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We develop a formalism for calculating resonant inelastic x-ray scattering (RIXS) spectra in systems of itinerant electrons with arbitrary band structures, accounting for the effect of the positively-charged core hole exactly. We apply this…

超导电性 · 物理学 2013-12-24 David Benjamin , Israel Klich , Eugene Demler

Inelastic x-ray scattering (IXS) with very high (meV) energy resolution has become a valuable spectroscopic tool, complementing the well established coherent inelastic neutron scattering (INS) technique for phonon dispersion investigations.…

强关联电子 · 物理学 2009-11-07 M. d'Astuto , P. K. Mang , P. Giura , A. Shukla , A. Mirone , M. Krisch , F. Sette , P. Ghigna , M. Braden , M. Greven

We use Ru $L_3$-edge (2838.5 eV) resonant inelastic x-ray scattering (RIXS) to quantify the electronic structure of Ca$_2$RuO$_4$, a layered $4d$-electron compound that exhibits a correlation-driven metal-insulator transition and…

强关联电子 · 物理学 2019-07-24 H. Gretarsson , H. Suzuki , Hoon Kim , K. Ueda , M. Krautloher , B. J. Kim , H. Yavaş , G. Khaliullin , B. Keimer

Resonant Inelastic X-ray Scattering (RIXS) in the soft x-ray range is an element-specific energy-loss spectroscopy used to probe the electronic and magnetic excitations in strongly correlated solids. In the recent years, RIXS has been…

Quasi-one-dimensional systems exhibit many-body effects elusive in higher dimensions. A prime example is spin-orbital separation, which has been measured by resonant inelastic X-ray scattering (RIXS) in Sr$_2$CuO$_3$. Here, we theoretically…

强关联电子 · 物理学 2022-10-03 Aaron Müller , Francesco Grandi , Martin Eckstein

We develop a theory of resonant inelastic x-ray scattering (RIXS) at the $K$ edge in La$_2$CuO$_4$ on the basis of the Keldysh Green's function formalism. In our previous analysis (Phys. Rev. B 71, 035110 (2005)), the scattering by the…

强关联电子 · 物理学 2015-06-25 Jun-ichi Igarashi , Takuji Nomura , Manabu Takahashi

We study the resonant inelastic x-ray scattering (RIXS) at the $K$ edge of Ge. We measure RIXS spectra with systematically varying momenta in the final state. The spectra are a measure of exciting an electron-hole pair. We find a single…

材料科学 · 物理学 2007-05-23 Yunori Nisikawa , Manabu Usuda , Jun-ichi Igarashi , Hironobu Shoji , Toshiaki Iwazumi

We present a formalism for the resonant inelastic x-ray scattering (RIXS) cross section. The resulting compact expression in terms of polarizability matrix elements, particularly lends itself to the implementation in an all-electron…

材料科学 · 物理学 2022-08-17 Christian Vorwerk , Francesco Sottile , Claudia Draxl

The community currently lacks a complete understanding of how resonant inelastic x-ray scattering (RIXS) experiments probe the electron-phonon ($e$-ph) interaction in solids. For example, most theoretical models of this process have focused…

强关联电子 · 物理学 2022-05-25 Krzysztof Bieniasz , Steve Johnston , Mona Berciu

We report resonant inelastic x-ray scattering (RIXS) excited by circularly polarized x-rays on Mn-Zn ferrite at the Mn L2,3-resonances. We demonstrate that crystal field excitations, as expected for localized systems, dominate the RIXS…

材料科学 · 物理学 2012-01-04 M. Magnuson , L. -C. Duda , S. M. Butorin , P. Kuiper , J. Nordgren

We use neutron scattering to study spin excitations in single crystals of LiFe$_{0.88}$Co$_{0.12}$As, which is located near the boundary of the superconducting phase of LiFe$_{1-x}$Co$_{x}$As and exhibits non-Fermi-liquid behavior…

A new method is presented for describing vibrational effects in x-ray absorption spectroscopy (XAS) and resonant inelastic x-ray scattering (RIXS) using a combination of the classical Franck-Condon (FC) approximation and classical…

材料科学 · 物理学 2017-12-20 Mathias P. Ljungberg

We report a comprehensive resonant inelastic x-ray scattering (RIXS) study of various iridate materials focusing on core-level excitations and transitions between crystal-field split d-levels. The 2p core hole created at the Ir $L_3$…

强关联电子 · 物理学 2018-05-10 Young-June Kim , J. P. Clancy , H. Gretarsson , G. Cao , Yogesh Singh , Jungho Kim , M. H. Upton , D. Casa , T. Gog

We report on the Cu 1s resonant inelastic X-ray scattering (RIXS) of Cu-O one-dimensional (1D) strongly correlated insulator systems with contrasting atomic arrangements, namely edge-sharing CuGeO3 and corner-sharing Sr2CuO3. Owing to good…

Electronic spin and orbital (dd) excitation spectra of (Ca{x}La{1-x})(Ba{1.75-x}La{0.25+x})Cu{3}O{y} samples are measured by resonant inelastic x-ray scattering (RIXS). In this compound, Tc of samples with identical hole dopings is strongly…

We investigate high-energy spin excitations in hole-doped La$_{2-x}$Ca$_{x}$CuO$_{4-\delta}$ films across a broad Ca doping range $x = 0.05-0.50$ using resonant inelastic x-ray scattering (RIXS). Polarization analysis and incident-photon…

Su-Schrieffer-Heeger (SSH)-like electron-phonon (e-ph) interactions can drive the formation of light (bi)polarons and several novel states of matter. It is, therefore, prudent to develop experimental protocols for identifying such couplings…

强关联电子 · 物理学 2024-12-23 Debshikha Banerjee , Jinu Thomas , Alberto Nocera , Steven Johnston

We investigate the spin dynamics of a 1D spin-1/2 Heisenberg tetramer chain. Employing a combination of Density Matrix Renormalization Group, quantum renormalization group, and perturbation theory techniques, we compute the energy levels…

强关联电子 · 物理学 2026-05-08 Junli Li , Jun-Qing Cheng , Trinanjan Datta , Dao-Xin Yao

Recent improvements in the energy resolution of resonant inelastic x-ray scattering experiments (RIXS) at the Cu-L$_3$ edge have enabled the study of lattice, spin, and charge excitations. Here, we report on the detection of a low intensity…

We use Ru $L_3$-edge resonant inelastic x-ray scattering (RIXS) to study the full range of excitations in Ca$_3$Ru$_2$O$_7$ from meV-scale magnetic dynamics through to the eV-scale interband transitions. This bilayer $4d$-electron…

强关联电子 · 物理学 2021-02-10 J. Bertinshaw , M. Krautloher , H. Suzuki , H. Takahashi , A. Ivanov , B. J. Kim , H. Gretarsson , B. Keimer