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The crystal structures and magnetic properties of three previously unreported A2B2F7 pyrochlore materials, NaSrMn2F7, NaCaFe2F7, and NaSrFe2F7 are presented. In these compounds, either S=2 Fe2+ or S=5/2 Mn2+ is on the B site, while…

强关联电子 · 物理学 2016-12-21 M. B. Sanders , J. W. Krizan , K. W. Plumb , T. M. McQueen , R. J. Cava

Centimeter-sized single crystals of Sr$_{1.5}$La$_{0.5}$RhO$_{4}$ were grown by the floating zone method at oxygen pressures of 20~bar. The quality of our single crystals was confirmed by X-ray Laue, powder and single crystal X-ray…

强关联电子 · 物理学 2017-09-06 Z. W. Li , H. Guo , Z. Hu , T. S. Chan , K. Nemkovski , A. C. Komarek

Up to now the crystallographic structure of the magnetoelectric perovskite EuTiO3 was considered to remain cubic down to low temperature. Here we present high resolution synchrotron X-ray powder diffraction data showing the existence of a…

We report the growth of YFe2O4-\delta\ single crystals by the optical floating zone method, showing for the first time the same magnetization as highly stoichiometric (\delta = 0.00) powder samples and sharp superstructure reflections in…

材料科学 · 物理学 2015-08-13 Thomas Mueller , Joost de Groot , Joerg Strempfer , Manuel Angst

By varying the parameters controlling the growth of crystals, including the thermodynamic variables, such as temperature, pressure, and reagent composition and the kinetic factors, namely reaction time and cooling rate, we found the most…

超导电性 · 物理学 2019-06-26 Nikolai D. Zhigadlo

Growth parameters play a significant role in the crystal quality and physical properties of layered materials. Here we present a case study on a van der Waals magnetic NbFeTe2 material. Two different types of polymorphic NbFeTe2 phases,…

We examine the resistivity and thermopower of single crystal specimens of the pyrochlore oxide Cd2Re2O7 at pressures up to 2GPa. Thermopower proves to be a sensitive tool in the study of the phase diagram of Cd2Re2O7. The 200K…

强关联电子 · 物理学 2009-11-10 N. Barisic , L. Forro , D. Mandrus , R. Jin , J. He , P. Fazekas

Highly crystalline TiO2 nanostructures were prepared through a facile inorganic acid-assisted hydrothermal treatment of hexagonal-structured assemblies of nanocrystalline titiania templated by cetyltrimethylammonium bromide (Hex-ncTiO2/CTAB…

材料科学 · 物理学 2012-11-20 Shuxi Dai , Yanqiang Wu , Toshio Sakai , Zuliang Du , Hideki Sakai , Masahiko Abe

Structural, vibrational and dielectric properties of (Pb1-xBix)(Ti1-xMnx)O3 (PBTM) (0 x 0.50) polycrystalline ceramics have been examined as a function of temperature. Synchrotron-based powder x-ray diffraction was employed to confirm phase…

We present a systematic growth study of epitaxial RuO$_2$(110) and IrO$_2$(110) on TiO$_2$(110) substrates by pulsed laser deposition. We describe the main challenges encountered in the growth process, such as a deteriorating material flux…

We synthesized strontium titanate SrTiO$_3$ (STO), Zr doped $\text{Sr}_\text{1-x}\text{Zr}_\text{x}\text{Ti}\text{O}_3$ and (Zr, Ni) co-doped $\text{Sr}_\text{1-x}\text{Zr}_\text{x}\text{Ti}_\text{1-y}\text{Ni}_\text{y}\text{O}_3$ samples…

Large high-quality single crystals of hole-doped iron-based superconductor (Ba$_{1-x}$K$_x$)Fe$_2$As$_2$ were grown over a broad composition range $0.22 \leq x \leq 1$ by inverted temperature gradient method. We found that high soaking…

We report the results of Hall coefficient R_H and magnetoresistance (MR) measurements on single crystalline samples of Sr3Ru2O7 grown by the floating zone method. R_H was found to be positive over the entire temperature range studied (0.3 -…

强关联电子 · 物理学 2010-10-11 Y. Liu , R. Jin , Z. Q. Mao , K. D. Nelson , M. K. Haas , R. J. Cava

By combining neutron scattering and magnetization measurements down to 80 mK, we determine the $(H,T)$ phase diagram of the Nd$_2$(Zr$_{1-x}$Ti$_x$)$_2$O$_7$ pyrochlore magnet compounds. In those samples, Zr is partially substituted by Ti,…

Barium titanate (BaTiO$_3$) is a prototypical ferroelectric perovskite that undergoes the rhombohedral-orthorhombic-tetragonal-cubic phase transitions as the temperature increases. In this work, we develop a classical interatomic potential…

材料科学 · 物理学 2016-11-23 Yubo Qi , Shi Liu , Ilya Grinberg , Andrew M. Rappe

We report the first single crystal growth of the correlated metal LaNiO3 using a high-pressure optical-image floating zone furnace. The crystals were studied using single crystal/powder x-ray diffraction, resistivity, specific heat, and…

材料科学 · 物理学 2017-10-17 Junjie Zhang , Hong Zheng , Yang Ren , J. F. Mitchell

We have grown underdoped (x = 0.11, 0.12) and optimally doped (x = 0.16) La2-xSrxCuO4 (LSCO) crystals by traveling-solvent floating-zone (TSFZ) technique. In order to obtain LSCO single crystals of high quality, we have made much effort to…

超导电性 · 物理学 2009-01-23 Xiaoli Shen , Zhengcai Li , Caixia Shen , Wei Lu , Xiaoli Dong , Fang Zhou* , Zhongxian Zhao

Millimeter sized single crystals of Mo3Sb7 are grown using the self-flux technique and a thorough characterization of their structural, magnetic, thermal and transport properties is reported. The structure parameters for the…

超导电性 · 物理学 2013-05-24 J. -Q. Yan , M. A. McGuire , A. F. May , H. Cao , A. D. Christianson , D. G. Mandrus , B. C. Sales

We investigated the growth of titanium oxide two-dimensional (2D) nanostructures on Au(111), produced by Ti evaporation and post-deposition oxidation. Scanning tunneling microscopy and spectroscopy (STM and STS) and low-energy electron…

材料科学 · 物理学 2016-12-21 F. Tumino , P. Carrozzo , L. Mascaretti , C. S. Casari , M. Passoni , S. Tosoni , C. E. Bottani , A. Li Bassi

Motivated by the experimental synthesis of two-dimensional (2D) perovskite materials, we study the stability of 2D SrTiO$_3$ from first principles. We find that the TiO$_6$ octahedral rotations emerge in 2D SrTiO$_3$ with a rotation angle…

材料科学 · 物理学 2023-10-27 Shota Ono , Yu Kumagai
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