相关论文: Exploiting vibrational strong coupling to make an …
Plasmonic molecular nanojunctions exhibit opto-mechanical coupling at the nanoscale, enabling intertwined optical, vibrational and electronic phenomena. Here, we demonstrate plasmon-mediated phonon pumping, driven by inelastic electron…
We present an X-ray based stimulated Raman approach to control the preparation of optically dark electronic states in generic molecular systems. Leveraging on the unique properties of core-level excited states, we demonstrate that optically…
Degenerate optomechanical parametric oscillators are optical resonators in which a mechanical degree of freedom is coupled to a cavity mode that is nonlinearly amplified via parametric down-conversion of an external pumping laser. Below a…
Raman-type laser excitation of a trapped atom allows one to realize the quantum mechanical counterpart of phenomena of nonlinear optics, such as Kerr-type nonlinearities, parametric amplification, and multi-mode mixing. Additionally, huge…
The transversely confined propagating light modes of a nano-photonic optical waveguide or nanofiber can mediate effectively infinite-range forces. We show that for a linear chain of particles trapped within the waveguide's evanescent field,…
A complex quantum system can be constructed by coupling simple quantum elements to one another. For example, trapped-ion or superconducting quantum bits may be coupled by Coulomb interactions, mediated by the exchange of virtual photons.…
We consider a hybrid plasmon-exciton system comprised of a resonant molecular subsystem and three Au wires supporting a dipole mode which can be coupled to a dark mode in controllable fashion by variation of a symmetry parameter. The…
Photonic resonances are a powerful tool for controlling light-matter interactions. However, unlocking many of the most scientifically intriguing and technologically promising phenomena requires entering the strong coupling regime, where…
We present a scheme for generating a synthetic magnetic field and spin-orbit coupling via Raman coupling in highly magnetic lanthanide atoms such as dysprosium. Employing these atoms offer several advantages for realizing strongly…
We consider an optical and mechanical mode interacting through both linear and quadratic dispersive couplings in a general cavity-optomechanical set-up. The parity and strength of an intrinsic quadratic optomechanical coupling (QOC)…
Photonic resonance modes can be spectrally coupled to the vibrational modes of molecules in the mid-infrared regime through interactions between localized electric fields and nearby molecules. According to recent studies, radiative loss…
We introduce a scheme for creating continuous variable entanglement between an atomic beam and an optical field, by using squeezed light to outcouple atoms from a BEC via a Raman transition. We model the full multimode dynamics of the atom…
In a recent experiment (N. Wagner et al., PNAS v103, p13279) on SF$_{6}$, a high-harmonic generating laser pulse is preceded by a pump pulse which stimulates Raman-active modes in the molecule. Varying the time delay between the two pulses…
We derive the transition rates, dephasing rates, and Lamb shifts for a system consisting of many molecules collectively coupled to a resonant cavity mode. Using a variational polaron master equation, we show that strong vibrational…
We report observations of novel dynamic behavior in resonantly-enhanced stimulated Raman scattering in Rb vapor. In particular, we demonstrate a dynamic hysteresis of the Raman scattered optical field in response to changes of the drive…
Polaritons are compositional light-matter quasiparticles that arise as a result of strong coupling between a vacuum field of a resonant optical cavity and electronic excitations in quantum emitters. Reaching such a regime is often hard, as…
We observe effects of collective atomic motion in a one-dimensional optical lattice coupled to an optomechanical system. In this hybrid atom-optomechanical system, the lattice light generates a coupling between the lattice atoms as well as…
Optical oscillators present a powerful optimization mechanism. The inherent competition for the gain resources between possible modes of oscillation entails the prevalence of the most efficient single mode. We harness this 'ultrafast'…
We study the means to prepare and coherently manipulate atomic wave packets in optical lattices, with particular emphasis on alkali atoms in the far-detuned limit. We derive a general, basis independent expression for the lattice operator,…
A tapered optical nanofiber simultaneously used to trap and optically interface of cold atoms through evanescent fields constitutes a new and well controllable hybrid quantum system. The atoms are trapped in two parallel 1D optical lattices…