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Analyzing three approximate methods to locate liquid-solid coexistence in simple systems, an observation is made that all of them predict the same functional dependence of the temperature on density at freezing and melting of the…

软凝聚态物质 · 物理学 2011-11-30 Sergey A. Khrapak , Gregor E. Morfill

Results of a systematic investigation of the vapour-liquid equilibria of 38 individual two-centre Lennard-Jones plus axial pointdipole model fluids (2CLJD) are reported over a range of reduced dipolar momentum 0 $\le \mu^{*2} \le$ 20 and of…

计算物理 · 物理学 2009-04-23 Jürgen Stoll , Jadran Vrabec , Hans Hasse

Molecular dynamic simulations for systems with $D=2,3$ Lennard-Jones-like interactions are studied. In the model, we assume that, at long distances, the two-body attractive potential decays as $r^{-\alpha}$. Thermodynamic extensivity…

凝聚态物理 · 物理学 2009-10-31 Sergio Curilef , Constantino Tsallis

We present a computer simulation study of a (6,12)-Lennard-Jones fluid confined to a slit pore, formed by two uniform planes. These interact via (3,9)-Lennard-Jones potential with the fluid particles. When the fluid approaches the…

软凝聚态物质 · 物理学 2009-02-20 N. Gribova , H. Maleki , A. Arnold , C. Holm , T. Schilling

Results of a systematic investigation of the vapour-liquid equilibria (VLE) of 30 individual two-centre Lennard-Jones plus pointquadrupole model fluids (2CLJQ) are reported over a range of reduced quadrupolar momentum $0 \le Q^{*2} \le 4$…

化学物理 · 物理学 2009-04-24 J. Stoll , J. Vrabec , H. Hasse

This paper investigates the relation between the density-scaling exponent $\gamma$ and the virial potential-energy correlation coefficient $R$ at several thermodynamic state points in three dimensions for the generalized $(2n,n)$…

软凝聚态物质 · 物理学 2024-01-17 Ida M. Friisberg , Lorenzo Costigliola , Jeppe C. Dyre

Linearly-sloped or `ramp' potentials belong to a class of core-softened models which possess a liquid-liquid critical point (LLCP) in addition to the usual liquid-gas critical point. Furthermore they exhibit thermodynamic anomalies in the…

统计力学 · 物理学 2009-11-11 Helen M. Gibson , Nigel B. Wilding

The phase behavior of fluids near weakly attractive substrates is studied by computer simulations of the coexistence curve of a Lennard-Jones (LJ) fluid confined in a slitlike pore. The temperature dependence of the density profiles of the…

统计力学 · 物理学 2009-11-10 I. Brovchenko , A. Geiger , A. Oleinikova

Framing the glass formation within standard statistical mechanics is an outstanding problem of condensed matter theory. To provide new insight, we investigate the structural properties of the Lennard-Jones fluid in the very-low temperature…

统计力学 · 物理学 2026-02-02 Bomont Jean-Marc , Bretonnet Jean-Louis , Costa Dino , Pastore Giorgio

The gas-liquid phase transition of the three-dimensional Lennard-Jones particles system is studied by molecular dynamics simulations. The gas and liquid densities in the coexisting state are determined with high accuracy. The critical point…

统计力学 · 物理学 2013-11-28 Hiroshi Watanabe , Nobuyasu Ito , Chin-Kun Hu

The phase diagram of the prototypical two-dimensional Lennard-Jones system, while extensively investigated, is still debated. In particular, there are controversial results in the literature as concern the existence of the hexatic phase and…

统计力学 · 物理学 2020-12-08 Yan-Wei Li , Massimo Pica Ciamarra

The supercooled dynamics of a Lennard-Jones model liquid is numerically investigated studying relevant points of the potential energy surface, i.e. the minima of the square gradient of total potential energy $V$. The main findings are:…

软凝聚态物质 · 物理学 2009-11-07 L. Angelani , R. Di Leonardo , G. Ruocco , A. Scala , F. Sciortino

We study the dynamics of particles in a multi-component 2d Lennard-Jones (LJ) fluid in the limiting case where {\it all the particles are different} (APD). The equilibrium properties of this APD system were studied in our earlier work…

软凝聚态物质 · 物理学 2016-06-22 Lenin S. Shagolsem , Yitzhak Rabin

We report a theoretical and simulation study of the drying and wetting phase transitions of a truncated Lennard-Jones fluid at a flat structureless wall. Binding potential calculations predict that the nature of these transitions depends on…

统计力学 · 物理学 2017-09-13 Robert Evans , Maria C. Stewart , Nigel B. Wilding

It was recently shown that vapor-liquid coexistence densities derived from Mie and Yukawa models collapse to define a single master curve when represented against the difference between the reduced second virial coefficient at the…

统计力学 · 物理学 2015-07-14 P. Orea , A. Romero-Martínez , E. Basurto , C. A. Vargas , G. Odriozola

We present an application of Wertheim's Thermodynamic Perturbation Theory (TPT1) to a simple coarse grained model made of flexibly bonded Lennard-Jones monomers. We use both the Reference Hyper-Netted-Chain (RHNC) and Mean Spherical…

统计力学 · 物理学 2016-08-15 L. González MacDowell , M. Mueller , C. Vega , K. Binder

The dynamical correlations of a model consisting of particles constrained on the line and interacting with a nearest--neighbour Lennard--Jones potential are computed by molecular--dynamics simulations. A drastic qualitative change of the…

统计力学 · 物理学 2009-11-11 Stefano Lepri , Paolo Sandri , Antonio Politi

Evaporation and condensation at a liquid/vapor interface are ubiquitous interphase mass and energy transfer phenomena that are still not well understood. We have carried out large scale molecular dynamics simulations of Lennard-Jones (LJ)…

软凝聚态物质 · 物理学 2012-01-12 Shengfeng Cheng , Jeremy B. Lechman , Steven J. Plimpton , Gary S. Grest

Using molecular dynamics simulations, we study a liquid model which consists of particles interacting via a spherically-symmetric two-scale Jagla ramp potential with both repulsive and attractive ramps. The Jagla potential displays…

软凝聚态物质 · 物理学 2009-11-11 Limei Xu , Sergey V. Buldyrev , C. Austen Angell , H. Eugene Stanley

We present a systematic study of the thermodynamics of two and three-dimensional generalized Lennard-Jones ($LJ$) systems focusing on the relationship between the range of the potential, the system density and its dimension. We found that…

统计力学 · 物理学 2007-05-23 M. J. Ison , A. Chernomoretz , C. O. Dorso
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