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Structural phase transitions in the organic inorganic metal halide perovskites are driven via rearrangement of methylammonium cation and distortion in the PbX6 octahedra. Compositional tuning is usually incorporated for suppression of the…

The hybrid organic inorganic perovskites (HOIPs) have attracted much attention for their potential applications as novel optoelectronic devices. Remarkably, the Rashba band splitting, together with specific spin orientations in k space…

材料科学 · 物理学 2020-07-21 Feng Lou , Teng Gu , Junyi Ji , Junsheng Feng , Hongjun Xiang , Alessandro Stroppa

The applicability and usefulness of Rashba model have been extended by recent observations in the field of spintronics, such as the spin-orbit torque at the junction interfaces between ferromagnetic (FM) metals and non-magnetic (NM) metals…

材料科学 · 物理学 2018-03-14 Akimasa Sakuma

The spin-split indirect bandgap in hybrid-halide perovskites provides a momentum-space realisation of a photon-ratchet intermediate band. Excited electrons thermalise to recombination-protected Rashba pockets offset in momentum space,…

In recent years, organic-inorganic hybrid perovskites have attracted wide attention due to their excellent optoelectronic properties in the application of optoelectronic devices. In the manufacturing process of perovskite solar cells,…

材料科学 · 物理学 2020-04-01 Lei Guo , Gao Xu , Gang Tang , Daining Fang , Jiawang Hong

The recent reaching of 20% of conversion efficiency by solar cells based on metal hybrid perovskites (MHP), e.g., the methylammonium (MA) lead iodide, CH3NH3PbI3 (MAPbI3), has excited the scientific community devoted to the photovoltaics…

化学物理 · 物理学 2018-12-14 Diego Guedes-Sobrinho , Ivan Guilhon , Marcelo Marques , Lara K. Teles

We show that the anomalous Hall effect (AHE) at a magnetic interface with strong spin-orbit coupling can be tuned with an external electric field. By altering the strength of the inversion symmetry breaking, the electric field changes the…

强关联电子 · 物理学 2018-12-24 Sayantika Bhowal , S. Satpathy

Spin-orbit coupling (SOC) combined with broken inversion symmetry play key roles in inducing Rashba effect. The combined spontaneous polarization and Rashba effect enable controlling a material's spin degrees of freedom electrically. In…

材料科学 · 物理学 2023-05-09 Amreen Bano , Dan Thomas Major

We report a model describing the molecular orientation disorder in CH3NH3PbI3, solving a classical Hamiltonian parametrised with electronic structure calculations, with the nature of the motions informed by ab-initio molecular dynamics. We…

介观与纳米尺度物理 · 物理学 2014-12-15 Jarvist M. Frost , Keith T. Butler , Aron Walsh

Tuning the thermal transport properties of hybrid halide perovskites is critical for their applications in optoelectronics, thermoelectrics, and photovoltaics. Here, we demonstrate an effective strategy to modulate the thermal transport…

材料科学 · 物理学 2024-01-02 Guang Wang , Hongzhao Fan , Zhongwei Chen , Yufei Gao , Zuankai Wang , Zhigang Li , Haipeng Lu , Yanguang Zhou

All-inorganic halide perovskites have attracted a great interest as a promising light harvester of perovskite solar cells due to their enhanced chemical stability. In this work we investigate the material properties of solid solutions…

材料科学 · 物理学 2020-04-22 Chol-Jun Yu , Un-Hyok Ko , Suk-Gyong Hwang , Yun-Sim Kim , Un-Gi Jong , Yun-Hyok Kye , Chol-Hyok Ri

The electronic properties of ABX3 (A = Cs, CH3NH3, NH2CHNH2; B = Sn, Pb; X = Cl, Br, I) type compounds in the cubic phase are systematically studied using the first-principles calculations. We find that these compounds have direct band gaps…

材料科学 · 物理学 2015-06-17 Li Lang , Ji-Hui Yang , Heng-Rui Liu , H. J. Xiang , X. G. Gong

Hybrid halide perovskites (HHPs) have attracted significant attention due to their remarkable optoelectronic properties that combine the advantages of low cost-effective fabrication methods of organic-inorganic materials. Notably,…

Hybrid organic-inorganic halide perovskites for photovoltaics have attracted research interest due to their unique material properties, but suffered from poor material stability. In this work, we investigated the surface phase diagrams of…

应用物理 · 物理学 2021-09-30 Yun-Sim Kim , Chol-Hyok Ri , Yun-Hyok Kye , Un-Gi Jong , Chol-Jun Yu

We investigate the structural, electronic and optical properties of mixed bromide-iodide lead perovskite solar cell CH$_3$NH$_3$Pb(I$_{1-x}$Br$_x$)$_3$ by means of the virtual crystal approximation (VCA) within density functional theory…

材料科学 · 物理学 2017-09-22 Un-Gi Jong , Chol-Jun Yu , Nam-Hyok Kim , Guk-Chol Ri

We investigate numerically the impact of the electron-phonon scattering on the optical properties of a perovskite material (CH3NH3PbI3). Using non-equilibrium Green functions formalism, we calculate the local density-of-states for several…

Metal halide perovskites exhibit a fairly linear increase of the bandgap with increasing temperature, when crystallized in a tetragonal or cubic phase. In general, both thermal expansion and electron-phonon interaction effects contribute…

We demonstrate experimentally and theoretically that two-dimensional (2D) heavy hole systems in single heterostructures exhibit a \emph{decrease} in spin-orbit interaction-induced spin splitting with an increase in perpendicular electric…

介观与纳米尺度物理 · 物理学 2009-11-10 B. Habib , E. Tutuc , S. Melinte , M. Shayegan , D. Wasserman , S. A. Lyon , R. Winkler

Spin splitting, or removal of spin degeneracy in the electronic energy band/level is often a measure of spin-orbit coupling strength and a way to manipulate spin degrees of freedom. We use first-principles simulations to predict giant spin…

材料科学 · 物理学 2024-03-18 Nikhilesh Maity , Ravi Kashikar , S. Lisenkov , I. Ponomareva

The effects of combined external electric and magnetic fields on elastic collisions in ultracold Li--Rb mixtures is studied using recently obtained, experimentally verified potentials. Our analysis provides both quantitative predictions for…

其他凝聚态物理 · 物理学 2009-09-14 Zhiying Li , Kirk W. Madison