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Large surface to volume ratios of semiconductor nanocrystals cause susceptibility to charge trapping, which can modify luminescence yields and induce single-particle blinking. Optical spectroscopies cannot differentiate between bulk and…

介观与纳米尺度物理 · 物理学 2013-03-08 Kipp J. van Schooten , Jing Huang , William J. Baker , Dmitri V. Talapin , Christoph Boehme , John M. Lupton

Two-dimensional halide perovskite nanoplatelets (NPLs) have exceptional light-emitting properties, including wide spectral tunability, ultrafast radiative decays, high quantum yields (QY), and oriented emission. To realize efficient…

Electrostatically stabilized nanocrystals (NCs) and, in particular, quantum dots (QDs) hold promise for forming strongly coupled superlattices due to their compact and electronically conductive surface ligands. However, studies on the…

Over the past decade, exciton-polaritons in semiconductor microcavities have attracted a great deal of interest as a driven-dissipative quantum fluid. These systems offer themselves as a versatile platform for performing Hamiltonian…

Semiconductor doped glasses had been used by the research and engineering communities as color filters or saturable absorbers well before it was realized that their optical properties were defined by tiny specs of semiconductor matter known…

介观与纳米尺度物理 · 物理学 2018-12-04 Oleg V. Kozlov , Rohan Singh , Bing Ai , Jihong Zhang , Chao Liu , Victor I. Klimov

Semiconducting single-walled carbon-nanotubes (SWCNTs) are an interesting material for strong-light matter coupling due to their stable excitons, narrow emission in the near infrared and high charge carrier mobilities. Furthermore, they…

材料科学 · 物理学 2021-03-17 Jan M. Lüttgens , Felix J. Berger , Jana Zaumseil

Nanocrystals based on metal-halide perovskites offer a promising material platform for highly efficient lighting. Using transient optical spectroscopy, we study excitation recombination dynamics in manganese-doped CsPb(Cl,Br)3 perovskite…

Photo-luminescence intermittency (blinking) in semiconductor nanocrystals (NCs), a phenomenon ubiquitous to single-emitters, is generally considered to be temporally random intensity fluctuations between bright (On) and dark (Off) states.…

介观与纳米尺度物理 · 物理学 2020-01-29 Amitrajit Mukherjee , Korak Kumar Ray , Chinmay Phadnis , Arunasish Layek , Soumya Bera , Arindam Chowdhury

Chalcogenide perovskites have received considerable interest in photovoltaic research community owing to their stability (thermal and aqueous), non-toxicity and lead free composition. However, to date a theoretical study mainly focusing on…

材料科学 · 物理学 2022-07-13 Pooja Basera , Saswata Bhattacharya

We introduce and theoretically analyze a scheme to prepare and detect non-Gaussian quantum states of an optically levitated particle via the interaction with a light pulse that generates cubic and inverted potentials. We show that this…

We report experiments demonstrating Quantum Interference Control (QuIC) based on two nonlinear optical absorption processes in semiconductors. We use two optical beams of frequencies $\omega$ and $3\omega /2$ incident on AlGaAs and measure…

介观与纳米尺度物理 · 物理学 2019-08-14 Kai Wang , Rodrigo A. Muniz , J. E. Sipe , S. T. Cundiff

Exciton-polaritons in a microcavity are composite two-dimensional bosonic quasiparticles, arising from the strong coupling between confined light modes in a resonant planar optical cavity and excitonic transitions, typically using excitons…

Coherent optical control of individual particles has been demonstrated both for atoms and semiconductor quantum dots. Here we demonstrate the emergence of quantum coherent effects in semiconductor Rydberg excitons in bulk Cu$_2$O. Due to…

介观与纳米尺度物理 · 物理学 2016-09-28 P. Grünwald , M. Aßmann , J. Heckötter , D. Fröhlich , M. Bayer , H. Stolz , S. Scheel

Hybrid lead halide perovskites, such as CH$_3$NH$_3$PbX$_3$ (X=I, Br), are direct gap semiconductors that offer many superior optoelectronic properties combined with extremely simple solution-processing fabrication methods. This makes them…

Future communication and computation technologies that exploit quantum information require robust and well-isolated qubits. Electron spins in III-V semiconductor quantum dots, while promising candidates, see their dynamics limited by…

The coherent spin dynamics of electrons are investigated for CsPbI$_3$ perovskite nanocrystals in a glass matrix using time-resolved Faraday ellipticity. In nanocrystals with a diameter of about 11 nm, the Larmor precession frequency has a…

The resonant interaction between quasi-one dimensional excitons and photons is investigated. For a single isolated organic quantum wire, embedded in its single crystal monomer matrix, the strong exciton-photon coupling regime is reached.…

强关联电子 · 物理学 2009-11-11 F. Dubin , J. Berrehar , R. Grousson , M. Schott , V. Voliotis

The relaxation of strongly-confined electrons and holes between 1P and 1S levels in colloidal PbSe nanocrystals has been time-resolved using femtosecond transient absorption spectroscopy. In contrast to II-VI and III-V semiconductor…

介观与纳米尺度物理 · 物理学 2009-11-10 Jeffrey M. Harbold , Frank W. Wise , Hui Du , Todd D. Krauss , Kyung-Sang Cho , Chris B. Murray

One of the key challenges in developing quantum networks is to generate single photons with high brightness, purity, and long temporal coherence. Semiconductor quantum dots potentially satisfy these requirements; however, due to…

Under continuous light illumination, it is known that localized domains with segregated halide compositions form in semiconducting mixed-halide perovskites, thus severely limiting their optoelectronic applications due to the negative…

材料科学 · 物理学 2023-03-21 Shengnan Feng , Rentong Duan , Yu Ju , Shuyi Li , Chunfeng Zhang , Shuxia Tao , Min Xiao , Xiaoyong Wang