相关论文: Fast dynamics in glass-forming salol investigated …
We provide broadband dielectric loss spectra of glass-forming glycerol with varying additions of LiCl. The measurements covering frequencies up to 10 THz extend well into the region of the fast beta process, commonly ascribed to caged…
We have studied the high-frequency dynamics of salol by inelastic x-ray scattering over a wide temperature range between 50 and 450 K, across the glass transition. We find that salol efficiently realizes the mechanism of dynamical arrest…
Dielectric spectroscopy is one of the most commonly used techniques for the investigation of the dynamic response of glass-forming materials. The tremendous slow-down of the particle motions when approaching the glass transition and…
We report a thorough dielectric characterization of the alpha relaxation of glass forming glycerol with varying additions of LiCl. Nine salt concentrations from 0.1 - 20 mol% are investigated in a frequency range of 20 Hz - 3 GHz and…
We study the slow dynamics of salol by varying both temperature and pressure using photon correlation spectroscopy and pressure-volume-temperature measurements, and compare the behavior of the structural relaxation time with equations…
We have performed dielectric spectroscopy on the molecular glass-formers glycerol, propylene carbonate (PC) and the ionic melts CKN and CRN. The frequency range covers almost 20 decades from some micro-Hz to some THz. The meausrement…
Broadband dielectric spectroscopy was used to study the molecular orientational dynamics of the glass-forming, thioether-linked cyanobiphenyl liquid crystal dimers. As was expected theoretically, two different relaxation processes that…
Mean square displacements of hydrogen atoms in glass-forming materials and proteins, as reported by incoherent elastic neutron scattering, show kinks in their temperature dependence. This crossover, known as the dynamical transition,…
We discuss a novel approach, the point-to-set correlation functions, that allows to determine relevant static and dynamic length scales in glass-forming liquids. We find that static length scales increase monotonically when the temperature…
The glasses in the system (100-x)TeO2-xCaCu3Ti4O12, (x=0.25 to 3 mol %) were fabricated. The color varied from olive green to brown as the CaCu3Ti4O12 (CCTO) content increased in TeO2 matrix. The X-ray powder diffraction and differential…
Glass sound velocity shift was observed to be longarithmically temperature dependent in both relaxation and resonance regimes: $\Delta c/c=\mathcal{C}\ln T$. It does not monotonically increase with temperature from $T=0$K, but to reach a…
Dielectric measurements at very low temperature indicate that in a glass with the eutectic composition BaO-Al$_2$O$_3$-SiO$_2$ a phase transition occurs at 5.84 mK. Below that temperature small magnetic fields of the order of 10 $\mu$T…
In low-temperature glasses, the sound velocity changes as the logarithmic function of temperature below $10$K: $[c(T) - c(T_0)]/c(T_0) = \mathcal{C}\ln(T/T_0)$. With increasing temperature starting from $T=0$K, the sound velocity does not…
We give evidence of a clear structural signature of the glass transition, in terms of a static correlation length with the same dependence on the system size which is typical of critical phenomena. Our approach is to introduce an external,…
We present quasi-elastic light scattering (LS) and dielectric (DS) spectra of the glass former alpha-picoline (13K < T < 320K). At high temperatures the evolution of the susceptibility minimum is well described by mode coupling theory (MCT)…
We present the results of broadband dielectric spectroscopy on two glass formers with strong Johari-Goldstein beta-relaxations. In addition to the alpha- and beta-relaxation dynamics, the extension of the spectra up to 1 THz also allows…
The high-pressure dynamics of a computer-modeled silica melt is studied in the framework of the mode-coupling theory of the glass transition (MCT) using static-structure input from molecular-dynamics (MD) computer simulation. The theory…
We propose that acousto-optical coupling of the electric field to strain fields around defects in disordered $^4$He is causing an increase of the dielectric function with decreasing temperature due to the arrested dynamics of defect…
We have measured the linear dielectric susceptibility of two molecular glass formers close to Tg in order to estimate the size of the dynamically correlated clusters of molecules which are expected to govern the physics of glass formation.…
The dynamic structure factor of glassy and liquid glycerol has been measured by inelastic X-ray scattering in the exchanged momentum ($Q$) region $Q$=2$\div$23 nm$^{-1}$ and in the temperature range 80$\div$570 K. Beside the propagating…