相关论文: Exploiting vibrational strong coupling to make an …
Time-resolved Raman spectroscopy techniques offer various ways to study the dynamics of molecular vibrations in liquids or gases and optical phonons in crystals. While these techniques give access to the coherence time of the vibrational…
With the purpose to devise a novel lasing scheme, we consider a two level system with both a transversal and longitudinal coupling to the electromagnetic field. If the longitudinal coupling is sufficiently strong, multi-photon transitions…
A theoretical model of resonant hyper-Raman scattering by an ensemble of spherical semiconductor quantum dots has been developed. The electronic intermediate states are described as Wannier-Mott excitons in the framework of the envelope…
In this study, we apply the monitoring master equation describing decoherence of internal states to an optically active molecule prepared in a coherent superposition of nondegenerate internal states interacting with thermal photons at low…
We present a Hamiltonian model describing two pairs of mechanical and optical modes under standard optomechanical interaction. The vibrational modes are mechanically isolated from each other and the optical modes couple evanescently. We…
We investigate how proximity to a metal nanostructure, particularly to a flat mirror or a cavity confined between two mirrors, affects the vibronic structure of Raman scattering signals. We find that such proximity, particularly for the…
Cavity electro-(opto-)mechanics allows us to access not only single isolated but also multiple mechanical modes in a massive object. Here we develop a multi-mode electromechanical system in which a several membrane vibrational modes are…
A strongly confined light field necessarily exhibits a local polarization that varies on a subwavelength scale. We demonstrate that a single optical mode of such kind can be used to selectively and simultaneously manipulate atomic ensembles…
Sympathetic cooling with ultracold atoms and atomic ions enables ultralow temperatures in systems where direct laser or evaporative cooling is not possible. It has so far been limited to the cooling of other microscopic particles, with…
Raman-based technologies have enabled many ground-breaking scientific discoveries related to surface science, single molecule chemistry and biology. For example, researchers have identified surface bound molecules by their Raman vibrational…
Interaction between light and molecular vibrations leads to hybrid light-matter states called vibrational polaritons. Even though many intriguing phenomena have been predicted for single-molecule vibrational strong coupling (VSC), several…
Metal-Insulator-Metal (MIM) plasmonic structures can confine electromagnetic waves to a deep subwavelength regime, enabling strong light-matter interactions with potential applications in nonlinear optics and on-chip photonic circuitry. In…
Networks of optical oscillators simulating coupled Ising spins have been recently proposed as a heuristic platform to solve hard optimization problems. These networks, called coherent Ising machines (CIMs), exploit the fact that the…
We report new inelastic Raman and neutron scattering spectra for glasses with different degrees of fragility; the data are compared for each sample to obtain the Raman coupling function $C(\omega)$. The study indicates a general linear…
We have employed the method of spectral moments to study the density of vibrational states and the Raman coupling coefficient of large 2- and 3- dimensional percolators at threshold and at higher concentration. We first discuss the over-and…
Optical half-wave microresonators enable to control the optical mode density around a quantum system and thus to modify the temporal emission properties. If the coupling rate exceeds the damping rate, strong coupling between a…
Raman scattering is the inelastic process where photons bounce off molecules, losing energy and becoming red-shifted. This weak effect is unique to each molecular species, making it an essential tool in e.g. spectroscopy and label-free…
A coherent coupler is proposed to spin a Bose-Einstein condensate composed of ultracold alkali atoms into a vortex state (VS). The proposal is based on a Raman transition induced by two copropagating $\sigma^+$ and $\sigma^-$ polarized…
The integration of neutral atoms with nanophotonic structures offer significant potential as a versatile platform to explore fundamental light-matter interactions as well as realizing novel quantum-optical devices. Here, we investigate the…
Surface-Enhanced Raman Scattering (SERS) allows for detection and identification of molecular vibrational fingerprints in minute sample quantities. The SERS process can be also exploited for optical manipulation of molecular vibrations. We…