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We theoretically investigate high-order harmonic generation (HHG) in Rydberg atoms driven by spatially inhomogeneous laser fields, induced, for instance, by plasmonic enhancement. It is well known that the laser intensity should to exceed…

原子物理 · 物理学 2016-07-08 Y. Tikman , I. Yavuz , M. F. Ciappina , A. Chacon , Z. Altun , M. Lewenstein

The generation and control of the properties of light beams carrying orbital angular momentum is fundamental to extend our understanding on the light-matter interaction process. In this letter, we investigate the use of anomalous and…

光学 · 物理学 2025-09-11 B. Kumar Das , M. Ciappina , W. Gao , C. Granados

High-harmonic generation (HHG) in solids has typically been explored in transparent dielectrics and semiconductors. Metals have long been dismissed due to their strong reflectivity at infrared wavelengths. Here, we demonstrate HHG from…

Titanium diselenide (TiSe$_{2}$) is a transition-metal dichalcogenide material that undergoes a charge-density-wave (CDW) transition at $T_{c}\approx 200\,\mathrm{K}$. In a recent experiment [I. Tyulnev {\it et al.}, Commun. Mater. 6, 152…

High-order harmonic generation (HHG) in aligned linear molecules can offer valuable information about strong-field interactions in lower-lying molecular orbitals, but extracting this information is difficult for three-dimensional molecular…

We establish time-resolved high harmonic generation (tr-HHG) as a powerful spectroscopy for photoinduced dynamics in strongly correlated materials through a detailed investigation of the insulator-to-metal transitions in vanadium dioxide.…

We present a detailed calculation of the linear and nonlinear optical response of four types of monolayer Two-Dimensional (2D) Transition-Metal Dichalcogenides (TMDCs), having the formula $\textrm{MX}_2$ with M=Mo,W and X=S,Se. The…

介观与纳米尺度物理 · 物理学 2018-08-28 Sina Khorasani

Single-layer transition metal dichalcogenides (TMDCs) can adopt two distinct structures corresponding to different coordination of the metal atoms. TMDCs adopting the T-type structure exhibit a rich and diverse set of phenomena, including…

介观与纳米尺度物理 · 物理学 2020-07-29 Daniel T. Larson , Wei Chen , Steven B. Torrisi , Jennifer Coulter , Shiang Fang , Efthimios Kaxiras

Two-dimensional transition metal dichalcogenides (TMDCs) are promising materials for next-generation optoelectronic devices, yet their implementation is hindered by limited sample stability and challenges in forming reliable electrical…

We present a study of the possibility to significantly enhance the efficiency of high-order harmonic generation (HHG) using few-cycle optical waveforms obtained by superposing two laser pulses of different color delayed optimally relative…

光学 · 物理学 2024-12-11 O. V. Meshkov , M. Yu. Emelin , M. Yu. Ryabikin

We study high-order harmonic generation (HHG) in model atoms driven by plasmonic-enhanced fields. These fields result from the illumination of plasmonic nanostructures by few-cycle laser pulses. We demonstrate that the spatial inhomogeneous…

Two-dimensional materials offer a versatile platform to study high-harmonic generation (HHG), encompassing as limiting cases bulk-like and atomic-like harmonic generation [Tancogne-Dejean and Rubio, Science Advance \textbf{4}, eaao5207…

材料科学 · 物理学 2018-10-31 Guillaume Le Breton , Angel Rubio , Nicolas Tancogne-Dejean

We propose a novel method for controlling the high-harmonic generation (HHG) with a high dynamic range in single-layer graphene. We find that, by utilizing shear strain, a significant enhancement or quenching of HHG is possible over a range…

介观与纳米尺度物理 · 物理学 2023-03-02 Tomohiro Tamaya , Hidefumi Akiyama , Takeo Kato

Low-dimensional transition metal dichalcogenides (TMDC) exhibit great photocatalytic performance and tunability. In this work, using first-principles simulations based on density functional theory (DFT), we demonstrate that external…

材料科学 · 物理学 2022-10-06 Zhao Liu , Biao Wang , Claudio Cazorla

High harmonic generation (HHG) in solids has recently emerged as a powerful all-optical approach for probing material properties and ultrafast electron dynamics in quantum systems. It has been widely applied for studying two-dimensional and…

光学 · 物理学 2026-04-28 Eyal Uzner , Ofer Neufeld

High-order harmonic generation (HHG) with relativistically strong laser pulses is considered employing electron ionization-recollisions from multiply charged ions in counterpropagating, linearly polarized attosecond pulse trains. The…

原子物理 · 物理学 2015-05-19 Markus C. Kohler , Michael Klaiber , Karen Z. Hatsagortsyan , Christoph H. Keitel

Excitons in semiconductors, bound pairs of excited electrons and holes, can form the basis for new classes of quantum optoelectronic devices. A van der Waals heterostructure built from atomically thin semiconducting transition metal…

High-harmonic generation (HHG) in solids has rapidly emerged as a promising platform for creating compact attosecond sources and probing ultrafast electron dynamics. Resonant metasurfaces are essential for enhancement of the otherwise small…

In the present paper, we investigate the high-order harmonic generation (HHG) from diatomic molecules with large internuclear distance using a strong field approximation (SFA) model. We find that the hump and dip structure emerges in the…

原子物理 · 物理学 2009-11-13 Y. J. Chen , J. Liu

High harmonic generation (HHG) is a widely explored process in solids, where intense lasers drive attosecond-to-femtosecond electron dynamics within bands, causing high-energy emission. While electrons and photons are considered the main…

光学 · 物理学 2026-04-28 Adam Herling , Ofer Neufeld