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We explore the general phenomenology of resonant inelastic scattering (RIXS) using CuB2O4, a network of CuO4 plaquettes electronically isolated by B+3 ions. Spectra show a small number of well-separated features, and we exploit the simple…

We investigate resonant inelastic X-ray scattering (RIXS) at the O $K$-edge in insulating cuprates by means of three methods: cluster perturbation theory (CPT), Hartree--Fock approximation (HFA) and exact diagonalization (ED) method. We…

强关联电子 · 物理学 2023-02-22 Yukihiro Matsubayashi , Sumio Ishihara

We present a novel derivation of resonant inelastic x-ray scattering (RIXS) which yields an expression for the RIXS cross section in terms of emission pathways between intermediate and final many-body states. Thereby electron-hole…

材料科学 · 物理学 2020-10-14 Christian Vorwerk , Francesco Sottile , Claudia Draxl

Generic low-energy spectral features related to $d$-$d$ excitations in nearly cubic vanadium perovskites are predicted for the expected $L$-edge resonant inelastic X-ray scattering (RIXS) measurements. Model Hamiltonian describing local…

强关联电子 · 物理学 2013-01-22 V. Yushankhai , L. Siurakshina

We develop a formalism to study indirect resonant inelastic x-ray scattering (RIXS) in systems with itinerant electrons, accounting for the attraction between valence electrons and the positively-charged core hole exactly, and apply this…

强关联电子 · 物理学 2014-07-16 David Benjamin , Israel Klich , Eugene Demler

We propose a method for realizing true, real-space imaging of charge dynamics in a periodic system, with angstrom spatial resolution and attosecond time resolution. In this method, inelastic x-ray scattering (IXS) is carried out with a…

强关联电子 · 物理学 2015-06-05 Yu Gan , Anshul Kogar , Peter Abbamonte

Nonresonant inelastic x-ray scattering (NIXS) is a possible tool to detect charge excitations in electron systems. In addition, multipole transitions at high-momentum-transfer region open a new possibility to determine orbital-selective…

强关联电子 · 物理学 2015-11-11 Kenji Tsutsui , Eiji Kaneshita , Takami Tohyama

We present a computational study of $L$-edge resonant inelastic x-ray scattering (RIXS) in correlated 3$d$ transition-metal oxides using an $ab$ $initio$ method based on local density approximation + dynamical mean-field theory (DMFT). The…

强关联电子 · 物理学 2020-03-25 Atsushi Hariki , Mathias Winder , Takayuki Uozumi , Jan Kuneš

We describe a new method for imaging ultrafast dynamics in condensed matter using inelastic x-ray scattering (IXS). We use the concepts of causality and irreversibility to construct a general solution to the inverse scattering problem (or…

其他凝聚态物理 · 物理学 2009-06-12 P. Abbamonte , G. C. L. Wong , D. Cahill , J. P. Reed , R. H. Coridan , N. W. Schmidt , G. H. Lai , Y. I. Joe , D. Casa

A new method is presented for describing vibrational effects in x-ray absorption spectroscopy (XAS) and resonant inelastic x-ray scattering (RIXS) using a combination of the classical Franck-Condon (FC) approximation and classical…

材料科学 · 物理学 2017-12-20 Mathias P. Ljungberg

We have performed resonant inelastic x-ray scattering (RIXS) near the Cu-K edge on cuprate superconductors La(2-x)Sr(x)CuO(4), La(2-x)Ba(x)CuO(4), La(2-x)Sr(x)Cu(1-y)Fe(y)O(4) and Bi(1.76)Pb(0.35)Sr(1.89)CuO(6+d), covering underdoped to…

Since its first successful applications in the early 2000s, x-ray Thomson scattering (XRTS) has emerged as one of the most successful tools for the diagnostics of extreme states of matter in the laboratory. By sampling the dynamic structure…

等离子体物理 · 物理学 2026-04-28 Tobias Dornheim , Hannah Bellenbaum , Thomas Gawne , Jan Vorberger , Dirk O. Gericke

We report particle-hole pair excitations in a cuprate insulator in the intermediate regimes of momentum-transfers using high energy inelastic x-ray scattering. The excitation spectra show dispersive features near the Mott edge which shed…

强关联电子 · 物理学 2009-11-07 M. Z. Hasan , E. D. Isaacs , Z-X. Shen , L. L. Miller

The response to the field sequence of nonresonant hole burning, a pump-wait-probe experiment originally designed to investigate slow relaxation in complex systems, is calculated for a model of Brownian oscillators, thus including inertial…

凝聚态物理 · 物理学 2016-08-31 Uli Häberle , Gregor Diezemann

X-ray echo spectroscopy, a counterpart of neutron spin-echo, is being introduced here to overcome limitations in spectral resolution and weak signals of the traditional inelastic x-ray scattering (IXS) probes. An image of a point-like x-ray…

光学 · 物理学 2016-02-26 Yuri Shvyd'ko

Resonant inelastic X-ray scattering (RIXS) is a promising technique for obtaining electron-phonon coupling constants. However, the ability to extract these coupling constants throughout the Brillouin zone for crystalline materials remains…

材料科学 · 物理学 2018-12-19 Andrey Geondzhian , Keith Gilmore

Specific heat and linear thermal expansivity are fundamental thermal dynamics and have been proven as interesting relaxing quantities to investigate in glass transition and glassy state. However, their possibility has much less been…

软凝聚态物质 · 物理学 2021-09-06 Pengfei Zhang , Marco Gandolfi , Francesco Banfi , Christ Glorieux , Liwang Liu

Recent experiments by Larson et al. demonstrate the feasibility of measuring local $dd$ excitations using nonresonant inelastic X-ray scattering (IXS). We establish a general framework for the interpretation where the $dd$ transitions…

强关联电子 · 物理学 2008-06-13 Michel van Veenendaal , M. W. Haverkort

Resonant inelastic X-ray scattering (RIXS) is used increasingly for characterizing low-energy collective excitations in materials. RIXS is a powerful probe, which often requires sophisticated theoretical descriptions to interpret the data.…

强关联电子 · 物理学 2021-09-22 Krzysztof Bieniasz , Steven Johnston , Mona Berciu

We present a theory of the resonant inelastic x-ray scattering (RIXS) to study electronic excitations in orbital ordered manganites. The charge and orbital excitations of the Mn 3d electron are caused by the Coulomb interactions in the…

强关联电子 · 物理学 2009-10-31 H. Kondo , S. Ishihara , S. Maekawa