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We present consistent results for molecular conduction using two central-complementary approaches: the non-equilibrium Green's function technique and the quantum master equation method. Our model describes electronic conduction in a…

介观与纳米尺度物理 · 物理学 2016-04-13 Bijay Kumar Agarwalla , Dvira Segal

We calculate the electron-phonon scattering and binding in semiconducting carbon nanotubes, within a tight binding model. The mobility is derived using a multi-band Boltzmann treatment. At high fields, the dominant scattering is inter-band…

材料科学 · 物理学 2009-11-10 Vasili Perebeinos , J. Tersoff , Phaedon Avouris

Electron-phonon (E-p) coupling incorporated density functional theory (DFT) based investigation of structural, electronic and vibrational properties of bulk MgSe and MgTe is presented. Electron-phonon coupling is incorporated to understand…

材料科学 · 物理学 2024-11-19 Maitry Joshi , Trupti K Gajaria , Prafulla K. Jha

A thorough understanding of the microscopic picture of heat conduction in solids is critical to a broad range of applications, from thermal management of microelectronics to more efficient thermoelectric materials. The transport properties…

材料科学 · 物理学 2021-02-04 Yujie Quan , Shengying Yue , Bolin Liao

We present a technique to calculate the transport properties through one-dimensional models of molecular wires. The calculations include inelastic electron scattering due to electron-lattice interaction. The coupling between the electron…

凝聚态物理 · 物理学 2009-10-31 H. Ness , S. A. Shevlin , A. J. Fisher

We have developed a first-principles method to calculate the electron-phonon coupling for specific modes and q-points in the Brillouin Zone for crystalline organic semiconductors. Using the obtained coupling strengths, we propose an…

In this work, we use a combination of first-principles calculations under the density functional theory framework and heat transport simulations using the atomistic Green's function (AGF) method to quantitatively predict the contribution of…

介观与纳米尺度物理 · 物理学 2017-03-01 Sridhar Sadasivam , Ning Ye , James Charles , Kai Miao , Joseph P. Feser , Tillmann Kubis , Timothy S. Fisher

We consider resonant transport through a molecular quantum dot coupled to a local vibration mode. Applying the non-equilibrium Green function technique in the polaron representation, we develop a non-perturbative scheme to calculate the…

介观与纳米尺度物理 · 物理学 2009-11-13 Alex Zazunov , Thierry Martin

This paper investigates the mobility of electrons scattering from the coupled system of electrons and longitudinal optical (LO) phonons in n-type GaAs. The Boltzmann equation is solved exactly for low electric fields by an iterative method,…

凝聚态物理 · 物理学 2016-08-31 B. A. Sanborn

In polar semiconductors and oxides, the long-range nature of the electron-phonon (\textit{e}-ph) interaction is a bottleneck to compute charge transport from first principles. Here, we develop an efficient ab initio scheme to compute and…

材料科学 · 物理学 2016-12-07 Jin-Jian Zhou , Marco Bernardi

The phonon Boltzmann transport equation (BTE) has been widely utilized to study thermal transport in solids. While for a number of materials the exact solution to the BTE has been obtained for a uniform heat flow, problems arising in…

介观与纳米尺度物理 · 物理学 2021-11-17 Vazrik Chiloyan , Samuel Huberman , Zhiwei Ding , Jonathan Mendoza , Alexei A. Maznev , Keith A. Nelson , Gang Chen

Employing the nonequilibrium Green's function method, we develop a fully quantum mechanical model to study the coupled electron-phonon transport in one-dimensional atomic junctions in the presence of a weak electron-phonon interaction. This…

介观与纳米尺度物理 · 物理学 2008-03-04 J. T. Lü , Jian-Sheng Wang

Structural phase transitions and soft phonon modes pose a longstanding challenge to computing electron-phonon (e-ph) interactions in strongly anharmonic crystals. Here we develop a first-principles approach to compute e-ph scattering and…

材料科学 · 物理学 2018-12-04 Jin-Jian Zhou , Olle Hellman , Marco Bernardi

Accurate models of carrier transport are essential for describing the electronic properties of semiconductor materials. To the best of our knowledge, the current models following the framework of the Boltzmann transport equation (BTE)…

材料科学 · 物理学 2015-06-17 Alireza Faghaninia , Joel W. Ager , Cynthia S. Lo

We study electron transport in polycyclic hydrocarbon molecules attached to two semi-infinite one-dimensional metallic electrodes by the use of Green's function formalism. Parametric calculations based on the tight-binding framework are…

介观与纳米尺度物理 · 物理学 2009-11-06 Santanu K. Maiti

Heat transport at nanoscales in semiconductors is investigated with a statistical method. The Boltzmann Transport Equation (BTE) which characterize phonons motion and interaction within the crystal lattice has been simulated with a Monte…

经典物理 · 物理学 2009-11-11 David Lacroix , Karl Joulain

Electron-phonon coupling is a key interaction that governs diverse physical processes such as carrier transport, superconductivity, and optical absorption. Calculating such interactions from first-principles with methods beyond…

材料科学 · 物理学 2025-08-21 Aleksandr Poliukhin , Nicola Colonna , Francesco Libbi , Samuel Poncé , Nicola Marzari

In this work, the effect of electron-phonon (e-ph) coupling on both electron and phonon transport of metals is investigated via first principles calculations. A Monte-Carlo (MC) approach for solving the coupled electron-phonon Boltzmann…

材料科学 · 物理学 2024-02-14 Jie Peng , W. Ryan Deskins , Maria Helena Braga , Anter El-Azab

Developing simplified, but accurate, theoretical approaches to treat heat transport on all length and time scales is needed to further enable scientific insight and technology innovation. Using a simplified form of the Boltzmann transport…

介观与纳米尺度物理 · 物理学 2015-06-23 Jesse Maassen , Mark Lundstrom

In this research work, roll-to-roll chemical vapor deposited graphene device electronic transport properties are benchmarked to elucidate and comprehend mobility degradation in the real-world commercial application of graphene devices.…

介观与纳米尺度物理 · 物理学 2022-10-13 Bhupesh Bishnoi