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We present a comprehensive study of the electronic, magnetic, and optical properties of CuGa$_{1-x}$Fe$_x$S$_2$, as a promising candidate for intermediate-band (IB) solar cells. We use hybrid exchange-correlation functional within the…

材料科学 · 物理学 2016-04-13 J. Koskelo , J. Hashemi , S. Huotari , M. Hakala

Hyperdoped metastable sulfur atoms endow crystalline silicon with a strong sub-bandgap light absorption. In order to explore such metastable states, we develop a new high-throughput first-principles calculation method to search for all of…

材料科学 · 物理学 2016-11-17 Ke-Fan Wang , Mingguo Liu , Yaping Ma , Zhenxiang Cheng , Yuanxu Wang , Xudong Xiao

Photocatalytic water splitting is a promising renewable energy source as an alternative for limited fossil fuels. The effectiveness of the conversion from solar energy to hydrogen fuel relies primarily on the material. Previously,…

材料科学 · 物理学 2022-01-04 Celine Wu , Xuan Luo

Topological insulators are characterized by the existence of band inversion and the possibility of the realization of surface states. Doping with a magnetic atom, which is a source of the time-reversal symmetry breaking, can lead to…

材料科学 · 物理学 2020-11-17 Andrzej Ptok , Konrad Jerzy Kapcia , Anna Ciechan

As an appealing concept for developing next-generation solar cells, intermediate-band solar cells (IBSCs) promise to drastically increase the quantum efficiency of photovoltaic conversion. Yet to date, a standing challenge lies in the lack…

材料科学 · 物理学 2012-10-10 Fengcheng Wu , Haiping Lan , Zhenyu Zhang , Ping Cui

Topological insulators are novel quantum materials with metallic surface transport, but insulating bulk behavior. Often, topological insulators are dominated by bulk contributions due to defect induced bulk carriers, making it difficult to…

We report a systematic angle-resolved photoemission spectroscopy on topological insulator (TI) TlBi1-xSbxTe2 which is bulk insulating at 0.5 < x < 0.9 and undergoes a metal-insulator-metal transition with the Sb content x. We found that…

介观与纳米尺度物理 · 物理学 2016-06-28 Chi Xuan Trang , Zhiwei Wang , Keiko Yamada , Seigo Souma , Takafumi Sato , Takashi Takahashi , Kouji Segawa , Yoichi Ando

New generation Indium based lead-free Cs2InAgCl6 is a promising halide material in photovoltaic applications due to its good air stability and non-toxic behavior. But its wide band gap (>3 eV) is not suitable for solar spectrum and hence…

The realization of bulk metallic altermagnetism has remained elusive despite the growing number of candidate materials. Here, we present evidence that moderate cobalt substitution ($\sim$15%) drives the correlated narrow-gap semiconductor…

By harvesting a wider range of the solar spectrum, intermediate band solar cells (IBSCs) can achieve efficiencies 50% higher than conventional single-junction solar cells. For this, additional requirements are imposed to the light-absorbing…

Due to high density of native defects, the prototypical topological insulator (TI), Bi$_2$Se$_3$, is naturally n-type. Although Bi$_2$Se$_3$ can be converted into p-type by substituting 2+ ions for Bi, only light elements such as Ca have…

材料科学 · 物理学 2020-02-12 Jisoo Moon , Zengle Huang , Weida Wu , Seongshik Oh

Topological insulators (TIs) are emergent materials with unique band structure, which allow the study of quantum effect in solids, as well as contribute to high performance quantum devices. To achieve the better performance of TI, here we…

Recombination through quantum dots (QDs) is a major factor that limits efficiency of QD intermediate-band (IB) solar cells. Our proposal for a new IB solar cell based on type-II GaSb QDs located outside the depletion region of a GaAs…

介观与纳米尺度物理 · 物理学 2012-10-08 A. Kechiantz , A. Afanasev , J. -L. Lazzari , A. Bhouri , Y. Cuminal , P. Christol

We observe an insulator-to-metal (I-M) transition in crystalline silicon doped with sulfur to non- equilibrium concentrations using ion implantation followed by pulsed laser melting and rapid resolidification. This I-M transition is due to…

材料科学 · 物理学 2015-05-27 Mark T. Winkler , Daniel Recht , Meng-Ju Sher , Aurore J. Said , Eric Mazur , Michael J. Aziz

We investigate the influence of an unoccupied band on the transport properties of a strongly correlated electron system. For that purpose, additional orbitals are coupled to a Hubbard model via hybridization. The filling is one electron per…

凝聚态物理 · 物理学 2009-10-28 Stefan Blawid , Hoangh Anh Tuan , Takashi Yanagisawa , Peter Fulde

In2O3 is a prototype wide-band-gap semiconductor that exhibits metallic conductivity when highly doped with Sn while retaining a high degree of transparency to visible light. It is widely used as a transparent window/electrode in solar…

材料科学 · 物理学 2019-03-27 Fernando P. Sabino , Su-Huai Wei , Anderson Janotti

Transition metal dichalcogenides (TMDs) show great promise as absorber materials in high-specific-power (i.e. high-power-per-weight) solar cells, due to their high optical absorption, desirable band gaps, and self-passivated surfaces.…

应用物理 · 物理学 2023-12-25 Koosha Nassiri Nazif , Frederick U. Nitta , Alwin Daus , Krishna C. Saraswat , Eric Pop

The intermediate band (IB) cell is a concept of highly efficient solar cells proposed by Luque and Marti in 1997. The IB concept uses nonlinear effect of two photon absorption enforced with concentration of such photons for generation of…

介观与纳米尺度物理 · 物理学 2012-09-11 A. Kechiantz , A. Afanasev , J. -L. Lazzari

The novel concept of non-compensated n-p codoping has made it possible to create tunable intermediate bands in the intrinsic band gap of TiO2, making the codoped TiO2 a promising material for developing intermediate band solar cells…

材料科学 · 物理学 2010-12-10 Tian-Li Feng , Guang-Wei Deng , Yi Xia , Feng-Cheng Wu , Ping Cui , Hai-Ping Lan , Zhen-Yu Zhang

Hyperdoping consists of the intentional introduction of deep-level dopants into a semiconductor in excess of equilibrium concentrations. This causes a broadening of dopant energy levels into an intermediate band between the valence and…

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