 物理学 2016-11-24 S. M. Souliou , Y. Li , X. Du , M. Le Tacon , A. Bosak

Optical measurements and band structure calculations are reported on 3D Dirac materials. The electronic properties associated with the Dirac cone are identified in the reflectivity spectra of Cd$_3$As$_2$ and Na$_3$Bi single crystals. In…

BaNi$_2$As$_2$ is a nonmagnetic analogue of the iron pnictide superconductors, and in its tetragonal state exhibits an incommensurate charge-density-wave (IC-CDW) and a sizable elastoresistance. In this work, phonons in BaNi$_2$As$_2$…

The unique structure of two-dimensional (2D) Dirac crystals, with electronic bands linear in the proximity of the Brillouin-zone boundary and the Fermi energy, creates anomalous situations where small Fermi-energy perturbations are known to…

介观与纳米尺度物理 · 物理学 2023-05-24 Sina Kazemian , Giovanni Fanchini

Nanostructured superlattices have been the focus of many researchers due to their physical and manipulatable properties. They aim to find promising materials for new electronic and thermoelectric devices. In the present study, we…

材料科学 · 物理学 2021-07-29 Leila Razzaghi , Farhad Khoeini , Ali Rajabpour , Maryam Khalkhali

This paper reports the first experimental observation of phonons and their softening on single crystalline LaPt$_2$Si$_2$ via inelastic neutron scattering. From the temperature dependence of the phonon frequency in close proximity to the…

Using atomic-force microscopy (AFM) and wide-band (0.02-8.5 eV) spectroscopic ellipsometry techniques we investigated morphology and optical properties of Cd3As2 films grown by non-reactive rf magnetron sputtering on two types of oriented…

材料科学 · 物理学 2023-01-16 Natalia Kovaleva , Ladislav Fekete , Dagmar Chvostova , Andrei Muratov

Topological semimetals are currently attracting increasing interest due to their potential applications in topological qubits and low-power electronics, which are closely related to their thermal transport properties. In this work, by…

材料科学 · 物理学 2018-05-09 San-Dong Guo , Peng Chen

Extensive inelastic neutron scattering measurements of phonons on a single crystal of CaFe2As2 allowed us to establish a fairly complete picture of phonon dispersions in the main symmetry directions. The phonon spectra were also calculated…

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