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The use of pressure to obtain new materials that can be recovered under ambient conditions is a central problem in high-pressure physics. Despite decades of research, this goal has only been achieved in the laboratory for a few notable…

材料科学 · 物理学 2025-08-19 Reetam Paul , Jonathan C. Crowhurst , Stanimir A. Bonev

[Abridged] Observations of protoplanetary disks suggest that they are depleted in gas-phase CO. It has been posed that gas-phase CO is chemically consumed and converted into less volatile species through gas-grain processes. Observations of…

天体物理仪器与方法 · 物理学 2022-10-05 J. Terwisscha van Scheltinga , N. F. W. Ligterink , A. D. Bosman , M. R. Hogerheijde , H. Linnartz

Hydrogen-based direct reduction offers a sustainable pathway to decarbonize the metal production industry. However, stable metal oxides, like Cr$_2$O$_3$, are notoriously difficult to reduce, requiring extremely high temperatures (above…

In-space manufacturing is essential for achieving long-term planetary colonization, particularly on Mars, where material transport from Earth is both costly and logistically restrictive. Traditional subtractive manufacturing methods are…

天体物理仪器与方法 · 物理学 2026-02-19 Zane Mebruer , Wan Shou

Two different types of experiments were performed. In the first experiment, we studied the low-temperature condensation of vaporized graphite inside bulk liquid helium, while in the second experiment, we studied the condensation of single…

原子与分子团簇 · 物理学 2018-05-07 S. A. Krasnokutski , M. Goulart , E. B. Gordon , A. Ritsch , C. Jäger , M. Rastogi , W. Salvenmoser , Th. Henning , P. Scheier

The C$_4$F$_7$N/CO$_2$/O$_2$ gas mixture is the most promising eco-friendly gas insulation medium available. However, there are few studies on the mechanism of the influence of the buffer gas O2 ratio and its role in the decomposition…

计算物理 · 物理学 2024-01-19 Fanchao Ye , Yitian Chu , Pascal Brault , Dunpin Hong , Shuangshuang Tian , Yi Li , Song Xiao , Xiaoxing Zhang

With 1.85 billion tons produced per year, steel is the most important material class in terms of volume and environmental impact. While steel is a sustainability enabler, for instance through lightweight design, magnetic devices, and…

Excessive CO2 emission from fossil fuel usage has resulted in global warming and environmental crises. To solve this problem, the photocatalytic conversion of CO2 to CO or useful components is a new strategy that has received significant…

材料科学 · 物理学 2023-01-27 Saeid Akrami , Tatsumi Ishihara , Masayoshi Fuji , Kaveh Edalati

Direct fired supercritical CO2 (sCO2) power cycles allow for the combustion of gaseous fuels under oxyfuel conditions with inherent carbon capture. As the CO2 is captured intrinsically, the efficiency penalty of capture on the overall plant…

化学物理 · 物理学 2022-03-14 James M. Harman-Thomas , Kevin J. Hughes , Mohamed Pourkashanian

The formation of solid calcium carbonate (CaCO3) from aqueous solutions or slurries containing calcium and carbon dioxide (CO2) is a complex process of considerable importance in the ecological, geochemical and biological areas. Moreover,…

Chemical looping methane partial oxidation provides an energy and cost effective route for methane utilization. However, there is considerable CO2 co-production in state-of-the-art chemical looping systems, rendering a decreased…

化学物理 · 物理学 2020-01-08 Yan Liu , Lang Qin , Zhuo Cheng , Josh W. Goetze , Fanhe Kong , Jonathan A. Fan , Liang-shih Fan

In an effort to develop breakthrough technologies that enable drastic reduction in CO2 emissions from steel industry (ULCOS project), the reduction of iron ore by pure hydrogen in a direct reduction shaft furnace was investigated. After…

材料科学 · 物理学 2014-02-10 Andrea Ranzani Da Costa , D. Wagner , Fabrice Patisson

Solid O2 has been proposed as a possible reservoir for oxygen in dense clouds through freeze-out processes. The aim of this work is to characterize quantitatively the physical processes that are involved in the desorption kinetics of CO-O2…

天体物理学 · 物理学 2009-11-13 K. Acharyya , G. W. Fuchs , H. J. Fraser , E. F. van Dishoeck , H. Linnartz

Increasing anthropogenic carbon dioxide (CO$_2$) emissions have led to rising global temperatures and climate change. Using earth-abundant metal-oxide catalysts such as Cu$_2$O for reducing CO$_2$ through RWGS reaction seems lucrative. In…

Nanostructured catalysts have attracted the increased attention for biomass conversion into high-valued chemicals due to the rapid depletion of fossil resources and increasingly severe environmental issues. Supercritical carbon dioxide…

化学物理 · 物理学 2024-03-26 Zhiwei Jiang , Yongjian Zeng , Ruichao Guo , Lu Lin , Rafael Luque , Kai Yan

We performed density-functional theory calculations using the generalized gradient approximation for the exhange-correlation functional to investigate the unusual catalytic behavior of Ru under elevated gas pressure conditions for the…

材料科学 · 物理学 2008-02-03 C. Stampfl , M. Scheffler

We investigate the formation and evolution of interstellar dust-grain ices under dark-cloud conditions, with a particular emphasis on CO2. We use a three-phase model (gas/surface/mantle) to simulate the coupled gas--grain chemistry,…

星系天体物理 · 物理学 2015-05-28 Robin T. Garrod , Tyler Pauly

CO2 conversion into value-added products has gained significant interest over the few last years, as the greenhouse gas concentrations constantly increase due to anthropogenic activities. Here we report on experiments for CO2 conversion by…

等离子体物理 · 物理学 2016-09-19 A Ozkan , Thierry Dufour , T Silva , N Britun , R Snyders , F Reniers , A Bogaerts

Fe- and steelmaking is the largest single industrial CO2 emitter, accounting for 6.5% of all CO2 emissions on the planet. This fact challenges the current technologies to achieve carbon-lean steel production and to align with the…

材料科学 · 物理学 2022-08-02 I. R. Souza Filho , Y. Ma , M. Kulse , D. Ponge , B. Gault , H. Springer , D. Raabe

Copper oxide II is a p-type semiconductor that can be used in several applications. Focusing on producing such material using an easy and low-cost technique, we followed an acetate one-pot-like route for producing a polymer precursor…

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