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相关论文: Confined H(1s) and H(2p) under different geometrie…

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Ground state energies for confined hydrogen (H) and helium (He) atoms, inside a penetrable/impenetrable compartment have been calculated using Diffusion Monte Carlo (DMC) method. Specifically, we have investigated spherical and ellipsoidal…

其他凝聚态物理 · 物理学 2009-11-13 M. Neek-Amal , G. Tayebirad , M. Molayem , M. E. Foulaadvand , L. Esmaeili Sereshki , A. Namiranian

The diffusion Monte Carlo method with symmetry-based state selection is used to calculate the quantum energy states of H$_2^+$ confined into potential barriers of atomic dimensions (a model for these ions in solids). Special solutions are…

化学物理 · 物理学 2019-04-03 Gaia Micca Longo , Savino Longo , Domenico Giordano

A rich literature has been produced on the quantum states of atoms and molecules confined into infinite potential wells with a specified symmetry. Apart from their interest as basic quantum systems, confined atoms and molecules are useful…

化学物理 · 物理学 2019-04-03 Savino Longo , Gaia Micca Longo , Domenico Giordano

The variational Monte Carlo method is used to evaluate the ground-state energy of the confined hydrogen molecule, H_2. Accordingly, we considered the case of hydrogen molecule confined by a hard prolate spheroidal cavity when the nuclear…

原子与分子团簇 · 物理学 2015-09-10 S. B. Doma , F. N. El-Gammal , A. A. Amer

Computational codes based on the Diffusion Monte Carlo method can be used to determine the quantum state of two-electron systems confined by external potentials of various nature and geometry. In this work, we show how the application of…

化学物理 · 物理学 2021-02-24 Gaia Micca Longo , Carla Maria Coppola , Domenico Giordano , Savino Longo

We numerically study the ground state properties of endohedrally confined hydrogen (H) or helium (He) atom by a molecule of C$_{60}$. Our study is based on Diffusion Monte Carlo method. We calculate the effects of centered and small…

其他凝聚态物理 · 物理学 2009-11-13 M. Neek-Amal , G. Tayebirad , R. Asgari

We present ground and excited state energies obtained from Diffusion Monte Carlo (DMC) calculations, using accurate multiconfiguration wave functions, for $N$ electrons ($N\le13$) confined to a circular quantum dot. We analyze the…

凝聚态物理 · 物理学 2009-10-31 F. Pederiva , C. J. Umrigar , E. Lipparini

Diffusion Monte Carlo (DMC) based on fixed-node approximation has enjoyed significant developments in the past decades and become one of the go-to methods when accurate ground state energy of molecules and materials is needed. The remaining…

化学物理 · 物理学 2023-08-07 Weiluo Ren , Weizhong Fu , Xiaojie Wu , Ji Chen

We have used diffusion Monte Carlo (DMC) simulations to calculate the energy barrier for H$_2$ dissociation on the Mg(0001) surface. The calculations employ pseudopotentials and systematically improvable B-spline basis sets to expand the…

材料科学 · 物理学 2009-11-13 M. Pozzo , D. Alfe`

Fixed-node diffusion Monte Carlo (DMC) is a stochastic algorithm for finding the lowest energy many-fermion wave function with the same nodal surface as a chosen trial function. It has proved itself among the most accurate methods available…

凝聚态物理 · 物理学 2009-10-31 W. M. C. Foulkes , Randolph Q. Hood , R. J. Needs

We use the diffusion quantum Monte Carlo (DMC) method to calculate the ground state phase diagram of solid molecular hydrogen and examine the stability of the most important insulating phases relative to metallic crystalline molecular…

材料科学 · 物理学 2015-06-16 S. Azadi , W. M. C. Foulkes , T. D. Kuehne

The many-body diffusion quantum Monte Carlo (DMC) method with twist-averaged boundary conditions is used to calculate the ground-state equation of state and the energetics of point defects in fcc aluminum using supercells up to 1331 atoms.…

材料科学 · 物理学 2012-10-22 Randolph Q. Hood , P. R. C. Kent , Fernando A. Reboredo

We present two Diffusion Monte Carlo (DMC) algorithms for systems of ultracold quantum gases featuring synthetic spin-orbit interactions. The first one is a discrete spin generalization of the T- moves spin-orbit DMC, which provides an…

量子气体 · 物理学 2018-12-05 J. Sanchez-Baena , J. Boronat , F. Mazzanti

A self-contained and tutorial presentation of the diffusion Monte Carlo method for determining the ground state energy and wave function of quantum systems is provided. First, the theoretical basis of the method is derived and then a…

计算物理 · 物理学 2009-10-30 Ioan Kosztin , Byron Faber , Klaus Schulten

Quantum Monte Carlo (QMC) methods represent a powerful family of computational techniques for tackling complex quantum many-body problems and performing calculations of stationary state properties. QMC is among the most accurate and…

材料科学 · 物理学 2025-01-08 Alfonso Annarelli , Dario Alfè , Andrea Zen

We study one-dimensional (1D) and two-dimensional (2D) Helium atoms using a new time-dependent quantum Monte Carlo (TDQMC) method. The TDQMC method employs random walkers, with a separate guiding wave attached to each walker. The ground…

原子物理 · 物理学 2025-02-07 I. P. Christov

We report variational and diffusion quantum Monte Carlo (VMC and DMC) studies of the binding curve of the ground-state chromium dimer. We employed various single determinant (SD) or multi-determinant (MD) wavefunctions multiplied by a…

化学物理 · 物理学 2012-04-06 Kenta Hongo , Ryo Maezono

The ground-state properties of two-dimensional liquid $^4$He at zero temperature are studied by means of a quadratic diffusion Monte Carlo method. As interatomic potential we use a revised version of the HFDHE2 Aziz potential which is…

凝聚态物理 · 物理学 2009-10-28 S. Giorgini , J. Boronat , J. Casulleras

The sampling of the configuration space in diffusion Monte Carlo (DMC) is done using walkers moving randomly. In a previous work on the Hubbard model [\href{https://doi.org/10.1103/PhysRevB.60.2299}{Assaraf et al.~Phys.~Rev.~B \textbf{60},…

The Diffusion Monte Carlo method is devoted to the computation of electronic ground-state energies of molecules. In this paper, we focus on implementations of this method which consist in exploring the configuration space with a {\bf fixed}…

数值分析 · 数学 2007-05-23 Tony Lelievre , Mohamed El Makrini , Benjamin Jourdain
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