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Fully symmetric A1g phonons are expected to play a dominant role in electron scattering in strong topological insulators (TIs), thus limiting the ballistic transport of future electronic devices. Here, we report on femtosecond time-resolved…

介观与纳米尺度物理 · 物理学 2018-02-14 Jianbo Hu , Kyushiro Igarashi , Takao Sasagawa , Kazutaka G. Nakamura , Oleg V. Misochko

The class of layered 3D-topological insulators have shown intriguingly anomalous temperature dependence in their thermal expansion coefficients. It was proposed that stacking faults are the origin of the observed anomalous thermal…

材料科学 · 物理学 2020-01-08 Gyan Prakash , Koushik Pal , U. V. Waghmare , A. K. Sood

In this Rapid Communication we investigate the coupling between excited electrons and phonons in the highly anisotropic electronic structure of the prototypical topological insulator Bi$_2$Te$_3$. Using time- and angle-resolved…

介观与纳米尺度物理 · 物理学 2016-10-13 E. Golias , J. Sánchez-Barriga

We report an observation of coherent phonons of $E_g^1$, $E_u^1$, $A_{1g}^1$, and $E_g^2$ symmetry generated in a single-crystal film of $Bi_2Se_3$ by an intense single-cycle THz pulse. The atomic vibrations reveal themselves through…

We report time- and angle-resolved photoemission spectroscopy measurements on the topological insulator Bi2Se3. We observe oscillatory modulations of the electronic structure of both the bulk and surface states at a frequency of 2.23 THz…

High quality single crystals of Bi2Se3 were grown using a modified Bridgman technique, the detailed study were carried out using Raman spectroscopy and characterized by Laue diffraction and high resolution transmission electron microscopy.…

Time-resolved two color pump-probe polarization spectroscopy was performed at room temperature on SrTiO3 films grown directly on Si with film thickness varying from 2 nm to 7.8 nm. The E soft mode with a characteristic frequency of 0.2 THz…

材料科学 · 物理学 2015-03-17 Cheng Cen , Maitri P. Warusawithana , Darrell G. Schlom , Jeremy Levy

We tailor the shape and phase of the pump pulse spectrum in order to study the coherent lattice dynamics in tellurium. Employing the coherent control via splitting the pump pulse into a two-pulse sequence, we show that the oscillations due…

材料科学 · 物理学 2010-11-10 O V Misochko , M V Lebedev , H Schaefer , T Dekorsy

We present a combined experimental and theoretical study of the surface vibrational modes of the topological insulator (TI) Bi$_2$Se$_3$ with particular emphasis on the low-energy region below 10 meV that has been difficult to resolve…

Cr2Ge2Te6 has been of interest for decades, as it is one of only a few ferromagnetic insulators. Recently, this material has been revisited due to its potential as a substrate for Bi2Te3, a topological insulator. This enables the…

材料科学 · 物理学 2014-10-09 Yao Tian , Huiwen Ji , R. J. Cava L. D. Alegria , J. R. Petta , Kenneth S. Burch

Raman scattering [K. M. F. Shahil et al., Appl. Phys. Lett. 96, 153103 (2010), V. Gnezdilov et al., Phys. Rev. B 84, 195118 (2011) and H. H. Kung et al., Phys. Rev. B 95, 245406 (2017)], inelastic helium scattering [X. Zhu et al., Phys.…

The spontaneous condensation of excitons in the excitonic insulating phase has been reported in Ta$_2$NiSe$_5$ below 325 K. In this context, we present the temperature-dependent optical pump optical probe spectroscopy of Ta$_2$NiSe$_5$,…

材料科学 · 物理学 2024-12-02 Vikas Arora , Sukanya Pal , Luminita Harnagea , D. V. S. Muthu , A K Sood

Density Functional Theory (DFT) calculations not only allow to predict the vibrational and optical properties of solids but also to understand and disentangle the mechanisms playing a key role in the generation of coherent optical phonons.…

材料科学 · 物理学 2025-10-09 A. Levchuk , R. Busselez , G. Vaudel , P. Ruello , V. Juvé , B. Arnaud

The tetradymite compound BiSbTeSe$_2$, is one of the most bulk-insulating three-dimensional topological insulators, which makes it important in the topological insulator research. It is a member of the solid-solution system…

We investigate coupled electron-lattice dynamics in the topological insulator Bi2Te3 with time-resolved photoemission and time-resolved x-ray diffraction. It is well established that coherent phonons can be launched by optical excitation,…

We report femtosecond time-resolved reflectivity measurements of coherent phonons in tellurium performed over a wide range of temperatures (3K to 296K) and pump laser intensities. A totally symmetric A$_{1}$ coherent phonon at 3.6 THz…

材料科学 · 物理学 2015-05-20 N. Kamaraju , Sunil Kumar , M. Anija , A. K. Sood

The evolution of the optical phonons in layered semiconductor alloys SnSe1-xSx is studied as a function of the composition by using polarized Raman spectroscopy with six different excitation wavelengths (784.8, 632.8, 532, 514.5, 488, and…

Degenerate pump-probe reflectivity experiments have been performed on a single crystal of bismuth telluride (Bi$_2$Te$_3$) as a function of sample temperature (3K to 296K) and pump intensity using $\sim$ 50 femtosecond laser pulses with…

材料科学 · 物理学 2015-05-20 N. Kamaraju , Sunil Kumar , A. K. Sood

We have applied femtosecond pump-probe technique with variable pump wavelength to study coherent lattice dynamics in Bi single crystal. Comparison of the coherent amplitude as a function of pump photon energy for two different in symmetry…

材料科学 · 物理学 2015-05-20 A. A. Melnikov , O. V. Misochko , S. V. Chekalin

We report on electric-field and temperature dependent transport measurements in exfoliated thin crystals of Bi$_{2}$Se$_{3}$ topological insulator. At low temperatures ($< 50$ K) and when the chemical potential lies inside the bulk gap, the…

介观与纳米尺度物理 · 物理学 2015-06-19 M. V. Costache , I. Neumann , J. F. Sierra , V. Marinova , M. M. Gospodinov , S. Roche , S. O. Valenzuela
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