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Tailoring thermal properties with nanostructured materials can be of vital importance for many applications. Generally classical phonon size effects are employed to reduce the thermal conductivity, where strong phonon scattering by…

应用物理 · 物理学 2019-10-14 Yue Xiao , Qiyu Chen , Dengke Ma , Nuo Yang , Qing Hao

The lattice thermal conductivity ($\kappa$) of two ceramic materials, cerium dioxide (CeO$_2$) and magnesium oxide (MgO), is computed up to 1500 K using first principles and the phonon Boltzmann Transport Equation (PBTE) and compared to…

Metallic transition-metal nitrides (TMNs) are promising conductive ceramics for many applications, whose thermal transport is of great importance in device design. It is found metallic TiN and HfN hold anomalous thermal transport behaviors…

材料科学 · 物理学 2020-06-30 Shouhang Li , Ao Wang , Yue Hu , Xiaokun Gu , Zhen Tong , Hua Bao

Periodic hole array phononic crystals (PnC) can strongly modify the phonon dispersion relations, and have been shown to influence thermal conductance coherently, especially at low temperatures where scattering is suppressed. One very…

介观与纳米尺度物理 · 物理学 2019-07-10 Yaolan Tian , Tuomas A. Puurtinen , Zhuoran Geng , Ilari J. Maasilta

Aluminum nitride (AlN) plays a key role in modern power electronics and deep-ultraviolet photonics, where an understanding of its thermal properties is essential. Here we measure the thermal conductivity of crystalline AlN by the…

Acoustic phonons play a special role in lattice heat transport, and confining these low-energy modes in low-dimensional materials may enable nontrivial transport phenomena. By applying lowest-order anharmonic perturbation theory to an…

介观与纳米尺度物理 · 物理学 2021-09-01 Daniel Bruns , Alireza Nojeh , A. Srikantha Phani , Jörg Rottler

Interest in high entropy alloy thermoelectric materials is predicated on achieving ultralow lattice thermal conductivity $\kappa\sub{L}$ through large compositional disorder. However, here we show that for a given mechanism, such as mass…

Excitations and scatterings among the quantized lattice vibrations, i.e., phonons, govern the lattice thermal conductivity ($\kappa_l$) in crystalline solids. Therefore, effective modulation of $\kappa_l$ can be achieved through selective…

材料科学 · 物理学 2025-07-09 Jyoti Duhan , Chris Wolverton , Koushik Pal

We present an \emph{ab initio} study of the role of interference effects in the thermal conductance of single-molecule junctions. To be precise, using a first-principles transport method based on density functional theory, we analyze the…

介观与纳米尺度物理 · 物理学 2017-12-27 J. C. Klöckner , J. C. Cuevas , F. Pauly

The lattice vibrations (phonon modes) of crystals underpin a large number of material properties. The harmonic phonon spectrum of a solid is the simplest description of its structural dynamics and can be straightforwardly derived from the…

材料科学 · 物理学 2022-03-03 Ioanna Pallikara , Prakriti Kayastha , Jonathan M. Skelton , Lucy D. Whalley

Metal mixed polymers are a cheap and effective way to produce flexible metals and superconductors. As part of an on-going effort to learn how to tune the properties of these systems with ion implantation, we present a study of the…

材料科学 · 物理学 2009-06-15 Andrew P. Stephenson , Ujjual Divakar , Adam P. Micolich , Paul Meredith , Ben J. Powell

A fundamental understanding of the phonon transport mechanism is important for optimizing the efficiency of thermoelectric devices. In this study, we investigate the thermal transport properties of the oxidized form of phosphorene called…

材料科学 · 物理学 2019-05-21 Seungjun Lee , Seoung-Hun Kang , Young-Kyun Kwon

The electrical resistivity, thermoelectric power and electronic thermal conductivity of simple (isotropic) metals are studied in a uniform way. Starting from results of a variational solution of the Boltzmann equation, a generalized…

材料科学 · 物理学 2009-11-07 M. Ausloos , K. Durczewski , J. Ulner

The lattice thermal conductivity of graphene is evaluated using a microscopic model that takes into account the lattice's discrete nature and the phonon dispersion relation within the Brillouin zone. The Boltzmann transport equation is…

软凝聚态物质 · 物理学 2024-01-18 J. Chen , Y. Liu

We report the first investigation of the photo-response of the conductivity of a new class of organic semiconductors based on functionalized pentacene. These materials form high quality single crystals that exhibit a thermally activated…

材料科学 · 物理学 2009-11-07 T. Tokumoto , J. S. Brooks , R. Clinite , X. Wei , J. E. Anthony , D. L. Eaton , S. R. Parkin

Energy transfer to acoustic phonons is the dominant low-temperature cooling channel of electrons in a crystal.For cold neutral graphene we find that the weak cooling power of its acoustical modes relative to the heat capacity of the system…

介观与纳米尺度物理 · 物理学 2013-05-29 R. Bistritzer , A. H. MacDonald

In this work, we present a comprehensive investigation of graphene's thermal conductivity using first-principles density functional perturbation theory calculations, with a focus on the phonon and lattice vibrational properties underlying…

材料科学 · 物理学 2024-12-25 Archishman Gupta , Ankit Arora

Two-dimensional (2-D) transition metal dichalcogenides (TMDs) have shown numerous interesting physical and chemical properties, making them promising materials for electronic, optoelectronic, and energy applications. Tuning thermal…

材料科学 · 物理学 2016-09-07 Xiaokun Gu , Ronggui Yang

Porous materials provide a large surface to volume ratio, thereby providing a knob to alter fundamental properties in unprecedented ways. In thermal transport, porous nanomaterials can reduce thermal conductivity by not only enhancing…

Topological semimetal may have potential applications like topological qubits, spintronics and quantum computations. Efficient heat dissipation is a key factor for the reliability and stability of topological semimetal-based…

材料科学 · 物理学 2018-03-14 San-Dong Guo , Bang-Gui Liu