相关论文: Coherent phonons in a $Bi_2Se_3$ film generated by…
Density Functional Theory (DFT) calculations not only allow to predict the vibrational and optical properties of solids but also to understand and disentangle the mechanisms playing a key role in the generation of coherent optical phonons.…
Selective excitation of coherent high-amplitude vibrations of atoms in a solid can induce exotic nonequilibrium states, in which the character of interactions between electronic, magnetic and lattice degrees of freedom is considerably…
We have studied the polarization dependence of coherent phonons in the topological insulator Bi2Te3. Using polarization-dependent femtosecond pump-probe spectroscopy, we measured coherent phonons as a function of angle when the pump and…
Time-resolved two color pump-probe polarization spectroscopy was performed at room temperature on SrTiO3 films grown directly on Si with film thickness varying from 2 nm to 7.8 nm. The E soft mode with a characteristic frequency of 0.2 THz…
We have applied femtosecond pump-probe technique with variable pump wavelength to study coherent lattice dynamics in Bi single crystal. Comparison of the coherent amplitude as a function of pump photon energy for two different in symmetry…
Transient reflectivity traces measured for nanometer-sized films of the topological insulator Bi2Se3 revealed GHz-range oscillations driven within the relaxation of hot carriers photoexcited with ultrashort laser pulses of 1.51 eV photon…
Driving coherent lattice motion with THz pulses has emerged as a novel pathway for achieving dynamic stabilization of exotic phases that are inaccessible in equilibrium quantum materials. In this work, we present a previously unexplored…
We report on the impulsive generation of coherent optical phonons in CdTe0.68Se0.32 nanocrystallites embedded in a glass matrix. Pump probe experiments using femtosecond laser pulses were performed by tuning the laser central energy to…
We directly measure by femtosecond time-resolved x-ray diffraction the E$_g$ symmetry coherent phonon excited in bismuth by strong optical excitation. The magnitude of the E$_g$ mode observed is 0.2 pm peak-to-peak, compared against the 2.7…
We investigate coherent lattice dynamics in optimally doped YBa$_2$Cu$_3$O$_{7-\delta}$ driven by ultrashort ($\sim$ 12 fs) near infrared (NIR) and near ultraviolet (NUV) pulses. Transient reflectivity experiments, performed at room…
We present a transient absorption setup combining broadband detection over the visible-UV range with high temporal resolution ($\sim$20fs) which is ideally suited to trigger and detect vibrational coherences in different classes of…
High quality single crystals of Bi2Se3 were grown using a modified Bridgman technique, the detailed study were carried out using Raman spectroscopy and characterized by Laue diffraction and high resolution transmission electron microscopy.…
Here, we investigate phonon mode- and electron band-selective electron-phonon couplings in centrosymmetric 1T$'$-MoTe$_2$ using time- and angle-resolved photoemission spectroscopy combined with frequency-domain analysis. Femtosecond…
Using $\approx$40 fs ultrashort laser pulses, we investigate the picosecond acoustic response from a prototypical phase change material, thin Ge$_{2}$Sb$_{2}$Te$_{5}$ (GST) films with various thicknesses. After excitation with a 1.53…
We demonstrate the generation of coherent phonons in a quartz Bulk Acoustic Wave (BAW) resonator through the photoelastic properties of the crystal, via the coupling to a microwave cavity enhanced by a photonic lambda scheme. This is…
Using first principles, all-electron calculations and dynamical simulations we study the behavior of the A_1g and E_g coherent phonons induced in Bi by intense laser pulses. We determine the potential landscapes in the laser heated material…
Fully symmetric A1g phonons are expected to play a dominant role in electron scattering in strong topological insulators (TIs), thus limiting the ballistic transport of future electronic devices. Here, we report on femtosecond time-resolved…
Ultrathin FeSe films grown on SrTiO$_{3}$ substrates are a recent milestone in atomic material engineering due to their important role in understanding unconventional superconductivity in Fe-based materials. Using femtosecond time- and…
We discuss the mechanism of coherent phonon generation by Stimulated Ionic Raman Scattering, a process different from conventional excitation with near visible optical pulses. Ionic Raman scattering is driven by anharmonic coupling between…
Zone-folded acoustic phonons (6 THz) in 4H silicon carbide (SiC) have been coherently excited using a femtosecond near-infrared pulse and measured through transient reflectivity with a pump and probe protocol. Their amplitude is coherently…