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We study non-perturbative effects of a static electric field on two-color photoassociation of different atoms. A static electric field induces anisotropy in scattering between two different atoms and hybridizes field-free rotational states…

原子物理 · 物理学 2014-05-08 Debashree Chakraborty , Bimalendu Deb

We report on two-photon photoassociation (PA) spectroscopy of ultracold heteronuclear LiRb molecules. This is used to determine the binding energies of the loosely bound levels of the electronic ground singlet and the lowest triplet states…

量子气体 · 物理学 2017-01-25 Sourav Dutta , Jesús Pérez-Ríos , D. S. Elliott , Yong P. Chen

The properties of photoassociation (PA) spectra near the intercombination line (the weak transition between $^{1}S_{0}$ and $^{3}P_{1}$ states) of group II atoms are theoretically investigated. As an example we have carried out a…

原子物理 · 物理学 2009-11-10 R. Ciurylo , E. Tiesinga , S. Kotochigova , P. S. Julienne

In this work we investigate small clusters of bosons using the hyperspherical harmonic basis. We consider systems with $A=2,3,4,5,6$ particles interacting through a soft inter-particle potential. In order to make contact with a real system,…

原子与分子团簇 · 物理学 2012-11-16 M. Gattobigio , A. Kievsky , M. Viviani

We demonstrate Feshbach optimized photoassociation (FOPA) into the $0_{g}^{-} (5$S$_{1/2}+5$P$_{1/2}$) state in $^{85}$Rb$_{2}$. FOPA uses the enhancement of the amplitude of the initial atomic scattering wave function due to a Feshbach…

原子物理 · 物理学 2016-01-20 S. P. Krzyzewski , T. G. Akin , J. Dizikes , Micheal A. Morrison , E. R. I. Abraham

When the atoms of a dimer remain most of the time very far apart, in so-called long-range molecular states, their mutual interaction is ruled by plain atomic properties. The high-resolution spectroscopic study of some molecular excited…

原子物理 · 物理学 2015-05-13 Nadia Bouloufa , Anne Crubellier , Olivier Dulieu

We calculate accurate potential energy curves for a ground-state He$^+$ ion interacting with a He atom in the lowest-energy metastable $^3\!S$ electronic state. We employ the full configuration interaction method, equivalent to exact…

原子物理 · 物理学 2023-11-30 Jacek Gȩbala , Michał Przybytek , Marcin Gronowski , Michał Tomza

Photoabsorption spectra of N$_2$ and CO were recorded at 900K, using the vacuum-ultraviolet Fourier-transform spectrometer at the DESIRS beamline of synchrotron SOLEIL. These high-temperature and high-resolution measurements allow for…

We have observed short-range photoassociation of LiRb to the two lowest vibrational states of the $d\,^3\Pi$ potential. These $d\,^3\Pi$ molecules then spontaneously decay to vibrational levels of the $a^3\,\Sigma^+$ state with generation…

Photoassociation (PA) of ultracold metastable helium to the 2s2p manifold is theoretically investigated using a non-perturbative close-coupled treatment in which the laser coupling is evaluated without assuming the dipole approximation. The…

原子物理 · 物理学 2015-05-14 Daniel G. Cocks , Ian B. Whittingham

We investigate the electronic structure of a perovskite-type Pauli paramagnet SrMoO3 (t2g2) thin film using hard x-ray photoemission spectroscopy and compare the results to the realistic calculations that combine the density functional…

The precision of the photoassociation spectroscopy of Yb dimer in degenerate gases is enough to improve the constraints on the new short-range gravity-like forces if the theoretical knowledge of the Born-Oppenheimer interatomic potential…

原子物理 · 物理学 2021-11-12 Giorgio Visentin , Alexei A. Buchachenko , Paweł Tecmer

The electronic structure of Si(110)"16 x 2" double-domain, single-domain and 1 x 1 surfaces have been investigated using spin- and angle-resolved photoemission at sample temperatures of 77 K and 300 K. Angle-resolved photoemission was…

We report the homonuclear photoassociation (PA) of ultracold ${}^{52}\mathrm{Cr}$ atoms in an optical dipole trap. This constitutes the first measurement of PA in an element with total electron spin $\tilde{S}>1$. Although Cr, with its…

原子物理 · 物理学 2016-03-09 Jahn Rührig , Tobias Bäuerle , Paul S. Julienne , Eite Tiesinga , Tilman Pfau

We have investigated rovibronic levels of the strongly mixed $b^3\Pi_1-c^3\Sigma^+_1-B^1\Pi_1$ states [the 2(1), 3(1), and 4(1) states in Hund's case (c) notation] of $^{85}$Rb$^{133}$Cs in the energy range of 13950$-$14200 cm$^{-1}$ using…

原子物理 · 物理学 2018-10-24 Toshihiko Shimasaki , Jin-Tae Kim , Yuqi Zhu , David DeMille

We formulate the theory for a diatomic molecule in a spatially degenerate electronic state interacting with a non-resonant laser field and investigate its rovibrational structure in the presence of the field. We report on \textit{ab initio}…

We present spectra of ultracold $^7$Li$^{85}$Rb molecules in their electronic ground state formed by spontaneous decay of weakly bound photoassociated molecules. Beginning with atoms in a dual species magneto-optical trap (MOT), weakly…

原子物理 · 物理学 2014-12-24 John Lorenz , Adeel Altaf , Sourav Dutta , Yong P. Chen , D. S. Elliott

The theory of the long-range interaction of metastable excited atomic states with ground-state atoms is analyzed. We show that the long-range interaction is essentially modified when quasi-degenerate states are available for virtual…

原子物理 · 物理学 2017-02-15 C. M. Adhikari , V. Debierre , A. Matveev , N. Kolachevsky , U. D. Jentschura

Photoassociation of spin-polarized metastable helium to the three lowest rovibrational levels of the J=1, $0_u^+$ state asymptoting to 2$s {}^{3}$S$_{1}+2p {}^{3}$P$_{0}$ is studied using a second-order perturbative treatment of the line…

原子物理 · 物理学 2015-05-13 Daniel G Cocks , Ian B Whittingham

We present an exact diagrammatic approach for the problem of dimer-dimer scattering in 3D for dimers being a resonant bound state of two fermions in a spin-singlet state, with corresponding scattering length $a_F$. Applying this approach to…

强关联电子 · 物理学 2016-08-16 I. V. Brodsky , A. V. Klaptsov , M. Yu. Kagan , R. Combescot , X. Leyronas