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We demonstrate that high-harmonic generation (HHG) in solids dominantly originates from strongly localized surface states through non-perturbative processes. Measurements reveal that HHG from bulk states is suppressed by at least 1-2 orders…
We consider several aspects of high-order harmonic generation in solids: the effects of elastic and inelastic scattering; varying pulse characteristics; and inclusion of material-specific parameters through a realistic band structure. We…
High-order harmonic generation (HHG) in solids has emerged as a versatile platform for exploring ultrafast and quantum-coherent phenomena in condensed matter. Recent advances reveal Berry-phase and topological effects in harmonic emission,…
High-order harmonic generation (HHG) in isolated atoms and molecules has been widely utilized in extreme ultraviolet (XUV) photonics and attosecond pulse metrology. Recently, HHG has also been observed in solids, which could lead to…
We analytically and numerically investigate the emission of high-harmonic radiation from model solids by intense few-cycle mid-infrared laser pulses. In single-active-electron approximation, we expand the active electron's wavefunction in a…
High-harmonic generation by a highly non-linear interaction of infrared laser fields with matter allows for the generation of attosecond pulses in the XUV spectral regime. This process, well established for atoms, has been recently extended…
High-harmonic generation (HHG) in the two topological phases of a finite, one-dimensional, periodic structure is investigated using a self-consistent time-dependent density functional theory (TDDFT) approach. For harmonic photon energies…
High-harmonic generation (HHG) in solids has emerged in recent years as a rapidly expanding and interdisciplinary field, attracting attention from both the condensed-matter and the atomic, molecular, and optics communities. It has exciting…
High-order harmonic generation is a powerful and sensitive tool for probing atomic and molecular structures, combining in the same measurement an unprecedented attosecond temporal resolution with a high spatial resolution, of the order of…
We find that a donor-doped band-gap material can enhance the overall high-order harmonic generation (HHG) efficiency by several orders of magnitude, compared with undoped and acceptor-doped materials. This significant enhancement, predicted…
High-harmonic generation (HHG) in solids has typically been explored in transparent dielectrics and semiconductors. Metals have long been dismissed due to their strong reflectivity at infrared wavelengths. Here, we demonstrate HHG from…
Optical modulation of high-harmonics generation in solids enables the detection of material properties such as the band structure and promising new applications such as super-resolution imaging in semiconductors. Various recent studies have…
High-harmonic generation in solids allows probing and controlling electron dynamics in crystals on few femtosecond timescales, paving the way to lightwave electronics. In the spatial domain, recent advances in the real-space interpretation…
Using real-space view of high harmonic generation (HHG) in solids, we develop a physically transparent and gauge-invariant approach for distinguishing intraband and interband HHG mechanisms. Our approach relies on resolving the harmonic…
High harmonic generation (HHG) from gas phase atoms (or molecules) has opened up a new frontier in ultrafast optics, where attosecond time resolution and Angstrom spatial resolution are accessible. The fundamental physical pictures of HHG…
The generation of high-order harmonics in bulk solids subjected to intense ultrashort laser pulses has opened up new avenues for research in extreme nonlinear optics and light-matter interaction on sub-cycle timescales. Despite significant…
We propose and experimentally demonstrate a scheme allowing to reach noncollinear phase-matching of high harmonic generation in solids, which may potentially lead to an enhancement of the generation efficiency. The principle is based on…
We investigate high-order harmonic generation in a solid, modeled as a multi-level system dressed by a strong infrared laser field. We show that the cutoff energies and the relative strengths of the multiple plateaus that emerge in the…
An accurate analytic model describing high-harmonic generation (HHG) in solids is derived. Extensive first-principles simulations within a time-dependent density-functional framework corroborate the conclusions of the model. Our results…
Thermotropic liquid crystals are versatile optical materials that exhibit a state of matter intermediate between liquids and solids. Their properties can change significantly with temperature, pressure, or other external factors, leading to…