中文
相关论文

相关论文: Lattice distortion in the spin-orbital entangled s…

200 篇论文

Oxide double perovskites wherein octahedra formed by both 3d elements and sp-based heavy elements give rise to unconventional magnetic ordering and correlated quantum phenomena crucial for futuristic applications. Here, by carrying out…

The local and intermediate structure of stoichiometric LaMnO$_3$ has been studied in the pseudocubic and rhombohedral phases at high temperatures (300 to 1150 K). Neutron powder diffraction data were collected and a combined Rietveld and…

强关联电子 · 物理学 2009-11-10 Xiangyun Qiu , Th. Proffen , J. F. Mitchell , S. J. L. Billinge

We present a combined study of the thermal expansion and the thermal conductivity of the perovskite series RCoO_3 with R = La, Nd, Pr and Eu. The well-known spin-state transition in LaCoO_3 is strongly affected by the exchange of the R ions…

强关联电子 · 物理学 2010-01-04 K. Berggold , M. Kriener , P. Becker , M. Benomar , M. Reuther , C. Zobel , T. Lorenz

We present a unique study of the frustrated spinel MgV2O4 which possesses highly coupled spin, lattice and orbital degrees of freedom. Using large single-crystal and powder samples, we find a distortion from spinel at room temperature…

The mixed rare-earth orthochromite Nd$_{0.5}$Dy$_{0.5}$CrO$_{3}$ has a N\'eel temperature ($T_\mathrm{{N}}$) of ${\sim}$ 175\,K, resulting in the G-type antiferromagnetic ordering of Cr$^{3+}$ spins. The inverse susceptibility shows a…

A fully ab initio scheme based on quantum chemical wavefunction methods is used to investigate the correlated multiorbital electronic structure of a 3d-metal compound, LaCoO3. The strong short-range electron correlations, involving both Co…

强关联电子 · 物理学 2009-11-13 L. Hozoi , U. Birkenheuer , H. Stoll , P. Fulde

Anisotropic optical spectra coupled with antiferromagnetic spin ordering (SO) and orbital ordering (OO) have been investigated for single crystals of LaVO_{3} and YVO_{3}. The orbital-dependent Mott-Hubbard gap transitions are observed…

强关联电子 · 物理学 2009-11-07 Shigeki Miyasaka , Yoichi Okimoto , Yoshinori Tokura

We report the observation of spin glass state in the double perovskite oxide Sr$_{2}$FeCoO$_{6}$ prepared through sol-gel technique. Initial structural studies using x rays reveal that the compound crystallizes in tetragonal $I 4/m$…

High-resolution ac susceptibility and thermal conductivity measurement on Cu2Te2O5X2(X=Br,Cl) single crystals are reported. For Br-sample, sample dependence prevents to distinguish between possibilities of magnetically ordered and…

强关联电子 · 物理学 2009-11-10 M. Prester , A. Smontara , I. Zivkovic , A. Bilusic , D. Drobac , H. Berger , F. Bussy

Using the multiband $d-p$ model and unrestricted Hartree-Fock approximation we investigate the electronic structure and spin-orbital order in three-dimensional MnO$_3$ lattice such as realized in LaMnO$_3$. The orbital order is induced and…

强关联电子 · 物理学 2019-04-04 Krzysztof Rościszewski , Andrzej M. Oleś

The Mn spin correlations were studied near the O'-O phase transition at T{JT} = 750 K, up to 950 K with 17O and 139La NMR in a stoichiometric LaMnO3 crystalline sample. The measured local hyperfine fields originate from the electron density…

强关联电子 · 物理学 2015-06-15 A. Trokiner , S. Verkhovskii , A. Gerashenko , Z. Volkova , O. Anikeenok , K. Mikhalev , M. Eremin

The samples LaCoO3 with dilute substitutions on cobalt sites have been studied using the resistivity, thermopower and magnetic susceptibility measurements over the temperature range up to ~900 K. The Co-site substitution does not affect the…

材料科学 · 物理学 2010-07-30 J. Hejtmanek , Z. Jirak , K. Knizek , M. Marysko , M. Veverka , C. Autret

Ferromagnetism and its evolution in the orthorhombic perovskite system Sr1-xCaxRuO3 have been widely believed to correlate with the structural distortion. The recent development of high-pressure synthesis of the Ba substituted Sr1-yBayRuO3…

强关联电子 · 物理学 2015-06-17 J. -G. Cheng , J. -S. Zhou , J. B. Goodenough

We investigate the ground state of the $d^1$ spin-orbital model for triply degenerate $t_{2g}$ orbitals on a triangular lattice which unifies intrinsic frustration of spin and orbital interactions with geometrical frustration. Using full or…

强关联电子 · 物理学 2011-03-14 Jiří Chaloupka , Andrzej M. Oleś

We investigated the spin-lattice coupling in orthorhombic pseudobrookite FeTi2O5 single crystal with highly ordered $ Fe^{2+} / Ti^{4+}$ occupation, which consists of quasi-1D S=2 chains running along a-axis. Both the magnetization and…

强关联电子 · 物理学 2024-05-31 Hao-Hang Xu , Jian Liu , L. L. Tao , Xian-Jie Wang , Sergey V. Streltsov , Yu Sui

The phase diagram of $Pr_{1-x}Ca_xMnO_3$ is modified x $\le$ 0.3, which suggests a reevaluation of the phase diagram of other manganites in that doping region. Rather than an orbital ordered phase reaching up to high temperatures of…

The functional properties of transition metal perovskite oxides are known to result from a complex interplay of magnetism, polarization, strain, and stoichiometry. Here, we show that for materials with a cooperative Jahn-Teller distortion,…

材料科学 · 物理学 2021-01-04 Chiara Ricca , Nicolas Niederhauser , Ulrich Aschauer

Magnetic ordering in the geometrically frustrated magnetic oxide spinels MgCr_2O_4 and ZnCr_2O_4 is accompanied by a structural change that helps relieve the frustration. Analysis of high-resolution synchrotron X-ray scattering reveals that…

^{139}La NMR measurements of La_{2/3}Ca_{1/3}MnO_3 performed in the paramagnetic state and high magnetic fields are reported. Analysis of the high temperature spectrum measured establishes that the spectrum it is a standard powder pattern…

强关联电子 · 物理学 2009-10-31 K. E. Sakaie , C. P. Slichter , P. Lin , M. Jaime , M. B. Salamon

We report on the electronic ground state of a layered perovskite vanadium oxide Sr$_2$VO$_4$ studied by the combined use of synchrotron radiation x-ray diffraction (SR-XRD) and muon spin rotation/relaxation ($\mu$SR) techniques, where…