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We report on the study of the magnetic excitations of Mott insulator La2CuO4 by using resonant inelastic x-ray scattering (RIXS) and cluster calculations within the framework of exact diagonalization. Our results demonstrate experimentally…

强关联电子 · 物理学 2025-10-06 A. Singh , H. Y. Huang , K. Tsutsui , T. Tohyama , S. Komiya , J. Okamoto , C. T. Chen , A. Fujimori , D. J. Huang

Young's archetypal double-slit experiment forms the basis for modern diffraction techniques: the elastic scattering of waves yields an interference pattern that captures the real-space structure. Here, we report on an inelastic incarnation…

Recent experiments on La$_2$CuO$_4$ suggest that indirect resonant inelastic X-ray scattering (RIXS) might provide a probe for transversal spin dynamics. We present in detail a systematic expansion of the relevant magnetic RIXS cross…

强关联电子 · 物理学 2011-07-22 Filomena Forte , Luuk J. P. Ament , Jeroen van den Brink

We derive general expressions for resonant inelastic x-ray scattering (RIXS) operators for $t_{2g}$ orbital systems, which exhibit a rich array of unconventional magnetism arising from unquenched orbital moments. Within the fast collision…

强关联电子 · 物理学 2017-08-16 B. J. Kim , Giniyat Khaliullin

We calculate the resonant inelastic X-ray scattering (RIXS) response of the Kitaev honeycomb model, an exactly solvable quantum-spin-liquid model with fractionalized Majorana and flux excitations. We find that the fundamental RIXS channels,…

强关联电子 · 物理学 2016-10-04 Gábor B. Halász , Natalia B. Perkins , Jeroen van den Brink

We calculate the resonant inelastic X-ray scattering (RIXS) response in a Mott insulator which is described by the Falicov-Kimball model. The model can be solved exactly within the single site dynamical mean-field theory (DMFT)…

强关联电子 · 物理学 2015-03-31 Nandan Pakhira , J. K. Freericks , A. M. Shvaika

Emergent symmetry breakings in condensed matter systems are often intimately linked to collective excitations. For example, the intertwined spin-charge stripe order in cuprate superconductors is associated with spin and charge excitations.…

The resonant inelastic x-ray scattering (RIXS) was measured in an insulating SrCuO$_{2}$ with changing the incident photon energy ($h\nu$) near the Cu $1s$ absorption edge (K-edge). Complex structures and their dependences on the momentum…

We report an Fe $L$-edge resonant inelastic x-ray scattering (RIXS) study of the unusual superconductor $\beta$-FeSe. The high energy resolution of this RIXS experiment ($\approx\,$55$\,$meV FWHM) made it possible to resolve low-energy…

超导电性 · 物理学 2019-01-16 M. C. Rahn , K. Kummer , N. B. Brookes , A. A. Haghighirad , K. Gilmore , A. T. Boothroyd

The orbital distribution of the spin fluctuation in the iron-based superconductors(IBSs) is the key information needed to understand the magnetism, superconductivity and electronic nematicity in these multi-orbital systems. In this work, we…

超导电性 · 物理学 2021-07-28 Da-Wei Yao , Tao Li

We analyze theoretically the resonant inelastic x-ray scattering (RIXS) at the Ni K edge in the stripe-ordered state of La_{2-x}Sr_xNiO_4 at x=1/3. In the calculation of RIXS spectra, the stripe-ordered ground state is described within the…

强关联电子 · 物理学 2012-01-18 Takuji Nomura , Eiji Kaneshita

Continued improvement of the energy resolution of resonant inelastic x-ray scattering (RIXS) spectrometers is crucial for fulfilling the potential of this technique in the study of electron dynamics in materials of fundamental and…

仪器与探测器 · 物理学 2017-09-11 Jungho Kim , D. Casa , Ayman Said , Richard Krakora , B. J. Kim , Elina Kasman , Xianrong Huang , T. Gog

We present RIXS data at O K edge from La2-xSrxCuO4 vs. doping between x=0.10 and x=0.22 with attention to the magnetic excitations in the Mid-Infrared region. The sampling done by RIXS is the same as in the undoped cuprates provided the…

超导电性 · 物理学 2012-06-29 V. Bisogni , M. Moretti Sala , A. Bendounan , N. B. Brookes , G. Ghiringhelli , L. Braicovich

We present a computational study of $L$-edge resonant inelastic x-ray scattering (RIXS) in correlated 3$d$ transition-metal oxides using an $ab$ $initio$ method based on local density approximation + dynamical mean-field theory (DMFT). The…

强关联电子 · 物理学 2020-03-25 Atsushi Hariki , Mathias Winder , Takayuki Uozumi , Jan Kuneš

We investigate theoretically the resonant inelastic x-ray scattering (RIXS) at the $K$ edge of Si on the basis of an ab initio calculation. We calculate the RIXS spectra with systematically varying transfered-momenta, incident-photon energy…

材料科学 · 物理学 2007-05-23 Yunori Nisikawa , Manabu Usuda , Jun-ichi Igarashi

We present a relativistic time-dependent density functional theory (TDDFT) approach for the simulation of resonant inelastic X-ray scattering (RIXS) spectra, based on both a full four-component (4c) Dirac-Coulomb Hamiltonian and a modern…

化学物理 · 物理学 2026-04-17 Lukas Konecny , Muhammed A. Dada , Daniel R. Nascimento , Michal Repisky

We provide a semiquantitative explanation of a recent experiment on the resonant inelastic x-ray scattering (RIXS) in insulating cuprate La2CuO4 (Y.J. Kim et al., Phys. Rev. Lett. 89, 177003 (2002).). We show theoretically that there are…

强关联电子 · 物理学 2009-11-10 Takuji Nomura , Jun-ichi Igarashi

We report a Cu K-edge resonant inelastic x-ray scattering (RIXS) study of orbital excitations in KCuF3 . By performing the polarization analysis of the scattered photons, we disclose that the excitation between the eg orbitals and the…

We report the high resolution resonant inelastic EUV scattering study of quantum Heisenberg antiferromagnet KCoF3. By tuning the EUV photon energy to cobalt M23 edge, a complete set of low energy 3d spin-orbital excitations is revealed.…

We studied the magnetic excitations in the quasi-one-dimensional (q-1D) ladder subsystem of Sr_(14-x) Ca_x Cu_24 O_41(SCCO) using Cu L_3-edge resonant inelastic X-ray scattering (RIXS). By comparing momentum-resolved RIXS spectra with…