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The Boson peak is believed to be the key to the fundamental understanding of the anomalous thermodynamic properties of glasses, notably the anomalous peak in the heat capacity at low temperatures; it is believed to be due to an excess of…

软凝聚态物质 · 物理学 2014-03-13 Rojman Zargar , John Russo , Peter Schall , Hajime Tanaka , Daniel Bonn

The excess low-frequency vibrational spectrum, called boson peak, and non-affine elastic response are the most important particularities of glasses. Herein, the vibrational and mechanical properties of polymeric glasses are examined by…

软凝聚态物质 · 物理学 2019-12-24 Naoya Tomoshige , Hideyuki Mizuno , Tatsuya Mori , Kang Kim , Nobuyuki Matubayasi

The inelastic scattering intensities of glasses and amorphous materials has a maximum at a low frequency, the so called Boson peak. Under applied hydrostatic pressure, $P$, the Boson peak frequency, $\omega_{\rm b}$, is shifted upwards. We…

无序系统与神经网络 · 物理学 2009-11-10 V. L. Gurevich , D. A. Parshin , H. R. Schober

We perform extensive molecular dynamics simulations of the TIP4P/2005 model of water to investigate the origin of the Boson peak reported in experiments on supercooled water in nanoconfined pores, and in hydration water around proteins. We…

软凝聚态物质 · 物理学 2013-05-21 Pradeep Kumar , K. Thor Wikfeldt , Daniel Schlesinger , Lars G. M. Pettersson , H. E. Stanley

A close inspection of neutron spectra of glass formers in the frequency region above the boson peak does not show the constant eigenvalue density expected for a random dynamical matrix, but a slow decrease towards higher eigenvalues. In…

无序系统与神经网络 · 物理学 2007-05-23 U. Buchenau , A. Wischnewski , M. Ohl , E. Fabiani

A hallmark of glasses is an excess of low-frequency, nonphononic vibrations, in addition to phonons. It is associated with the intrinsically nonequilibrium and disordered nature of glasses, and is generically manifested as a THz peak -- the…

无序系统与神经网络 · 物理学 2024-09-02 Avraham Moriel , Edan Lerner , Eran Bouchbinder

Glasses are amorphous solids, in the sense that they display elastic behaviour. In crystals, elasticity is associated with phonons, quantized sound-wave excitations. Phonon-like excitations exist also in glasses at very high frequencies…

凝聚态物理 · 物理学 2016-08-31 T. S. Grigera , V. Martin-Mayor , G. Parisi , P. Verrocchio

Despite the presence of topological disorder, phonons seem to exist also in glasses at very high frequencies (THz) and they remarkably persist into the supercooled liquid. A universal feature of such a systems is the Boson peak, an excess…

凝聚态物理 · 物理学 2009-11-10 S. Ciliberti , T. S. Grigera , V. Martin-Mayor , G. Parisi , P. Verrocchio

We investigate a prominent vibrational feature in amorphous silica, the so-called boson peak, by means of molecular dynamics computer simulations. The dynamic structure factor S(q,nu) in the liquid, as well as in the glass state, scales…

统计力学 · 物理学 2009-10-31 Jurgen Horbach , Walter Kob , Kurt Binder

In glasses, atomic disorder combined with atomic connectivity makes understanding of the nature of the vibrations much more complex than in crystals or molecules. With a simple model, however, it is possible to show how disorder generates…

无序系统与神经网络 · 物理学 2019-08-23 B. Hehlen , B. Rufflé

Implications of reduction procedures applied to the low energy part of the vibrational density of states in glasses and supercooled liquids are considered by advancing a detailed comparison between the excess - over the Debye limit -…

无序系统与神经网络 · 物理学 2009-11-11 S. N. Yannopoulos , K. S. Andrikopoulos , G. Ruocco

A hallmark of structural glasses and other disordered solids is the emergence of excess low-frequency vibrations, on top of the Debye spectrum $D_{\rm Debye}(\omega)$ of phonons ($\omega$ denotes the vibrational frequency), which exist in…

软凝聚态物质 · 物理学 2023-08-25 Edan Lerner , Eran Bouchbinder

Boson peak, the excess low energy excitations in the terahertz regime, is one of the most unique features of disordered systems and has been linked to many anomalous properties of glass materials. The nature and structural origin of the…

The boson peak appears in all amorphous solids and is an excess of vibrational states at low frequencies compared to the phonon spectrum of the corresponding crystal. Until recently, the consensus was that it originated from "defects" in…

材料科学 · 物理学 2016-12-16 Tobias Brink , Leonie Koch , Karsten Albe

We present a numerical simulation study of the density-dependence (rho = 2.2 - 4.0 g/cm^3) of the high-energy collective dynamics in vitreous silica at mesoscopic wavevectors (Q = 1 - 18 nm^-1). The density-dependence of the longitudinal…

无序系统与神经网络 · 物理学 2007-05-23 O. Pilla , S. Caponi , A. Fontana , M. Montagna , F. Rossi , G. Viliani , L. Angelani , G. Ruocco , G. Monaco , F. Sette

We show that a {\em vibrational instability} of the spectrum of weakly interacting quasi-local harmonic modes creates the maximum in the inelastic scattering intensity in glasses, the Boson peak. The instability, limited by anharmonicity,…

无序系统与神经网络 · 物理学 2009-11-07 V. L. Gurevich , D. A. Parshin , H. R. Schober

We perform classical molecular-dynamics simulation to study the effect of densification on the vibrational spectrum of a model silica glass. We concentrate this study on the so-called Boson peak and compare our results, obtained from a…

无序系统与神经网络 · 物理学 2009-10-31 P. Jund , R. Jullien

The Boson peak (BP), an excess of vibrational density of states, is ubiquitous for amorphous materials and is believed to hold the key to understanding the dynamics of glass and glass transition. Previous studies have established an energy…

材料科学 · 物理学 2023-11-08 X. Y. Li , H. P. Zhang , S. Lan , D. L. Abernathy , C. H. Hu , L. R. Fan , M. Z. Li , X. -L. Wang

Glasses have a large excess of low-frequency vibrational modes in comparison with continuous elastic body, the so-called Boson Peak, which appears to correlate with several crucial properties of glasses, such as transport or fragility. I…

材料科学 · 物理学 2014-11-19 Matthieu Wyart

Vibrational spectra of proteins and topologically disordered solids display a common anomaly at low frequencies, known as Boson peak. We show that such feature in globular proteins can be deciphered in terms of an energy landscape picture,…

软凝聚态物质 · 物理学 2007-05-23 Stefano Ciliberti , Paolo De Los Rios , Francesco Piazza
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