相关论文: Coherent spin dynamics in gadolinium-doped CaWO4 c…
Obtaining a high Rabi oscillation frequency homogeneously across a spatially-extended population of nitrogen-vacancy (NV) center electronic spins in diamond is useful for efficient spin-state manipulation of the NV ensemble and in using NVs…
Interfacing photonic and solid-state qubits within a hybrid quantum architecture offers a promising route towards large scale distributed quantum computing. Ideal candidates for coherent qubit interconversion are optically active spins…
Electron spins hold great promise for quantum computation due to their long coherence times. An approach to realize interactions between distant spin-qubits is to use photons as carriers of quantum information. We demonstrate strong…
Raman heterodyne spectroscopy is a powerful tool for characterizing the energy and dynamics of spins. The technique uses an optical pump to transfer coherence from a spin transition to an optical transition where the coherent emission is…
Using soft-x-ray absorption spectroscopy at the Co-$L_{2,3}$ and O-$K$ edges, we demonstrate that the Co$^{3+}$ ions with the CoO$_{5}$ pyramidal coordination in the layered Sr$_2$CoO$_3$Cl compound are unambiguously in the high spin state.…
Polyoxometalate single ion magnet [GdW$_{30}$P$_5$O$_{110}$]$^{12-}$ has been studied by generalized Rabi oscillation experiments. It was possible to increase the number of coherent rotations tenfold through matching the Rabi frequency with…
Counting the microwave photons emitted by an ensemble of electron spins when they relax radiatively has recently been introduced as a sensitive new method for electron paramagnetic resonance spectroscopy at millikelvin temperatures. Here,…
Properties of trivalent cobalt oxide compounds are largely influenced by the spin state of the six 3d electrons at each Co site. High-spin Co3+ ions, where orbital angular momentum is only partially quenched, often exhibit significant…
The simple resonant Rabi oscillation of a two-level system in a single-mode coherent field reveals complex features at the mesoscopic scale, with oscillation collapses and revivals. Using slow circular Rydberg atoms interacting with a…
We study spin dynamics for two electrons confined to a double quantum dot under the influence of an oscillating exchange interaction. This leads to driven Rabi oscillations between the $\ket{\uparrow\downarrow}$--state and the…
The spinel cobalt oxide Co3O4 is a magnetic semiconductor containing cobalt ions in Co2+ and Co3+ oxidation states. We have studied the electronic, magnetic and bonding properties of Co3O4 using density functional theory (DFT) at the…
A low-noise cryogenic microwave spectroscopy experiment was performed on a high-purity lithium fluoride (LiF) crystal. The spectroscopy data revealed avoided level crossing interactions in whispering gallery modes, indicative of electron…
We analyze a prototypical particle-in-a-box model for a hole spin qubit. This quantum dot is subjected to static magnetic and electric fields, and to a radio-frequency electric field that drives Rabi oscillations owing to spin-orbit…
A hole spin is a potential solid-state q-bit, that may be more robust against nuclear spin induced dephasing than an electron spin. Here we propose and demonstrate the sequential preparation, control and detection of a single hole spin…
We have observed an environmentally induced quantum dynamical phase transition in the dynamics of a two spin experimental swapping gate [J. Chem. Phys. 124, 194507 (2006)]. There, the exchange of the coupled states |+,-> and ,+> gives an…
We have investigated the valence, spin, and orbital state of the Co ions in the one-dimensional cobaltate Ca3Co2O6 using x-ray absorption and x-ray magnetic circular dichroism at the Co-L2,3 edges. The Co ions at both the octahedral Co_oct…
The 3d electronic structure and phase transition in pure and Cr doped V2O3 are theoretically investigated in relation to the 3d spin-orbit interaction and lattice distortion. A model consisting of the nearest-neighbor V ion pair with full…
Decay of Rabi oscillations of equivalent spins diluted in diamagnetic solid matrix and coupled by magnetic dipole interactions is studied. It is shown that these interactions result in random shifts of spin transient nutation frequencies…
Hole spins in semiconductor quantum dots can be efficiently manipulated with radio-frequency electric fields owing to the strong spin-orbit interactions in the valence bands. Here we show that the motion of the dot in inhomogeneous strain…
We propose a new treatment of the dynamics of a periodically time-dependent Liouvillian by mapping it onto a time-independent problem and give a systematic expansion for its effective Liouvillian. In the case of a two-level system, the…