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Glasses have a wide range of technological applications. The recent discovery of ultrastable glasses that are obtained by depositing the vapor of a glass-forming liquid onto the surface of a cold substrate has sparked renewed interest in…

统计力学 · 物理学 2014-09-04 Amir Haji-Akbari , Pablo G. Debenedetti

The viscoelastic properties of thin polymeric films represent a central issue, especially for nanotechnological applications. In particular, it is highly relevant the dependence of viscoelasticity on the temperature. For polystyrene it is…

We consider thin fluid films placed on thermally conductive substrates and exposed to time-dependent spatially uniform heat source. The evolution of the films is considered within the long-wave framework in the regime such that both…

软凝聚态物质 · 物理学 2016-06-16 Nanyi Dong , Lou Kondic

Thin liquid films on surfaces are part of our everyday life, they serve e.g. as coatings or lubricants. The stability of a thin layer is governed by interfacial forces, described by the effective interface potential, and has been subject of…

Controlling thermal energy transfer at the nanoscale has become critically important in many applications and thermal properties since it often limits device performance. In this work, we study the effects on thermal conductivity arising…

We apply a previously developed asymptotic model (J. Fluid. Mech. 915, A133 (2021)) to study instabilities of free surface films of nanometric thickness on thermally conductive substrates in two and three spatial dimensions. While the…

流体动力学 · 物理学 2021-10-26 Ryan H. Allaire , Linda J. Cummings , Lou Kondic

Recent experiments have demonstrated that the glass transition temperature of thin polymer films can be shifted as compared to the same polymer in the bulk, the amplitude and the sign of this effect depending on the interaction between the…

统计力学 · 物理学 2007-05-23 D. Long , P. Sotta

We perform molecular dynamics simulations of an idealized polymer melt surrounding a nanoscopic filler particle to probe the effects of a filler on the local melt structure and dynamics. We show that the glass transition temperature $T_g$…

软凝聚态物质 · 物理学 2009-10-31 Francis W. Starr , Thomas B. Schrøder , Sharon C. Glotzer

Pattern formation induced by wrinkling is a very common phenomenon exhibited in soft-matter substrates. In all these systems wrinkles develop in presence of compressively stressed thin films lying on compliant substrates. Here we…

介观与纳米尺度物理 · 物理学 2019-03-26 Maria Caterina Giordano , Francesco Buatier de Mongeot

The proton dynamics of a 2D water monolayer confined inside a graphene slit pore is studied in Cartesian and molecular frames of reference using molecular dynamics simulations. The vibrational density of states of the proton was calculated…

介观与纳米尺度物理 · 物理学 2021-09-24 Mohd Moid , Yacov Finkelstein , Raymond Moreh , Prabal K Maiti

Manganite thin films are promising candidates for studying the strongly correlated electron systems. Understanding the growth-and morphology-driven changes in the physical properties of manganite thin films is vital for their applications…

Epsilon-near-zero materials are exceptional candidates for studying electrodynamics and nonlinear optical processes at the nanoscale. We demonstrate that by alternating a metal and a highly doped conducting-oxide, the epsilon-near-zero…

光学 · 物理学 2020-07-17 Maria Antonietta Vincenti , Domenico de Ceglia , Michael Scalora

We present results of molecular dynamics (MD) simulations for a non-entangled polymer melt confined between two completely smooth and repulsive walls, interacting with inner particles via the potential $U_{\rm wall}\myeq (\sigma/z)^9$,…

软凝聚态物质 · 物理学 2009-11-07 F. Varnik , J. Baschnagel , K. Binder

Equilibrium molecular dynamics simulations are used to investigate the effect of phase transitions on the transport properties of highly-confined water between parallel graphene sheets. An abrupt reduction by several orders of magnitude in…

计算物理 · 物理学 2019-01-23 Frederike Jaeger , Omar K. Matar , Erich A. Müller

We report molecular dynamics simulation results on the equilibrium properties of polymer thin films adsorbed onto flat and curved substrates. We first systematically determine the contact angle of polymer droplets on flat substrates as a…

软凝聚态物质 · 物理学 2023-12-15 Gabriel Catalini , Nicolás A. García , Daniel A. Vega , Arash Nikoubashman

This study reveals the influence of the surface energy and solid/liquid boundary condition on the breakup mechanism of dewetting ultra-thin polymer films. Using silane self-assembled monolayers, SiO$_2$ substrates are rendered hydrophobic…

软凝聚态物质 · 物理学 2017-05-03 Matthias Lessel , Joshua D. McGraw , Oliver Bäumchen , Karin Jacobs

We develop the Elastically Collective Nonlinear Langevin Equation theory to investigate, for the first time, glassy dynamics in capped metallic glass thin films. Finite-size effects on the spatial gradient of structural relaxation time and…

软凝聚态物质 · 物理学 2022-02-02 Anh D. Phan

The van der Waals forces across a very thin liquid layer (nanofilm) in contact with a plane solid wall make the liquid nonhomogeneous. The dynamics of such flat liquid nanofilms is studied in isothermal case. The Navier-Stokes equations are…

经典物理 · 物理学 2008-09-23 Henri Gouin , Sergey Gavrilyuk

We extend the force-level ECNLE theory to treat the spatial gradients of the alpha relaxation time and glass transition temperature, and the corresponding film-averaged quantities, to the geometrically asymmetric case of finite thickness…

软凝聚态物质 · 物理学 2024-01-15 Anh D. Phan , Kenneth S. Schweizer

We analyze thermodynamics of water samples confined in nanopores and prove that although the freezing temperature can be dramatically lower, the suppression of the ice nucleation leading to the freezing temperature depression is a truly…

软凝聚态物质 · 物理学 2012-06-18 P. O. Fedichev , L. I. Menshikov
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