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相关论文: Quantum magnetisms in uniform triangular lattices …

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LiZn$_2$Mo$_3$O$_8$ has been proposed to contain $S~=~1/2$ Mo$_3$O$_{13}$ magnetic clusters arranged on a triangular lattice with antiferromagnetic nearest-neighbor interactions. Here, microwave and terahertz electron spin resonance (ESR),…

Inelastic neutron scattering for temperatures below 30 K from a powder of LiZn2Mo3O8 demonstrates this triangular-lattice antiferromagnet hosts collective magnetic excitations from spin 1/2 Mo3O13 molecules. Apparently gapless (\Delta < 0.2…

Molecular magnets based on [Mo$_3$]$^{11+}$ units with one unpaired electron per trimer have attracted recent interest due to the identification of quantum spin liquid candidacy in some family members. Here, we present comprehensive…

A spin-1/2 triangular-lattice antiferromagnet is a prototypical frustrated quantum magnet, which exhibits remarkable quantum many-body effects that arise from the synergy between geometric spin frustration and quantum fluctuations. It can…

We unveil the microscopic origin of largely debated magnetism in the Mo$_{3}$O$_{8}$ cluster systems. Upon considering an extended Hubbard model at 1/6 filling on the anisotropic kagom\'e lattice formed by the Mo atoms, we argue that its…

强关联电子 · 物理学 2022-06-22 S. A. Nikolaev , I. V. Solovyev , S. V. Streltsov

LiZn$_2$Mo$_3$O$_8$ is an electrically insulating geometrically frustrated antiferromagnet in which inorganic Mo$_3$O$_{13}$ clusters each behaves as a single $S = 1/2$ unit, with the clusters arranged on a two-dimensional triangular…

强关联电子 · 物理学 2016-08-18 J. P. Sheckelton , J. R. Neilson , T. M. McQueen

The geometrically frustrated two dimensional triangular lattice magnets A${_4}$B'B${_2}$O$_{12}$ (A = Ba, Sr, La; B' = Co, Ni, Mn; B = W, Re) have been studied by x-ray diffraction, AC and DC susceptibilities, powder neutron diffraction,…

The recent synthesis of the chromium selenide compound LiCrSe$_2$ constitutes a valuable addition to the ensemble of two-dimensional triangular lattice antiferromagnets (2D-TLA). In this work we present the very first comprehensive study of…

$\gamma$-${\rm Ba}_{3}{\rm CoNb}_{2}{\rm O}_{9}$ realizes a disordered simple-cubic spin-$1/2$ lattice in which Co$^{2+}$ ions randomly occupy one third of the sites, placing the system close to the site-percolation threshold for magnetic…

We detail the optimized synthesis of the Mo$_3$O$_8$-type cluster Mott insulator (CMI) Na$_3$Sc$_2$(MoO$_4$)$_2$Mo$_3$O$_8$, which has been considered a candidate for realizing the spin liquid ground state. The optimized…

强关联电子 · 物理学 2024-08-29 Yuya Haraguchi , Daigo Ishikita , Hiroko Aruga Katori

We report thermodynamic properties, magnetic ground state, and microscopic magnetic model of the spin-1 frustrated antiferromaget Li$_{2}$NiW$_{2}$O$_{8}$ showing successive transitions at $T_{\rm N1}\simeq 18$ K and $T_{\rm N2}\simeq 12.5$…

Quantum spin liquids~(QSLs) represent a unique quantum disordered state of matter that hosts long-range quantum entanglement and fractional excitations. However, structural disorder resulting from site mixing between different types of ions…

We have performed magnetic susceptibility, heat capacity, muon spin relaxation, and neutron scattering measurements on three members of the family Ba3MRu2O9, where M = In, Y and Lu. These systems consist of mixed-valence Ru dimers on a…

强关联电子 · 物理学 2017-05-31 D. Ziat , A. A. Aczel , R. Sinclair , Q. Chen , H. D. Zhou , T. J. Williams , M. B. Stone , A. Verrier , J. A. Quilliam

The complex metal oxides Mn2ASbO6 (A=In, Sc) with a corundum-related structure A3BO6 have been prepared as polycrystalline powders by a solid state reaction route. The crystal structure and magnetic properties have been investigated using a…

材料科学 · 物理学 2011-11-21 S. A. Ivanov , P. Nordblad , R. Mathieu , R. Tellgren , E. Politova , G. André

Here, we report the synthesis and magnetic properties of a Yb-based triangular-lattice compound LiYbS$_2$. At low temperatures, it features an effective spin-$\frac{1}{2}$ state due to the combined effect of crystal electric field and spin…

强关联电子 · 物理学 2020-04-22 K. M. Ranjith , Ph. Schlender , Th. Doert , M. Baenitz

We report a muSR study of LiCrO2, which has a magnetic lattice made up of a stacking of triangular Heisenberg antiferromagnetic (Cr3+, S = 3/2) layers. A static magnetically ordered state is observed below the transition temperature T_N =…

强关联电子 · 物理学 2009-06-09 A. Olariu , P. Mendels , F. Bert , L. K. Alexander , A. V. Mahajan , A. D. Hillier , A. Amato

We present microscopic magnetic properties of a two dimensional triangular lattice Sc2Ga2CuO7, consisting of single and double triangular Cu planes. A Curie-Weiss temperature theta_CW = --44 K and an antiferromagnetic (AFM) exchange…

强关联电子 · 物理学 2017-12-06 P. Khuntia , R. Kumar , A. V. Mahajan , M. Baenitz , Y. Furukawa

Quantum magnetic properties in a geometrically frustrated lattice of spin-1/2 magnet, such as quantum spin liquid or solid and the associated spin fractionalization, are considered key in developing a new phase of matter. The feasibility of…

强关联电子 · 物理学 2018-03-21 J. Gunasekera , A. Dahal , Y. Chen , J. Rodriguez , L. Harriger , S. Thomas , T. Heitmann , V. Dugaev , A. Ernst , D. K. Singh

A linear spin-wave approach, a variational method and exact diagonlization are used to investigate the magnetic long-range order (LRO) of the spin-1/2 Heisenberg antiferromagnet on a two-dimensional 1/7-depleted triangular (maple leaf)…

强关联电子 · 物理学 2009-11-07 D. Schmalfuss , P. Tomczak , J. Schulenburg , J. Richter

We uncover four new spin-charge ordered ground states in the strong coupling limit of the Kondo lattice model on triangular geometry. Two of the states at one-third electronic filling ($n=1/3$) consist of decorated ferromagnetic chains…

强关联电子 · 物理学 2015-06-23 Sahinur Reja , Rajyavardhan Ray , Jeroen van den Brink , Sanjeev Kumar
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