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We study inelastic electron tunneling through a molecular junction using the non-equilibrium Green function (NEGF) formalism. The effect of the mutual influence between the phonon and the electron subsystems on the electron tunneling…

介观与纳米尺度物理 · 物理学 2009-11-10 Michael Galperin , Mark A. Ratner , Abraham Nitzan

Within a phonon-assisted resonance level model we develop a self-consistent procedure for calculating electron transport currents in molecular junctions with intermediate to strong electron-phonon interaction. The scheme takes into account…

介观与纳米尺度物理 · 物理学 2007-05-23 Michael Galperin , Abraham Nitzan , Mark A. Ratner

We study the nonlinear elastic quantum electronic transport properties of nanoscopic devices using the Nonequilibrium Green's function (NEGF) method. The Green's function method allows us to expand the $I-V$ characteristics of a given…

介观与纳米尺度物理 · 物理学 2009-07-14 Alexis R. Hernández , Caio H. Lewenkopf

Coherent electronic transport through a molecular device is studied using non-equilibrium Green's function (NEGF) formalism. Such device is made of a carbon nanowire which is connected to ferromagnetic electrodes. The molecule itself is…

介观与纳米尺度物理 · 物理学 2007-05-23 Kamil Walczak , Gloria Platero

We present a combined theoretical approach to study the nonequilibrium transport properties of nanoscale systems coupled to metallic electrodes and exhibiting strong electron-phonon interactions. We use the Keldysh Green function formalism…

介观与纳米尺度物理 · 物理学 2015-05-20 R. C. Monreal , F. Flores , A. Martin-Rodero

Off-resonant charge transport through molecular junctions has been extensively studied since the advent of single-molecule electronics and it is now well understood within the framework of the non-interacting Landauer approach. Conversely,…

We overview nonequilibrium Green function combined with density functional theory (NEGF-DFT) modeling of independent electron and phonon transport in nanojunctions with applications focused on a new class of thermoelectric devices where a…

介观与纳米尺度物理 · 物理学 2012-04-19 Branislav K. Nikolic , Kamal K. Saha , Troels Markussen , Kristian S. Thygesen

Non-equilibrium Green's functions (NEGF) formalism combined with extended Huckel (EHT) and charging model are used to study electrical conduction through single-molecule junctions. Analyzed molecular complex is composed of asymmetric…

介观与纳米尺度物理 · 物理学 2009-11-11 Kamil Walczak , Sergey Edward Lyshevski

We present an application of a new formalism to treat the quantum transport properties of fully interacting nanoscale junctions. We consider a model single-molecule nanojunction in the presence of two kinds of electron-vibron interactions.…

介观与纳米尺度物理 · 物理学 2013-04-08 H. Ness , L. K. Dash

Computationally inexpensive approximations describing electron-phonon scattering in molecular-scale conductors are derived from the non-equilibrium Green's function method. The accuracy is demonstrated with a first principles calculation on…

介观与纳米尺度物理 · 物理学 2007-05-23 Magnus Paulsson , Thomas Frederiksen , Mads Brandbyge

We present an application of a new formalism to treat the quantum transport properties of fully interacting nanoscale junctions [Phys. Rev. B {\bf 84}, 235428 (2011)]. We consider a model single-molecule nanojunction in the presence of two…

介观与纳米尺度物理 · 物理学 2012-10-15 H. Ness , L. K. Dash

The calculation of the nonlinear conductance of a single-molecule junction is revisited. The self energy on the junction resulting from the electron-phonon interaction has at low temperatures logarithmic singularities (in the real part) and…

介观与纳米尺度物理 · 物理学 2015-05-14 O. Entin-Wohlman , Y. Imry , A. Aharony

A local-orbital based ab initio approach to obtain the Green function for large heterogeneous systems is developed. First a Green function formalism is introduced based on exact diagonalization. Then the self energy is constructed from an…

介观与纳米尺度物理 · 物理学 2007-05-23 M. Albrecht , A. Schnurpfeil , G. Cuniberti

We describe a first-principles method for calculating electronic structure, vibrational modes and frequencies, electron-phonon couplings, and inelastic electron transport properties of an atomic-scale device bridging two metallic contacts…

介观与纳米尺度物理 · 物理学 2007-05-23 Thomas Frederiksen , Magnus Paulsson , Mads Brandbyge , Antti-Pekka Jauho

We use the effective-mass approximation and the density-functional theory with the local-density approximation for modeling two-dimensional nano-structures connected phase-coherently to two infinite leads. Using the non-equilibrium Green's…

介观与纳米尺度物理 · 物理学 2009-11-10 Paula Havu , Ville Havu , Martti Puska , Risto Nieminen

Within the framework of nonequilibrium Green's functions, we investigate the thermoelectric transport in a single molecular junction with electron-phonon and electron-electron interactions. By transforming into a displaced phonon basis, we…

介观与纳米尺度物理 · 物理学 2012-04-26 Jie Ren , Jian-Xin Zhu , James E. Gubernatis , Chen Wang , Baowen Li

We present a novel ab initio non-equilibrium approach to calculate the current across a molecular junction. The method rests on a wave function based description of the central region of the junction combined with a tight binding…

材料科学 · 物理学 2009-11-11 Martin Albrecht , Bo Song , Alexander Schnurpfeil

In this paper we develop the Non-Equilibrium Green's Function (NEGF) formalism for a dissipative molecular junction that consists of a central molecular system with one-dimensional electronic transport coupled to a phonon environment and…

介观与纳米尺度物理 · 物理学 2021-08-12 Matthew A Lane , Lev Kantorovich

Electron transport through a diatomic molecular tunnel junction shows wave like interference phenomenon. By using Keldysh non-equilibrium Green's function (NEGF) theory, we have explicitly presented current and differential conductance…

介观与纳米尺度物理 · 物理学 2012-12-18 Muhammad Imran

Quantum transport through single molecules is essentially affected by molecular vibrations. We investigate the behavior of the prototype single-level model with intermediate electron-vibron coupling and arbitrary coupling to the leads. We…

介观与纳米尺度物理 · 物理学 2009-11-13 Dmitry A. Ryndyk , Gianaurelio Cuniberti
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