相关论文: Molecular quantum rotors in gyroscopic motion with…

Recently Rydberg atom-ion bound states have been observed using a high resolution ion microscope (Nature 605, 453 (2022)) and the corresponding vibrational dynamics has been spectroscopically analyzed. The atom-ion bond is created by an…

This work presents a mechanism by which non-reciprocal wave transmission is achieved in a class of gyric metamaterial lattices with embedded rotating elements. A modulation of the device's angular momentum is obtained via prescribed…

Extremely fast rotating molecules carrying significantly more energy in their rotation than in any other degree of freedom are known as "super rotors". It has been speculated that super rotors may exhibit a number of unique properties.…

A non-spinning permanent ferromagnet is predicted to behave as a gyroscope at sufficiently low frequencies, which can be seen as a manifestation of the Einstein-de Haas effect. This yet unexplored regime has been recently proposed for…

We suggest a protocol for the sympathetic cooling of a molecular asymmetric top rotor co-trapped with laser-cooled atomic ions, based on resonant coupling between the molecular ion's electric dipole moment and a common normal mode of the…

The generation of unidirectional motion has been a long-standing challenge in engineering of molecular motors and, more generally, machines. A molecular motor is characterized by a set of low energy states that differ in their…

With the exception of the harmonic oscillator, quantum wave-packets usually spread as time evolves. We show here that, using the nonlinear resonance between an internal frequency of a system and an external periodic driving, it is possible…

We show that an array of polar molecules interacting with Rydberg atoms is a promising hybrid system for scalable quantum computation. Quantum information is stored in long-lived hyperfine or rotational states of molecules which interact…

We present a simple quantum mechanical model describing excited rotational states of molecules in superfluid helium nanodroplets, as recently studied in non-adiabatic molecular alignment experiments [Cherepanov et al., Phys. Rev. A 104,…

This paper discusses quantum algorithms for the generator coordinate method (GCM) that can be used to benchmark molecular systems. The GCM formalism defined by exponential operators with exponents defined through generators of the Fermionic…

We propose the implementation of Galileo group symmetry operations or, in general, linear coordinate transformations, in a quantum simulator. With an appropriate encoding, unitary gates applied to our quantum system give rise to Galilean…

Direct dynamics methods using Gaussian wavepackets have to rely only on local properties, such as gradients and hessians at the center of the wavepacket, so as to be compatible with the usual quantum chemistry methods. Matrix elements of…

It is proposed that nuclear (or electron) spins in a trapped molecule would be well isolated from the environment and the state of each spin can be measured by means of mechanical detection of magnetic resonance. Therefore molecular traps…

Quantum computing provides a novel avenue towards simulating dynamical phenomena, and, in particular, scattering processes relevant for exploring the structure of matter. However, preparing and evolving particle wave packets on a quantum…

Evaluating multi-center molecular integrals with Cartesian Gaussian-type basis sets has been a long-standing bottleneck in electronic structure theory calculation for solids and molecules. We have developed a vector-coupling and…

Typically the motion of self-propelled active particles is described in a quiescent environment establishing an inertial frame of reference. Here we assume that friction, self-propulsion and uctuations occur relative to a non-inertial frame…

We propose a method for arbitrary manipulations of a quantum wavepacket in an optical lattice by a suitable modulation of the lattice amplitude. A theoretical model allows to determine the modulation corresponding to a given wavepacket…

The atom-optics kicked rotor can be used to prepare specific momentum distributions on a discrete basis set. We implement a continuous-time quantum walk and a quantum search protocol in this momentum basis. In particular we propose ways to…

Applied magnetic fields can couple to atomic displacements via generalized Lorentz forces, which are commonly expressed as gyromagnetic $g$ factors. We develop an efficient first-principles methodology based on density-functional…

In single-molecule transistors, we observe inelastic cotunneling features that correspond energetically to vibrational excitations of the molecule, as determined by Raman and infrared spectroscopy. This is a form of inelastic electron…