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Introducing hierarchical disorder from multiple defects into materials through nanostructuring is one of the most promising directions to achieve extremely low thermal conductivities and thus improve thermoelectric performance. The success…

材料科学 · 物理学 2019-09-16 Laura de Sousa Oliveira , Vassilios Vargiamidis , Neophytos Neophytou

Engineering of phonons, i.e., collective lattice vibrations in crystals, is essential for manipulating physical properties of materials such as thermal transport, electron-phonon interaction, confinement of lattice vibration, and optical…

材料科学 · 物理学 2022-02-04 Seung Gyo Jeong , Ambrose Seo , Woo Seok Choi

To elucidate the relationship between a crystal's structure, its thermal conductivity, and its phonon dispersion characteristics, an analysis is conducted on layered diatomic Lennard-Jones crystals with various mass ratios. Lattice dynamics…

材料科学 · 物理学 2007-05-23 A. J. H. McGaughey , M. I. Hussein , E. S. Landry , M. Kaviany , G. M. Hulbert

The thermal conductivity of monolayer graphene is an outstanding challenge with no consensus reached on its exact value and length convergence so far. We consider four-phonon scattering, phonon renormalization, and an exact solution to…

介观与纳米尺度物理 · 物理学 2023-10-02 Zherui Han , Xiulin Ruan

Antiferroelectrics have received blooming interests because of a wide range of potential applications in energy storage, solid-state cooling, thermal switch, transducer, actuation, and memory devices. Many of those applications are the most…

材料科学 · 物理学 2023-12-29 Yangyang Si , Tianfu Zhang , Chenhan Liu , Sujit Das , Bin Xu , Roman G Burkovsky , Xian-Kui Wei , Zuhuang Chen

We study the effect of the electron-phonon interaction on the finite frequency dependent electronic thermal conductivity of two dimensional graphene. We calculate it for various acoustic phonons present in graphene and characterized by…

强关联电子 · 物理学 2017-04-07 Pankaj Bhalla

Understanding thermal and electrical transport in topological materials is essential for advancing their applications in quantum technologies and energy conversion. Herein, we employ first-principles calculations to systematically…

IV-VI materials are some of the most efficient bulk thermoelectric materials due to their proximity to soft-mode phase transitions, which leads to low lattice thermal conductivity. It has been shown that the lattice thermal conductivity of…

材料科学 · 物理学 2021-07-21 Jiang Cao , Đorđe Dangić , José D. Querales-Flores , Stephen Fahy , Ivana Savić

Recently, three-component new fermions in topological semimetal MoP are experimentally observed, which may have potential applications like topological qubits, low-power electronics and spintronics. These are closely related to thermal…

材料科学 · 物理学 2017-07-04 San-Dong Guo

Low-dimensional electronic and glassy phononic transport are two important ingredients of highly-efficient thermoelectric material, from which two branches of the thermoelectric research emerge. One focuses on controlling electronic…

材料科学 · 物理学 2015-07-14 Xue-Ya Mi , Xiaoxiang Yu , Kai-Lun Yao , Xiaoming Huang , Nuo Yang , Jing-Tao Lü

Since solid-state heat transport in a highly porous nanocomposite strongly depends on the thermal boundary conductance (TBC) between constituent nanomaterials, further suppression of the TBC is important for improving performance of thermal…

In the pursuit of advanced ceramic materials with exceptional irradiation-resistance and high-temperature tolerance for nuclear applications, compositionally complex carbides (CCCs) have emerged as a highly promising class of candidate…

While using first-principles-based Boltzmann transport equation approach to predict the thermal conductivity of crystalline semiconductor materials has been a routine, the validity of the approach is seldom tested for high-temperature…

介观与纳米尺度物理 · 物理学 2020-03-05 Xiaokun Gu , Shouhang Li , Hua Bao

An increasing number of theoretical calculations on few-layer materials have been reporting a non-zero sound velocity for all three acoustic phonon modes. In contrast with these reports, here we show that the lowest phonon dispersion branch…

材料科学 · 物理学 2017-02-06 Jesús Carrete , Wu Li , Lucas Lindsay , David A. Broido , Luis J. Gallego , Natalio Mingo

Understanding heat transport in semiconductors and insulators is of fundamental importance because of its technological impact in electronics and renewable energy harvesting and conversion. Anharmonic Lattice Dynamics provides a powerful…

材料科学 · 物理学 2020-10-13 Giuseppe Barbalinardo , Zekun Chen , Nicholas W. Lundgren , Davide Donadio

Elemental antimony (Sb) is a promising material for phase-change memory, neuromorphic computing and nanophotonic applications, because its compositional simplicity can prevent phase segregation upon extensive programming. Scaling down the…

We study thermal transport in folded graphene nanoribbons using molecular dynamics simulations and the non-equilibrium Green's function method. It is found that the thermal conductivity of flat graphene nanoribbons can be modulated by…

介观与纳米尺度物理 · 物理学 2015-06-05 Nuo Yang , Xiaoxi Ni , Jin-Wu Jiang , Baowen Li

Thermal boundary conductance at a metal-dieletric interface is a quantity of prime importance for heat management at the nanoscale. While the boundary conductance is usually ascribed to the coupling between metal phonons and dielectric…

介观与纳米尺度物理 · 物理学 2015-06-23 J. Lombard , F. Detcheverry , S. Merabia

We systematically demonstrate the temperature-dependent thermal transport properties in crystalline Ge$_2$Sb$_2$Te$_5$via first-principles density functional theory-informed linearized Boltzmann transport equation. The investigation,…

材料科学 · 物理学 2023-12-18 Kanka Ghosh , Andrzej Kusiak , Jean-Luc Battaglia

The structural stability of thermoelectric materials is a subject of growing importance for their energy harvesting applications. Here, we study the microscopic mechanisms governing the structural stability change of zinc antimony at its…

材料科学 · 物理学 2016-11-04 Xiaolong Yang , Jianping Lin , Guanjun Qiao , Zhao Wang