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Drug-loaded hydrogels provide a means to deliver pharmaceutical agents to specific sites within the body at a controlled rate. The aim of this paper is to understand how controlled drug release can be achieved by tuning the initial…

最优化与控制 · 数学 2022-02-07 Matthew J. Penn , Matthew G. Hennessy

We investigate the dynamics of alginate gels, an important class of biopolymer-based viscoelastic materials, by combining mechanical tests and non-conventional, time-resolved light scattering methods. Two relaxation modes are observed upon…

软凝聚态物质 · 物理学 2013-10-14 Domenico Larobina , Luca Cipelletti

Molecular dynamics simulations are a powerful tool to study diffusion processes in battery electrolyte and electrode materials. From a single molecular dynamics simulation many properties relevant to diffusion can be obtained, including the…

化学物理 · 物理学 2018-07-09 Niek J. J. de Klerk , Eveline van der Maas , Marnix Wagemaker

Hydrogels are crosslinked polymer networks with high water content, widely employed in biomedical applications such as drug delivery, tissue engineering, and regenerative medicine. Injectable, depot-forming hydrogels enable sustained…

We analyse the dynamics of different routes to collapse of a constrained polyelectrolyte gel in contact with an ionic bath. The evolution of the gel is described by a model that incorporates non-linear elasticity, Stefan-Maxwell diffusion…

软凝聚态物质 · 物理学 2025-01-22 Giulia L. Celora , Matthew G. Hennessy , Andreas Münch , Barbara Wagner , Sarah L. Waters

Biological systems achieve adaptive mechanical responses through reaction-diffusion processes that couple chemical wave propagation to structural transitions. Although synthetic hydrogels with enzymatic reactions offer a platform for…

软凝聚态物质 · 物理学 2026-03-31 Natascha Gray , Zoe Grämiger , André R. Studart , Rafael Libanori

Curable hydrogels have tunable properties that make them well-suited for applications in drug delivery, cell therapies, and 3D bioprinting. Advances in microfluidic droplet generation enable rapid fabrication of polymer-filled droplets.…

流体动力学 · 物理学 2025-12-02 Sabrina Marnoto , Avi J. Patel , Sara M. Hashmi

A recent study has demonstrated that phase separation in binary liquid mixtures is arrested in the presence of elastic networks and can lead to a nearly uniformly-sized distribution of the dilute-phase droplets. At longer timescales, these…

软凝聚态物质 · 物理学 2020-10-28 Mrityunjay Kothari , Tal Cohen

Hyaluronic acid is an abundant polyelectrolyte in the human body that forms extracellular hydrogels in connective tissues. It is essential for regulating tissue biomechanics and cell-cell communication, yet hyaluronan overexpression is…

Piezoionic hydrogels offer a route to mechanically driven bioelectronic interfaces, but their output is limited by rapid, symmetric ion redistribution that dissipates charge gradients. In biological electrocytes, efficient signal generation…

介观与纳米尺度物理 · 物理学 2026-05-01 Tofayel Ahammad Ovee , Daniel Kroeger , Jean-François Louf

It is of great importance to develop inorganic solid electrolytes with high ionic conductivity, thus enabling solid state Li-ion batteries to address the notorious safety issue about the current technology due to use of highly flammable…

化学物理 · 物理学 2017-07-17 Zhuo Wang , Min Jie Xuan , Hong Jie Xu , Guosheng Shao

This paper examines the response of electrolyte-saturated polymer gels, embedded with charged spherical inclusions, to a weak gradient of electrolyte concentration. These composites present a model system to study microscale electrokinetic…

软凝聚态物质 · 物理学 2009-11-11 Reghan J. Hill

Thermoresponsive hydrogels have been studied intensively for creating smart drug carriers and controlled drug delivery. Understanding the drug release kinetics and corresponding transport mechanisms of nanoparticles (NPs) in a…

软凝聚态物质 · 物理学 2020-05-12 Yi Wang , Zhen Li , Jie Ouyang , George Em Karniadakis

Local drug delivery has received much recognition in recent years, yet it is still unpredictable how drug efficacy depends on physicochemical properties and delivery kinetics. The purpose of the current study is to provide a useful…

动力系统 · 数学 2016-01-26 Koyel Chakravarty , D C Dalal

The swelling kinetics of charged polymer gels reflect the complex competition among elastic, mixing, and ionic contributions. Here, we used dynamic light scattering to investigate the collective diffusion coefficient of model gels, whose…

软凝聚态物质 · 物理学 2024-02-01 Shoei Sano , Takashi Yasuda , Takeshi Fujiyabu , Naoyuki Sakumichi , Takamasa Sakai

Soft pair potentials predict a reentrant liquid phase for high concentrations, a behavior not observed experimentally. Here, very soft microgels confined at an oil-water interface are used as a model system of particles interacting via a…

Ion-conducting glasses and polymer systems show several characteristic peculiarities in their composition-dependent diffusion properties and in their dynamic response. First we give a brief review of the current understanding of the ion…

凝聚态物理 · 物理学 2016-08-31 O. Durr , P. Pendzig , W. Dieterich , A. Nitzan

Intracrystalline diffusion is an invaluable tool for estimating timescales of geological events. Diffusion is typically modeled using gradients in chemical potential. However, chemical potential is derived for uniform pressure and…

材料科学 · 物理学 2023-06-22 Benjamin L. Hess , Jay J. Ague

We investigate diffusion of a peptide drug through Graphene Oxide (GO) membranes that are modeled as a porous layered laminate constructed from aligned flakes of GO. Our experiments using a peptide drug show a tunable non-linear dependence…

材料科学 · 物理学 2015-12-29 T. M. Puvirajesinghe , Z. L. Zhi , R. V. Craster , S. Guenneau

The oxygen-exchange behavior has been studied in half-doped manganese and cobalt perovskite oxides. We have found that the oxygen diffusivity in Gd_{0.5}Ba_{0.5}MnO_{3-\delta} can be enhanced by orders of magnitude by inducing…

材料科学 · 物理学 2007-05-23 A. A. Taskin , A. N. Lavrov , Yoichi Ando
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