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Field-induced magnetic ordering in the Haldane chain compound SrNi$_{2}$V$_{2}$O$_{8}$ and effect of anisotropy have been investigated using single crystals. Static susceptibility, inelastic neutron scattering, high-field magnetization, and…

强关联电子 · 物理学 2013-10-02 A. K. Bera , B. Lake , A. T. M. N. Islam , B. Klemke , E. Faulhaber , J. M. Law

The magnetic ground state of the quasi-one-dimensional spin-1 antiferromagnetic chain is sensitive to the relative sizes of the single-ion anisotropy ($D$) and the intrachain ($J$) and interchain ($J'$) exchange interactions. The ratios…

We consider quasi one dimensional spin-1 Heisenberg chains with crystal field anisotropy in a uniform magnetic field. We determine the dynamical structure factor in various limits and obtain a fairly complete qualitative picture of how it…

强关联电子 · 物理学 2009-11-10 Fabian H. L. Essler , Ian Affleck

We report an inelastic neutron scattering study of antiferromagnetic spin dynamics in the Haldane chain compound Ni(C2H8N2)2NO2ClO4 (NENP) under external hydrostatic pressure P = 2.5 GPa. At ambient pressure, the magnetic excitations in…

凝聚态物理 · 物理学 2016-08-31 I. A. Zaliznyak , D. C. Dender , C. Broholm , Daniel H. Reich

We consider spin-1 Haldane chains with single-ion anisotropy, which exists in known Haldane chain materials. We develop a perturbation theory in terms of anisotropy, where magnon-magnon interaction is important even in the low temperature…

Inelastic neutron scattering on deuterated single-crystal samples is used to study Haldane-gap excitations in the new S=1 one-dimensional quantum antiferromagnet NDMAP, that was recently recognized as an ideal model system for high-field…

强关联电子 · 物理学 2009-10-31 A. Zheludev , Y. Chen , C. L. Broholm , Z. Honda , K. Katsumata

[Ni(HF$_2$)(3-Clpyridine)$_4$]BF$_4$ (NBCT) is a one-dimensional, $S = 1$ spin chain material that shows no magnetic neutron Bragg peaks down temperatures of 0.1 K. Previous work identified NBCT to be in the Haldane phase and near a quantum…

Two quasi-1-dimensional S=1 quantum antiferromagnetic materials, PbNi2V2O8 and SrNi2V2O8, are studied by inelastic neutron scattering on powder samples. While magnetic interactions in the two systems are found to be very similar, subtle…

强关联电子 · 物理学 2009-10-31 A. Zheludev , T. Masuda , I. Tsukada , Y. Uchiyama , K. Uchinokura , P. Boni , S. -H. Lee

Inelastic neutron scattering experiments on Nd2BaNiO5 single-crystals and powder samples are used to study the dynamic coupling of 1-dimensional Haldane-gap excitations in the S=1 Ni2+ -chains to local crystal-field transitions, associated…

强关联电子 · 物理学 2019-08-17 A. Zheludev , S. Maslov , T. Yokoo , J. Akimitsu , S. Raymond , S. E. Nagler , K. Hirota

The spin-1 Haldane chain is an example of the symmetry-protected-topological (SPT) phase in one dimension. Experimental realization of the spin chain materials usually involves both the uniaxial-type, $D(S^z)^2$, and the rhombic-type,…

强关联电子 · 物理学 2017-11-30 Yu-Chin Tzeng , Hiroaki Onishi , Tsuyoshi Okubo , Ying-Jer Kao

The molecular coordination complex NiI$_2$(3,5-lut)$_4$ [where (3,5-lut) $=$ (3,5-lutidine) $=$ (C$_7$H$_9$N)] has been synthesized and characterized by several techniques including synchrotron X-ray diffraction, ESR, SQUID magnetometry,…

The ground-state phase diagram of $S=2$ antiferromagnetic Heisenberg chains with coexisting uniform and alternating single-site anisotropies is investigated by the numerical exact diagonalization and density matrix renormalization group…

强关联电子 · 物理学 2014-02-18 Kazuo Hida

Inelastic neutron scattering experiments on the S=1 quasi-one-dimensional bond-alternating antiferromagnet Ni(C9D24N4)(NO2)ClO4 have been performed under magnetic fields below and above a critical field Hc at which the energy gap closes.…

We report the results of elastic and inelastic neutron scattering experiments on the Haldane gap quantum antiferromagnet Ni(C5D14N2)2N3(PF6) performed at mK temperatures in a wide range of magnetic field applied parallel to the S = 1 spin…

Inelastic neutron scattering experiments on the Haldane-gap quantum antiferromagnet \nd are performed at mK temperatures in magnetic fields of almost twice the critical field $H_c$ applied perpendicular to the spin cahins. Above $H_c$ a…

强关联电子 · 物理学 2009-11-10 A. Zheludev , Z. Honda , C. Broholm , K. Katsumata , S. M. shapiro , A. Kolezhuk , S. Park , Y. Qiu

Improving matrix-product state techniques based on the purification of the density matrix, we are able to accurately calculate the finite-temperature dynamic response of the infinite spin-1 XXZ chain with single-ion anisotropy in the…

强关联电子 · 物理学 2018-02-21 Florian Lange , Satoshi Ejima , Holger Fehske

We consider a quasi-one-dimensional system of spin-1 Heisenberg antiferromagnetic chains in 2D and 3D hypercubic lattices with interchain coupling $J$ and uniaxial single-ion anisotropy $D$. Using large scale numerical simulations, we map…

强关联电子 · 物理学 2014-06-24 Keola Wierschem , Pinaki Sengupta

[Ni(HF$_2$)(3-Clpyradine)$_4$]BF$_4$ (NBCT) is a one-dimensional (1-D), $S=1$ spin chain material that shows no long-range magnetic order down to thermometer temperatures of 0.1 K. Previous ambient pressure inelastic neutron scattering…

强关联电子 · 物理学 2022-06-14 D. M. Pajerowski , A. P. Podlesnyak , J. Herbrych , J. Manson

We reexamine the one-dimensional spin-1 $XXZ$ model with on-site uniaxial single-ion anisotropy as to the appearance and characterization of the symmetry-protected topological Haldane phase. By means of large-scale density-matrix…

强关联电子 · 物理学 2015-01-20 Satoshi Ejima , Holger Fehske

We investigate the magnetic field behaviour of an antiferromagnetic Heisenberg spin-1 chain with the most general single-ion anisotropy. We discuss the regime in which the magnetic field is below the transition value. The splitting of the…

凝聚态物理 · 物理学 2009-10-22 O. Golinelli , Th. Jolicoeur , R. Lacaze
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