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We present a rapid-scan, time-domain terahertz spectrometer employing femtosecond Er:fiber technology and an acousto-optic delay with attosecond precision, enabling scanning of terahertz transients over a 12.4 ps time window at a waveform…

光学 · 物理学 2016-04-14 B. Urbanek , M. Möller , M. Eisele , S. Baierl , D. Kaplan , C. Lange , R. Huber

Electrical pulse stimulation drives many important physical phenomena in condensed matter as well as in electronic systems and devices. Often, nanoscopic and mesoscopic mechanisms are hypothesized, but methods to image electrically driven…

介观与纳米尺度物理 · 物理学 2023-06-05 Thomas E Gage , Daniel B Durham , Haihua Liu , Supratik Guha , Ilke Arslan , Charudatta Phatak

Linear terahertz time-domain spectroscopy (THz-TDS) is a sensitive probe for material characterization including thickness measurements of thin layers. These applications critically rely on a sufficiently large bandwidth, which is not…

We probe the electron transport properties in the shell of GaAs/In0.2Ga0.8As core/shell nanowires at high electric fields using optical pump / THz probe spectroscopy with broadband THz pulses and peak electric fields up to 0.6 MV/cm. The…

介观与纳米尺度物理 · 物理学 2020-06-24 Rakesh Rana , Leila Balaghi , Ivan Fotev , Harald Schneider , Manfred Helm , Emmanouil Dimakis , Alexej Pashkin

Terahertz spectrometers with a wide instantaneous frequency coverage for passive remote sensing are enormously attractive for many terahertz applications, such as astronomy, atmospheric science and security. Here we demonstrate a wide-band…

Terahertz (THz)-based electron manipulation has recently been shown to hold tremendous promise as a technology for manipulating and driving the next-generation of compact ultrafast electron sources. Here, we demonstrate an ultrafast…

We use ultrafast x-ray pulses to characterize the lattice response of SrTiO3 when driven by strong terahertz (THz) fields. We observe transient changes in the diffraction intensity with a delayed onset with respect to the driving field.…

材料科学 · 物理学 2017-03-30 M. Kozina , T. van Driel , M. Chollet , T. Sato , J. M. Glownia , S. Wandel , M. Radovic , U. Staub , M. C. Hoffmann

Strong-field mid-infrared pump--terahertz (THz) probe spectroscopy has been proven as a powerful tool for light control of different orders in strongly correlated materials. We report the construction of an ultrafast broadband infrared…

仪器与探测器 · 物理学 2017-10-10 S. J. Zhang , Z. X. Wang , T. Dong , N. L. Wang

We present results of wavelength-dependent ultrafast pump-probe experiments on micelle-suspended single-walled carbon nanotubes. The linear absorption and photoluminescence spectra of the samples show a number of chirality-dependent peaks,…

介观与纳米尺度物理 · 物理学 2009-11-10 J. Kono , G. N. Ostojic , S. Zaric , M. S. Strano , V. C. Moore , J. Shaver , R. H. Hauge , R. E. Smalley

Single-shot terahertz (THz) spectroscopy probes sub-picosecond, non-repetitive events by combining the advantages of laser absorption techniques with the phase-sensitive detection of interferometric methods. However, its usage as a…

光学 · 物理学 2025-01-07 Charan R. Nallapareddy , Thomas C. Underwood

Resolving sub-10 nm spin switching and the associated terahertz (THz) electrodynamics during the colossal magnetoresistance (CMR) transition is a definitive frontier in reaching the fundamental spatial, temporal, and energy-dissipation…

Development of ultrafast lasers and non-linear optical techniques over the last two decades provides tools to access real-time dynamics of low energy excitations in superconductors. For example, time-resolved THz spectroscopy and time- and…

超导电性 · 物理学 2022-04-20 Jure Demsar

Atomically-thin molybdenum disulfide is emerging as a new nanomaterial with potential applications in the fields of electronic and photonics. Charge carrier dynamics plays an essential role in determining its electronic and optical…

介观与纳米尺度物理 · 物理学 2012-07-09 Rui Wang , Brian A. Ruzicka , Nardeep Kumar , Matthew Z. Bellus , Hsin-Ying Chiu , Hui Zhao

Ultrafast optical imaging has enabled direct observation of femtosecond-nanosecond dynamics, yet three-dimensional (3D) dynamic measurements at high numerical aperture (NA) remain hindered by the intrinsically shallow depth of field (DoF)…

We study the nature of photo-excited charge carriers in CsPbBr3 nanocrystal thin films by ultrafast optical pump - THz probe spectroscopy. We observe a deviation from a pure Drude dispersion of the THz dielectric response that is ascribed…

Terahertz and sub-terahertz band detection has a key role both in fundamental interactions physics and technological applications, such as medical imaging, industrial quality control and homeland security. In particular, transition edge…

We employ optical pump-THz probe spectroscopy to chart the ultrafast superconductivity suppression in NbN over a broad range of excitation fluences. Our measurements uncover a pronounced lengthening of the superconductivity quenching time…

Clarifying electronic and vibronic properties at individual molecule level provides key insights to future chemistry, nanoelectronics, and quantum information technologies. The single electron tunneling spectroscopy has been used to study…

介观与纳米尺度物理 · 物理学 2018-09-05 Shaoqing Du , Kenji Yoshida , Ya Zhang , Ikutaro Hamada , Kazuhiko Hirakawa

Real-time time-dependent density functional theory, in conjunction with the Ehrenfest molecular dynamics scheme, is becoming a popular methodology to investigate ultrafast phenomena on the nanoscale. Thanks to recent developments, it is…

材料科学 · 物理学 2020-08-18 Jannis Krumland , Ana M. Valencia , Stefano Pittalis , Carlo A. Rozzi , Caterina Cocchi

Ultrafast electron microscopy aims for imaging transient phenomena occurring on nanoscale. One of its goals is to visualize localized optical and plasmonic modes generated by coherent excitation in the vicinity of various types of…