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相关论文: Dissipation dynamics and spin-orbit force in time-…

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The ultra-fast demagnetization of small iron clusters initiated by an intense optical excitation is studied with time-dependent spin density functional theory (TDSDFT). In particular we investigate the effect of the spin-orbit interaction…

介观与纳米尺度物理 · 物理学 2016-07-27 Maria Stamenova , Jacopo Simoni , Stefano Sanvito

We introduce a new microscopic approach to calculate the dependence of fusion barriers and cross-sections on isospin dynamics. The method is based on the time-dependent Hartree-Fock theory and the isoscalar and isovector properties of the…

核理论 · 物理学 2017-02-01 K. Godbey , A. S. Umar , C. Simenel

This article concerns the time-dependent Hartree-Fock (TDHF) approximation of single-particle dynamics in systems of interacting fermions. We find that the TDHF approximation is accurate when there are sufficiently many particles and the…

量子物理 · 物理学 2015-02-25 Claude Bardos , Francois Golse , Alex D. Gottlieb , Norbert J. Mauser

A particle-number projection technique is used to calculate transfer probabilities in the $^{16}$O+$^{208}$Pb reaction below the fusion barrier. The time evolution of the many-body wave function is obtained with the time-dependent…

核理论 · 物理学 2010-11-11 Cédric Simenel

The spin-dependent localized Hartree-Fock (SLHF) density-functional approach is extended to the treatment of the inner-shell excited-state calculation of open-shell atomic systems. In this approach, the electron spin-orbitals in an…

原子物理 · 物理学 2009-11-13 Zhongyuan Zhou , Shih-I Chu

L\"owdin's symmetry dilemma is an ubiquitous issue in approximate quantum chemistry. In the context of Hartree-Fock (HF) theory, the use of Slater determinants with some imposed constraints to preserve symmetries of the exact problem may…

化学物理 · 物理学 2021-07-22 Leonardo A. Cunha , Joonho Lee , Diptarka Hait , C. William McCurdy , Martin Head-Gordon

The isospin dependence of the spin-orbit potential is investigated for an effective Skyrme like energy-functional suitable for density-dependent Hartree-Fock calculations. The magnitude of the isospin dependence is obtained from a fit to…

核理论 · 物理学 2016-02-17 M. M. Sharma , G. A. Lalazissis , J. Koenig , P. Ring

It is well known that non-central nuclear forces, such as the spin-orbital coupling and the tensor force, play important roles in understanding many interesting features of nuclear structures. However, their dynamical effects in nuclear…

核理论 · 物理学 2015-11-17 Jun Xu , Bao-An Li , Wen-Qing Shen , Yin Xia

We employ the time-dependent Hartree-Fock (TDHF) method to study various aspects of the reactions utilized in searches for superheavy elements. These include capture cross-sections, quasifission, prediction of $P_{\mathrm{CN}}$, and other…

核理论 · 物理学 2016-04-12 A. S. Umar , V. E. Oberacker

To investigate the two-body dissipation effects on the synthesis of superheavy elements, we calculate low-energy collisions of the $N=50$ isotones ($^{82}$Ge, $^{84}$Se, $^{86}$Kr and $^{88}$Sr) on $^{208}$Pb using the time-dependent…

核理论 · 物理学 2016-03-23 M. Tohyama , S. Umar

Background: The time-dependent Hartree-Fock (TDHF) theory has been successful in describing low-energy heavy ion collisions. Recently, we have shown that multinucleon transfer processes can be reasonably described in the TDHF theory…

核理论 · 物理学 2014-12-24 Kazuyuki Sekizawa , Kazuhiro Yabana

A previously proposed non-canonical coupled-perturbed Kohn-Sham density functional theory (KS-DFT)/Hartree-Fock (HF) treatment for spin-orbit coupling is here generalized to infinite periodic systems. The scalar-relativistic periodic…

The equilibration of macroscopic degrees of freedom during the fusion of heavy nuclei, like the charge and the shape, are studied in the Time-Dependent Hartree-Fock theory. The pre-equilibrium Giant Dipole Resonance (GDR) is used to probe…

核理论 · 物理学 2008-11-26 Cédric Simenel , Philippe Chomaz , Gilles De France

Time-dependent Hartree-Fock theory is used to describe density oscillations of symmetry-unrestricted two-dimensional nanostructures. In the small amplitude limit the results reproduce those obtained within a perturbative approach such as…

介观与纳米尺度物理 · 物理学 2009-11-07 Antonio Puente , Llorenç Serra , Vidar Gudmundsson

We estimate the prediction sensitivity with respect to Hartree-Fock exchange in approximate density functionals for representative Fe(II) and Fe(III) octahedral complexes. Based on the observation that the range of parameters spanned by the…

材料科学 · 物理学 2015-07-16 Efthymios I. Ioannidis , Heather J. Kulik

We report successful implementation of the time-dependent second-order many-body perturbation theory using optimized orthonormal orbital functions called time-dependent optimized second-order many-body perturbation theory [TD-OMP2] to reach…

化学物理 · 物理学 2020-08-26 Himadri Pathak , Takeshi Sato , Kenichi L. Ishikawa

We analyze the details of mass exchange in the vicinity of the Coulomb barrier for heavy-ion collisions involving neutron-rich nuclei using the time-dependent Hartree-Fock (TDHF) theory. We discuss the time-dependence of transfer and show…

核理论 · 物理学 2008-11-26 A. S. Umar , V. E. Oberacker , J. A. Maruhn

We propose a framework to learn the time-dependent Hartree-Fock (TDHF) inter-electronic potential of a molecule from its electron density dynamics. Though the entire TDHF Hamiltonian, including the inter-electronic potential, can be…

化学物理 · 物理学 2024-12-05 Harish S. Bhat , Prachi Gupta , Christine M. Isborn

The charge-exchange spin-dipole (SD) excitations of 208Pb are studied by using a fully self-consistent Skyrme Hartree-Fock plus Random Phase Approximation (HF+RPA) formalism which includes the tensor interaction. It is found, for the first…

核理论 · 物理学 2015-05-19 C. L. Bai , H. Q. Zhang , H. Sagawa , X. Z. Zhang , G. Colo , F. R. Xu

The real-time dynamics of local magnetic moments exchange coupled to a metallic system of conduction electrons is subject to dissipative friction even in the absence of spin-orbit coupling. Phenomenologically, this is usually described by a…

介观与纳米尺度物理 · 物理学 2025-01-08 Nicolas Lenzing , David Krüger , Michael Potthoff