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The colloidal 2D materials based on graphene and its modifications are of great interest when it comes to forming LC phases. These LC phases allow controlling the orientational order of colloidal particles, paving the way for the efficient…

材料科学 · 物理学 2023-05-30 H. Gharagulyan , Y. Melikyan , V. Hayrapetyan , Kh. Kirakosyan , D. A. Ghazaryan , M. Yeranosyan

A deeper understanding of the cathode electrolyte interphase (CEI) formation mechanism is essential to elucidate battery degradation. Here, we combine Liquid Electrochemical Transmission Electron Microscopy (ec-TEM) with Gas…

Controlled formation of porous silicon has been of primary importance for numerous landmark applications such as light emitting sources, sensors, actuators, drug delivery systems, and energy storage applications. Frequently explored methods…

Embedding silicon nanoparticles in an intermetallic matrix is a promising strategy to produce remarkable bulk anode materials for lithium-ion (Li-ion) batteries with low potential, high electrochemical capacity and good cycling stability.…

To reduce the experimental validation workload for chemical researchers and accelerate the design and optimization of high-energy-density lithium metal batteries, we aim to leverage models to automatically predict Coulombic Efficiency (CE)…

机器学习 · 计算机科学 2024-07-31 Xinhe Li , Zhuoying Feng , Yezeng Chen , Weichen Dai , Zixu He , Yi Zhou , Shuhong Jiao

Lithium thiophosphates (LPS) with the composition (Li$_2$S)$_x$(P$_2$S$_5$)$_{1-x}$ are among the most promising prospective electrolyte materials for solid-state batteries (SSBs), owing to their superionic conductivity at room temperature…

材料科学 · 物理学 2022-01-28 Haoyue Guo , Qian Wang , Alexander Urban , Nongnuch Artrith

The orientational and translational order of a thermotropic ferroelectric liquid crystal (2MBOCBC) imbibed in self-organized, parallel, cylindrical pores with radii of 10, 15, or 20 nm in anodic aluminium oxide monoliths (AAO) are explored…

Pressure-induced phase transformation occurs during silicon (Si) wafering processes. \b{eta}-tin (Si-II) phase is formed at high pressures, followed by the transformation to Si-XII, Si-III or/and amorphous Si ({\alpha}-Si) phases during the…

Solid-state lithium batteries have attracted considerable attention due to their potential to provide improved safety and higher energy density compared with conventional liquid electrolyte batteries. However, the stability of the interface…

材料科学 · 物理学 2026-04-14 Deobrat Singh , Li-Yun Tian , Moyses Araujo , Raquel Lizarraga

The increasing relevance of energy storage technologies demands high-capacity cathode materials for Li-ion batteries. Recently, Li-rich defect anti-fluorite Li$_5$FeO$_4$ has emerged as a high-capacity cathode material exhibiting…

材料科学 · 物理学 2022-06-24 Anu Maria Augustine , Vishnu Sudarsanan , P. Ravindran

Superelastic NiTi tubes are promising candidates for eco-friendly elastocaloric cooling, but their cyclic stability suffers severely from functional degradation. Herein, we investigate the functional degradation of nanocrystalline NiTi…

材料科学 · 物理学 2021-07-26 Dingshan Liang , Peng Hua , Junyu Chen , Fuzeng Ren , Qingping Sun

Nanoconfined liquid crystals (LCs) and their nanocomposites are driving the next generation of photonic applications. Consequently, deepening our understanding of mesophase stability, defect topology, and the dynamic response of LCs at the…

Lithium metal batteries (LMBs), when coupled with a localized high-concentration electrolyte and a high-voltage nickel-rich cathode, offer a solution to the increasing demand for high energy density and long cycle life. However, the…

材料科学 · 物理学 2024-01-12 Tao Meng , Shanshan Yang , Yitong Peng , Xiwei Lan , Pingan Li , Kangjia Hu , Xianluo Hu

Our investigations on porous Si show that on increase of pressure it undergoes crystalline phase transitions instead of pressure induced amorphization - claimed earlier, and the amorphous phase appears only on release of pressure. This…

材料科学 · 物理学 2010-07-23 Nandini Garg , K. K. Pandey , K. V. Shanavas , C. A. Betty , Surinder M Sharma

Solid-state batteries require electrolytes that sustain high ionic conductivity under the mechanical environment of a functioning cell. Lattice strain, arising from stack pressure, thermal cycling, or lattice mismatch at interfaces, can…

材料科学 · 物理学 2026-05-08 Wei-Fan Huang , Jin Dai , Jiahui Pan , Mingjian Wen

Metal fluoride and oxides can store multiple lithium-ions through conversion chemistry to enable high energy-density lithium-ion batteries. However, their practical applications have been hindered by an unusually large voltage hysteresis…

材料科学 · 物理学 2016-07-08 Linsen Li , Ryan Jacobs , Peng Gao , Liyang Gan , Feng Wang , Dane Morgan , Song Jin

A common thread in designing electrochemically-based renewable energy devices comprises materials that exploit nano-scale morphologies, e.g., supercapacitors, batteries, fuel cells, and bulk heterojunction organic photovoltaics. In these…

斑图形成与孤子 · 物理学 2019-02-25 Alon Z. Shapira , Nir Gavish , Arik Yochelis

Electrolyte reduction products form the solid-electrolyte interphase (SEI) on negative electrodes of lithium-ion batteries. Even though this process practically stabilizes the electrode-electrolyte interface, it results in continued…

化学物理 · 物理学 2018-11-22 Birger Horstmann , Fabian Single , Arnulf Latz

This computational research study analyzes the increase of the specific charge capacity that comes with the reduction of the anisotropic volume expansion during lithium ion insertion within silicon nanowires. This research paper is a…

应用物理 · 物理学 2024-03-03 Donald C. Boone

In this study, we propose a novel approach for investigating the formation of solid electrolyte interphase (SEI) in Na-ion batteries (NIB) through the coupling of in situ liquid electrochemical transmission electron microscopy (ec-TEM) and…