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相关论文: A new high pressure form of Ba3NiSb2O9

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By using a high pressure, high temperature (HPHT) technique, the antiferromagnetically ordered ($T_N$ = 13.5 K) 6H-A phase of Ba$_3$NiSb$_2$O$_9$ was transformed into two new gapless quantum spin liquid(QSL) candidates with S=1 (Ni$^{2+}$)…

强关联电子 · 物理学 2011-11-08 J. G. Cheng , G. Li , L. Balicas , J. S. Zhou , J. B. Goodenough , Cenke Xu , H. D. Zhou

Inelastic neutron scattering is used to study the low-energy magnetic excitations in the spin-1 triangular lattice of the 6H-B phase of Ba$_3$NiSb$_2$O$_9$. We study two powder samples: Ba$_3$NiSb$_2$O$_9$ synthesized under high pressure…

强关联电子 · 物理学 2017-02-08 B. Fak , S. Bieri , E. Canevet , L. Messio , C. Payen , M. Viaud , C. Guillot-Deudon , C. Darie , J. Ollivier , P. Mendels

The quantum spin liquid (QSL) is an exotic phase of magnetic materials where the spins continue to fluctuate without any symmetry breaking down to zero temperature. Among the handful reports of QSL with spin $S\ge$1, examples with magnetic…

We report the structural and magnetic properties of the 4}\textit{\textcolor{black}{d }}\textcolor{black}{(M = Rh) based and 5}\textit{\textcolor{black}{d }}\textcolor{black}{(M = Ir) based systems Ba$_{3}$M$_{x}$Ti$_{3-x}$O$_{9}$…

Recently, a number of experiments indicate the possible presence of spin liquid phases in quantum magnets with spin-1/2 and spin-1 moments sitting on triangular-lattice-based structures in Ba3CuSb2O9 and Ba3NiSb2O9 respectively. In relation…

强关联电子 · 物理学 2013-06-04 Kyusung Hwang , Tyler Dodds , Subhro Bhattacharjee , Yong Baek Kim

We report the structural transformation of hexagonal Ba3YIr2O9 to a cubic double perovskite form (stable in ambient conditions) under an applied pressure of 8GPa at 1273K. While the ambient pressure (AP) synthesized sample undergoes…

强关联电子 · 物理学 2013-10-28 Tusharkanti Dey , A. V. Mahajan , R. Kumar , B. Koteswararao , F. C. Chou , A. A. Omrani , H. M. Ronnow

Ba3IrTi2O9 crystallizes in a hexagonal structure consisting of a layered triangular arrangement of Ir4+ (Jeff=1/2). Magnetic susceptibility and heat capacity data show no magnetic ordering down to 0.35K inspite of a strong magnetic coupling…

强关联电子 · 物理学 2012-10-29 Tusharkanti Dey , A. V. Mahajan , P. Khuntia , M. Baenitz , B. Koteswararao , F. C. Chou

We study the ground state and spin excitations in Ba3MnSb2O9, an easy-plane S = 5/2 triangular lattice antiferromagnet. By combining single-crystal neutron scattering, electric spin resonance (ESR), and spin wave calculations, we determine…

The search for Kitaev's quantum spin liquid (KQSL) state in real materials has recently expanded with the prediction that honeycomb lattices of divalent, high-spin cobalt ions could host the dominant bond-dependent exchange interactions…

We report the synthesis and characterization of a new quantum magnet [2-[Bis(2-hydroxybenzyl)aminomethyl]pyridine]Ni(II)-trimer (BHAP-Ni3) in single-crystalline form. Our combined experimental and theoretical investigations reveal an exotic…

Motivated by recent experiments on material Ba3NiSb2O9, we propose two novel spin liquid phases (A and B) for spin-1 systems on a triangular lattice. At the mean field level, both spin liquid phases have gapless fermionic spinon excitations…

强关联电子 · 物理学 2013-05-30 Cenke Xu , Fa Wang , Yang Qi , Leon Balents , Matthew P. A. Fisher

A previously unreported layered spin 1/2 triangular lattice polymorph of TiI3 is described, synthesized under 6 GPa of applied pressure at 900 C, but stable at atmospheric pressure. This air-sensitive material has a CdI2-type layered…

The rare-earth-based geometrically frustrated triangular magnets have attracted considerable attention due to the intricate interplay between strong spin-orbit coupling and the crystal electric field (CEF), which often leads to effective…

The magnetic phases of the ideal spin-1/2 triangular-lattice antiferromagnet Ba$_3$CoSb$_2$O$_9$ are identified and studied using $^{135,137}$Ba nuclear magnetic resonance (NMR) spectroscopy in magnetic fields ranging to 30T, oriented…

强关联电子 · 物理学 2015-01-13 G. Koutroulakis , T. Zhou , C. D. Batista , Y. Kamiya , J. D. Thompson , S. E. Brown , H. D. Zhou

Strongly correlated ground states and exotic quasiparticle excitations in low-dimensional systems are central research topics in the solid state research community. The present work develops a new layered material and explores the physical…

强关联电子 · 物理学 2023-02-09 Xianghan Xu , Guangming Cheng , Danrui Ni , Xin Gui , Weiwei Xie , Nan Yao , R. J. Cava

Quantum spin liquids (QSLs) represent a novel state of matter in which quantum fluctuations prevent conventional magnetic order from being established, and the spins remain disordered even at zero temperature. There have been many…

强关联电子 · 物理学 2018-10-11 Zhen Ma , Kejing Ran , Jinghui Wang , Song Bao , Zhengwei Cai , Shichao Li , Jinsheng Wen

Ba$_8$CoNb$_6$O$_{24}$ presents a system whose Co$^{2+}$ ions have an effective spin 1/2 and construct a regular triangular-lattice antiferromagnet (TLAFM) with a very large interlayer spacing, ensuring purely two-dimensional character. We…

强关联电子 · 物理学 2018-04-17 Y. Cui , J. Dai , P. Zhou , P. S. Wang , T. R. Li , W. H. Song , J. C. Wang , L. Ma , Z. Zhang , S. Y. Li , G. M. Luke , B. Normand , T. Xiang , W. Yu

A recently discovered material, 6H-B-Ba3NiSb2O9 was found to display unusual low-temperature phenomenology, interpreted as a quantum spin liquid with spin S = 1 on a triangular lattice. We study a spin S = 1 quantum exchange model on an AB…

强关联电子 · 物理学 2012-08-27 Gang Chen , Michael Hermele , Leo Radzihovsky

We successfully synthesized and characterized the triangular lattice anitferromagnet Ba$_8$MnNb$_6$O$_{24}$, which comprises equilateral spin-5/2 Mn$^{2+}$ triangular layers separated by six non-magnetic Nb$^{5+}$ layers. The detailed…

材料科学 · 物理学 2019-06-03 R. Rawl , L. Ge , Z. Lu , Z. Evenson , C. R. Dela Cruz , Q. Huang , M. Lee , E. S. Choi , M. Mourigal , H. D. Zhou , J. Ma

Quantum spin liquids (QSL) are theoretical states of matter with long-range entanglement and exotic quasiparticles. However, they generally elude quantitative theory, rendering their underlying phases mysterious and hampering efforts to…

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