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Spatial distributions are presented that quantitatively capture how polymer properties (e.g., segment alignment, density, and potential energy) vary with distance from nascent polymer crystals (nuclei) in prototypical polyethylene melts. It…

材料科学 · 物理学 2020-07-15 Kyle Wm. Hall , Simona Percec , Wataru Shinoda , Michael L. Klein

We study the spontaneous crystallization of an assembly of highly monodisperse steel spheres under shaking, as it evolves from localized icosahedral ordering towards a packing reaching crystalline ordering. Towards this end, real space…

软凝聚态物质 · 物理学 2018-12-06 Indu Dhiman , Simon A. J. Kimber , Anita Mehta , Tapan Chatterji

The nucleation of the first order phase transition of superfluid 3He-B from superfluid 3He-A is quite remarkable since it requires a seed of the order of a micron. We have studied this nucleation for 3He confined to a very dilute silica…

凝聚态物理 · 物理学 2009-11-07 G. Gervais , K. Yawata , N. Mulders , W. P. Halperin

There exists a class of nuclei that are obtained by adding one nucleon to a loosely-bound nucleon-core system, for example $^{12}$Be, $^9$C, $^{18}$Ne. For such nuclei, one-nucleon overlap integrals that represent single-particle motion can…

核理论 · 物理学 2009-11-13 N. K. Timofeyuk , I. J. Thompson , J. A. Tostevin

We report observations of the self-assembly of coated droplets into regular clusters at the sudden expansion of a microfluidic channel. A double emulsion consisting of a regular train of coated microdroplets was created upstream of the…

软凝聚态物质 · 物理学 2020-10-19 Kerstin Schirrmann , Gabriel Cáceres-Aravena , Anne Juel

The nucleation of a lamellar phase from a supercooled homogeneous phase in a fluctuation driven first-order transition is studied, based on a phenomenological free energy due to Brazovskii. The absence of phase coexistence in the…

patt-sol · 物理学 2009-10-28 P. C. Hohenberg , J. B , Swift

Co-assembly of inorganic nanoparticles (NPs) and nanostructured polymer matrix represents an intricate interplay of enthalpic or entropic forces. Particle size largely affects the phase behavior of the nanocomposite. Theoretical studies…

软凝聚态物质 · 物理学 2022-04-25 Le Ma , Hejin Huang , Peter Ercius , Alfredo Alexander-Katz , Ting Xu

Structures of light unstable nuclei, Li, Be, B, and C isotopes are systematically studied with a microscopic method of antisymmetrized molecular dynamics. The theoretical method is found to be very useful to study ground and excited states…

核理论 · 物理学 2009-11-07 Y. Kanada-En'yo , H. Horiuchi

The article is dedicated to the experimental study in the relativistic approach to the problems of nuclear cluster physics for the prospects of the \href{http://becquerel.jinr.ru/}{BECQUEREL} experiment. The nuclear emulsion method applied…

The phase behaviour of blends of ABC triblock and ac diblock copolymers is examined using self-consistent field theory. Several equilibrium lamellar structures are observed, depending on the volume fraction of the diblocks, phi_2, the…

软凝聚态物质 · 物理学 2009-11-07 Robert A. Wickham , An-Chang Shi

Classical theories of crystal nucleation and growth from the liquid assume activated processes that are interface limited, with the atoms individually joining the growing interface by jumps that occur at a rate that is determined by the…

原子物理 · 物理学 2023-01-02 Fangzheng Chen , Zohar Nussinov , K. F. Kelton

The turbulent burning of nuclei is a common phenomenon in the evolution of stars. Here we examine a challenging case: the merging of the neon and oxygen burning shells in a 23 M$_{\odot}$ star. A previously unknown quasi-steady state is…

太阳与恒星天体物理 · 物理学 2018-09-12 Miroslav Mocák , Casey Meakin , Simon Wattana Campbell , David Arnett

We investigated the relative stability of the amorphous vs crystalline nanoparticles of size ranging between 0.8 and 1.8 nm. We found that, at variance from bulk systems, at low T small nanoparticles are amorphous and they undergo to an…

介观与纳米尺度物理 · 物理学 2015-05-27 Sergio Orlandini , Simone Meloni , Luciano Colombo

A nonequilibrium molecular dynamics computer simulation on microsegregated solutions of symmetrical diblock copolymers is reported. As the polymer concentration increases, the system undergoes phase transitions in the following order: body…

软凝聚态物质 · 物理学 2007-05-23 Igor Rychkov , Kenichi Yoshikawa

We report studies of the Yb$^{3+}$ site distribution in Er$^{3+}$ co-doped upconverting alkaline earth fluoride nanoparticles using high-resolution absorption measurements. Similar to bulk crystals, Yb$^{3+}$ single ion cubic (O$_h$), and…

材料科学 · 物理学 2020-04-30 Sangeetha Balabhadra , Michael F. Reid , Vladimir Golovko , Jon-Paul R. Wells

Monolayer cluster growth in far-from-equilibrium systems is investigated by applying simulation and analytic techniques to minimal hard core particle (exclusion) models. The first model (I), for post-deposition coarsening dynamics, contains…

统计力学 · 物理学 2009-11-10 F. D. A. Aarao Reis , R. B. Stinchcombe

Self-propelled particles can spontaneously form dense phases from a dilute suspension in a process referred to as motility-induced phase separation. The properties of the out-of-equilibrium structures that are formed are governed by the…

软凝聚态物质 · 物理学 2016-09-08 Sven Erik Ilse , Christian Holm , Joost de Graaf

We present a simple chemical strategy for the formation of a self-propelling cluster via the process of capture and assembly of passive colloids on the surface of a chemically active colloid. The two species of colloids that are isotropic…

生物物理 · 物理学 2019-10-02 Prabha Chuphal , Ishwar Venugopal , Snigdha Thakur

In this study, novel achiral mesogens containing 4,4'-biphenyl central core connected on both sides through an ester function to 1-(4-(alkyloxy)phenyl)-1H-[1,2,3]-triazolyl group have been synthesized and characterized. Different mesophases…

软凝聚态物质 · 物理学 2023-12-07 Souria Benalloua , Salima Saidi-Besbes , Abdelatif Bouyacoub , Eric Grelet

The isothermal, isobaric spontaneous crystallization of a supercooled polymer melt is investigated by MD simulation of an ensemble of fully-flexible linear chains. Frustration is introduced via two incommensurate length scales set by the…

软凝聚态物质 · 物理学 2018-11-19 Andrea Giuntoli , Sebastiano Bernini , Dino Leporini