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We present experimental results from a new scheme for magneto-optically trapping strontium monofluoride (SrF) molecules, which provides increased confinement compared to our original work. The improved trap employs a new approach to…

原子物理 · 物理学 2015-06-23 D. J. McCarron , E. B. Norrgard , M. H. Steinecker , D. DeMille

Laser cooling and trapping are central to modern atomic physics. The workhorse technique in cold-atom physics is the magneto-optical trap (MOT), which combines laser cooling with a restoring force from radiation pressure. For a variety of…

原子物理 · 物理学 2014-10-20 J. F. Barry , D. J. McCarron , E. B. Norrgard , M. H. Steinecker , D. DeMille

We demonstrate loading of SrF molecules into an optical dipole trap (ODT) via in-trap $\Lambda$-cooling. We find that this cooling can be optimized by a proper choice of relative ODT and $\Lambda$ beam polarizations. In this optimized…

原子物理 · 物理学 2021-10-27 Thomas K. Langin , Varun Jorapur , Yuqi Zhu , Qian Wang , David DeMille

Calcium monofluoride (CaF) molecules are loaded into an optical dipole trap (ODT) and subsequently laser cooled within the trap. Starting with magneto-optical trapping, we sub-Doppler cool CaF and then load $150(30)$ CaF molecules into an…

We report a magneto-optical trap of strontium monohydroxide (SrOH) containing 2000(600) molecules at a temperature of 1.2(3) mK. The lifetime is 91(9) ms, which is limited by decay to optically unaddressed vibrational states. This provides…

There is substantial interest in producing samples of ultracold molecules for possible applications in quantum computation, quantum simulation of condensed matter systems, precision measurements, controlled chemistry, and high precision…

原子物理 · 物理学 2013-05-30 J. F. Barry , E. S. Shuman , E. B. Norrgard , D. DeMille

We report optical trapping of laser-cooled molecules at sufficient density to observe molecule-molecule collisions for the first time in a bulk gas. SrF molecules from a red-detuned magneto-optical trap (MOT) are compressed and cooled in a…

原子物理 · 物理学 2024-05-09 Varun Jorapur , Thomas K. Langin , Qian Wang , Geoffrey Zheng , David DeMille

We report an optical dipole trap of strontium monohydroxide (SrOH) with 1400(300) trapped molecules. Through optical pumping, we access vibrational states that are proposed for improved probes of the electron's electric dipole moment (eEDM)…

Magneto-optical trapping of molecules has thus far been restricted to molecules with $^2\Sigma$ electronic ground states. These species are chemically reactive and only support a simple laser cooling scheme from their first excited…

We demonstrate significantly improved magneto-optical trapping of molecules using a very slow cryogenic beam source and RF modulated and DC magnetic fields. The RF MOT confines $1.1(3) \times 10^5$ CaF molecules at a density of $4(1) \times…

It has been roughly three decades since laser cooling techniques produced ultracold atoms, leading to rapid advances in a vast array of fields. Unfortunately laser cooling has not yet been extended to molecules because of their complex…

原子物理 · 物理学 2015-05-27 E. S. Shuman , J. F. Barry , D. DeMille

Calcium monofluoride (CaF) is magnetically slowed and trapped using optical pumping. Starting from a collisionally cooled slow beam, CaF with an initial velocity of ~ 30 m/s is slowed via magnetic forces as it enters a 800 mK deep magnetic…

原子物理 · 物理学 2014-03-26 Hsin-I Lu , Ivan Kozyryev , Boerge Hemmerling , Julia Piskorski , John M. Doyle

We demonstrate a 1D magneto-optical trap of the polar free radical calcium monohydroxide (CaOH). A quasi-closed cycling transition is established to scatter $\sim 10^3$ photons per molecule, predominantly limited by interaction time. This…

We propose a method for laser cooling and trapping a substantial class of polar molecules, and in particular titanium (II) oxide (TiO). This method uses pulsed electric fields to nonadiabatically remix the ground-state magnetic sublevels of…

原子物理 · 物理学 2008-12-13 Benjamin K. Stuhl , Brian C. Sawyer , Dajun Wang , Jun Ye

We report the experimental realization of a conveyor-belt magneto-optical trap for calcium monofluoride (CaF) molecules. The obtained highly-compressed cloud has a mean radius of 64(5) $\mu$m and a peak number density of $3.6(5) \times…

As a heavy molecule, barium monofluoride (BaF) presents itself as a promising candidate for measuring permanent electric dipole moment. The precision of such measurements can be significantly enhanced by utilizing a cold molecular sample.…

原子物理 · 物理学 2024-10-29 Zixuan Zeng , Shuhua Deng , Shoukang Yang , Bo Yan

We improve the efficiency of sawtooth-wave-adiabatic-passage (SWAP) cooling for strontium atoms in three dimensions and combine it with standard narrow-line laser cooling. With this technique, we create strontium magneto-optical traps with…

原子物理 · 物理学 2019-06-26 S. Snigirev , A. J. Park , A. Heinz , I. Bloch , S. Blatt

We demonstrate the long-term ($<$ 1 minute) trapping of Stark-decelerated OH radicals in their $X~^{2}\Pi _{3/2}~(\nu = 0,~J = 3/2,~M_{J} = 3/2,~f)$ state in a permanent magnetic trap. The trap environment was cryogenically cooled to a…

化学物理 · 物理学 2019-08-05 Dominik Haas , Claudio von Planta , Thomas Kierspel , Dongdong Zhang , Stefan Willitsch

We describe experiments demonstrating efficient transfer of molecules from a magneto-optical trap (MOT) into a conservative magnetic quadrupole trap. Our scheme begins with a blue-detuned optical molasses to cool SrF molecules to $\sim\!50$…

原子物理 · 物理学 2018-07-11 D. J. McCarron , M. H. Steinecker , Y. Zhu , D. DeMille

We report on the electrostatic trapping of neutral SrF molecules. The molecules are captured from a cryogenic buffer-gas beam source into the moving traps of a 4.5 m long traveling-wave Stark decelerator. The SrF molecules in…

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