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We report on THz, infrared reflectivity and transmission experiments for wave numbers from 10 to 8000 cm$^{-1}$ ($\sim$ 1 meV - 1 eV) and for temperatures from 5 to 295 K on the Kitaev candidate material {\alpha}-RuCl$_3$. As reported…

强关联电子 · 物理学 2017-10-18 S. Reschke , F. Mayr , Zhe Wang , Seung-Hwan Do , K. -Y. Choi , A. Loidl

Raman scattering has been employed to investigate lattice and magnetic excitations of the honeycomb Kitaev material $\alpha$-RuCl$_3$ and its Heisenberg counterpart CrCl$_3$. Our phonon Raman spectra give evidence for a first-order…

强关联电子 · 物理学 2017-06-07 A. Glamazda , P. Lemmens , S. -H. Do , Y. S. Kwon , K. -Y. Choi

We report X-ray diffraction and magnetic susceptibility studies of the structural phase transition in $\alpha$-RuCl$_{3}$. By utilizing a single crystal sample with predominantly single twin domain, we show that $\alpha$-RuCl$_{3}$ goes…

强关联电子 · 物理学 2023-11-08 Subin Kim , Ezekiel Horsley , Jacob P. C. Ruff , Beatriz D. Moreno , Young-June Kim

A new-type structural transition has been found in Li2RuO3 with honeycomb lattice of edge-sharing RuO6-octahedra. With decreasing temperature T, the electrical resistivity exhibits an anomalous increase at T=Tc~540 K, suggesting the (metal…

强关联电子 · 物理学 2015-06-25 Yoko Miura , Yukio Yasui , Masatoshi Sato , Naoki Igawa , Kazuhisa Kakurai

The discovery of ordered magnetism in two-dimensional van der Waals materials at the monolayer limit challenges the Mermin-Wagner theorem, which forbids spontaneous breaking of continuous symmetries in two dimensions at finite temperatures.…

Most transition-metal trihalides are dimorphic. The representative chromium-based triad, CrCl3, CrBr3, CrI3, is characterized by the low-temperature phase adopting the trigonal BiI3 type while the structure of the high-temperature phase is…

$\alpha$-RuCl$_3$ has attracted significant attention as a prime candidate for the spin-1/2 Kitaev spin liquid in two-dimensional honeycomb lattices. Although its ground state is magnetically ordered, the order is suppressed under a…

强关联电子 · 物理学 2025-07-15 Jiefu Cen , Hae-Young Kee

The crystallographic and magnetic properties of the cleavable 4d3 transition metal compound a-MoCl3 are reported, with a focus on the behavior above room temperature. Crystals were grown by chemical vapor transport and characterized using…

The Kitaev quantum spin liquid (QSL) on the two-dimensional honeycomb lattice epitomizes an entangled topological state, where the spins fractionalize into Majorana fermions. This state has aroused tremendous interest because it harbors…

We report a room-temperature optical reflectivity study performed on [112]-oriented Cd$_3$As$_2$ single crystals over a broad energy range under external pressure up to 10 GPa. The abrupt drop of the band dispersion parameter…

材料科学 · 物理学 2018-05-23 E. Uykur , R. Sankar , D. Schmitz , C. A. Kuntscher

The local structure of V$_{2}$O$_{3}$, an archetypal strongly correlated electron system that displays a metal-insulator transition around 160 K, has been investigated via pair distribution function (PDF) analysis of neutron and x-ray total…

The majority of research on $\alpha$-RuCl$_3$ has focused on applying in-plane magnetic fields to suppress antiferromagnetic order and induce a quantum spin liquid (QSL). However, this effort has been complicated by the materials…

A pseudo honeycomb system Li2RuO3 exhibits a second-order-like transition at temperature T=Tc=540 K to a low-T nonmagnetic phase with a significant lattice distortion forming Ru-Ru pairs. For this system, we have calculated the band…

强关联电子 · 物理学 2015-05-13 Yoko Miura , Masatoshi Sato , Youichi Yamakawa , Tatsuro Habaguchi , Yoshiaki Ono

We investiaged the optical properties of four-layer BaRuO$_{3}$, which shows a fermi-liquid-like behavior at low temperature. Its optical conductivity spectra clearly displayed the formation of a pseudogap and the development of a coherent…

强关联电子 · 物理学 2009-11-07 Y. S. Lee , J. S. Lee , K. W. Kim , T. W. Noh , Jaejun Yu , Yunkyu Bang , M. K. Lee , C. B. Eom

High-resolution thermal expansion and magnetostriction measurements were performed on single crystals of $\alpha$-RuCl$_3$ in magnetic fields applied parallel to the Ru-Ru bonds. The length changes were measured in the direction…

Layered transition metal dichalcogenides (TMDs) stabilize in multiple structural forms with profoundly distinct and exotic electronic phases. Interfacing different layer types is a promising route to manipulate TMDs' properties, not only as…

The nature of the pseudogap phase of cuprate high-temperature superconductors is a major unsolved problem in condensed matter physics. We studied the commencement of the pseudogap state at temperature T* using three different techniques…

Topologically ordered states of matter are generically characterized by excitations with quantum number fractionalization. A prime example is the spin liquid realized in Kitaev's honeycomb-lattice compass model where spin-flip excitations…

强关联电子 · 物理学 2018-11-12 C. Wellm , J. Zeisner , A. Alfonsov , A. U. B. Wolter , M. Roslova , A. Isaeva , T. Doert , M. Vojta , B. Büchner , V. Kataev

GeSe and SnSe monochalcogenide monolayers and bilayers undergo a two-dimensional phase transition from a rectangular unit cell to a square unit cell at a temperature $T_c$ well below the melting point. Its consequences on material…

The results of a single-crystal X-ray-diffraction study of the evolution of crystal structures of VI3 with temperature with emphasis on phase transitions are presented. Some related specific-heat and magnetization data are included. The…

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