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An adaptive modeling method (AMM) that couples a deep neural network potential and a classical force field is introduced to address the accuracy-efficiency dilemma faced by the molecular simulation community. The AMM simulated system is…

化学物理 · 物理学 2018-11-14 Linfeng Zhang , Han Wang , Weinan E

Lipid bilayer membranes are the fundamental biological barriers that permit life. The bilayer dynamics largely participates in orchestrating cellular workings and is characterized by substantial stability together with extreme plasticity…

软凝聚态物质 · 物理学 2022-12-05 Matteo Bottacchiari , Mirko Gallo , Marco Bussoletti , Carlo Massimo Casciola

Machine learning (ML) is transforming all areas of science. The complex and time-consuming calculations in molecular simulations are particularly suitable for a machine learning revolution and have already been profoundly impacted by the…

化学物理 · 物理学 2019-11-11 Frank Noé , Alexandre Tkatchenko , Klaus-Robert Müller , Cecilia Clementi

Accurate force fields are necessary for predictive molecular simulations. However, developing force fields that accurately reproduce experimental properties is challenging. Here, we present a machine learning directed, multiobjective…

We introduce a variational approximation to the microscopic dynamics of rare conformational transitions of macromolecules. Within this framework it is possible to simulate on a small computer cluster reactions as complex as protein folding,…

软凝聚态物质 · 物理学 2015-02-19 S. a Beccara , L. Fant , P. Faccioli

A force field is a critical component in molecular dynamics simulations for computational drug discovery. It must achieve high accuracy within the constraints of molecular mechanics' (MM) limited functional forms, which offers high…

机器学习 · 计算机科学 2024-10-10 Tianze Zheng , Ailun Wang , Xu Han , Yu Xia , Xingyuan Xu , Jiawei Zhan , Yu Liu , Yang Chen , Zhi Wang , Xiaojie Wu , Sheng Gong , Wen Yan

Methodologies for creating reactive potential energy surfaces from molecular mechanics force-fields are becoming increasingly popular. To date, molecular mechanics force-fields use harmonic expressions to treat bonding stretches, which is a…

化学物理 · 物理学 2019-05-22 R. J. Shannon , B. Hornung , D. P. Tew , D. R. Glowacki

Microscopic stress fields are widely used in molecular simulations to understand mechanical behavior. Recently, decomposition methods of multibody forces to central force pairs between the interacting particles have been proposed. Here, we…

软凝聚态物质 · 物理学 2016-11-23 Koh M. Nakagawa , Hiroshi Noguchi

Molecular dynamics (MD) simulates the time evolution of atomic systems governed by interatomic forces, and the fidelity of these simulations depends critically on the underlying force model. Classical force fields (CFFs) rely on fixed…

Molecular Dynamics simulations are becoming a powerful tool for examining and predicting atomic and molecular processes in various environment. The present review shows how, in the fields of plasma physics, chemistry and interactions with…

等离子体物理 · 物理学 2023-12-14 Pascal Brault

We present a molecular dynamics study of the effects of carbon- and iron-ion induced shock waves in DNA duplexes in liquid water. We use the CHARMM force field implemented within the MBN Explorer simulation package to optimize and…

生物物理 · 物理学 2016-10-21 Pablo de Vera , Nigel J. Mason , Fred. J. Currell , Andrey V. Solov'yov

To address the computational challenges of ab initio molecular dynamics and the accuracy limitations of empirical force fields, the introduction of machine learning force fields has proven effective in various systems including metals and…

软凝聚态物质 · 物理学 2023-12-18 Junbao Hu , Liyang Zhou , Jian Jiang

With recent advances in structural biology, including experimental techniques and deep learning-enabled high-precision structure predictions, molecular dynamics methods that scale up to large biomolecular systems are required. Current…

生物物理 · 物理学 2022-06-24 Tim Hempel , Simon Olsson , Frank Noé

The convergence of statistical learning and molecular physics is transforming our approach to modeling biomolecular systems. Physics-informed machine learning (PIML) offers a systematic framework that integrates data-driven inference with…

生物大分子 · 定量生物学 2025-11-11 Aaryesh Deshpande

Physics students now have access to interactive molecular dynamics simulations that can model and animate the motions of hundreds of particles, such as noble gas atoms, that attract each other weakly at short distances but repel strongly…

物理教育 · 物理学 2015-02-27 Daniel V. Schroeder

The MACE architecture represents the state of the art in the field of machine learning force fields for a variety of in-domain, extrapolation and low-data regime tasks. In this paper, we further evaluate MACE by fitting models for published…

化学物理 · 物理学 2023-08-16 David Peter Kovacs , Ilyes Batatia , Eszter Sara Arany , Gabor Csanyi

Molecular Dynamics (MD) simulations are essential for understanding the atomic-level behavior of molecular systems, giving insights into their transitions and interactions. However, classical MD techniques are limited by the trade-off…

生物大分子 · 定量生物学 2026-04-21 Ziyang Yu , Wenbing Huang , Yang Liu

Molecular simulations are essential tools in computational chemistry, enabling the prediction and understanding of molecular interactions and thermodynamic properties of biomolecules. However, traditional force fields face significant…

化学物理 · 物理学 2024-06-17 Junhan Chang , Duo Zhang , Yuqing Deng , Hongrui Lin , Zhirong Liu , Linfeng Zhang , Hang Zheng , Xinyan Wang

Developing accurate and efficient coarse-grained representations of proteins is crucial for understanding their folding, function, and interactions over extended timescales. Our methodology involves simulating proteins with molecular…

生物大分子 · 定量生物学 2023-10-11 Carles Navarro , Maciej Majewski , Gianni de Fabritiis

With the rapid advancement of computational techniques, Molecular Dynamics (MD) simulations have emerged as powerful tools in biomedical research, enabling in-depth investigations of biological systems at the atomic level. Among the diverse…

生物大分子 · 定量生物学 2024-09-05 Reza Bozorgpour