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Correlated band theory is employed to investigate the magnetic and electronic properties of different arrangements of oxygen di- and tri-vacancy clusters in SrTiO$_3$. Hole and electron doping of oxygen deficient SrTiO$_3$ yields various…

材料科学 · 物理学 2016-03-30 Alejandro Lopez-Bezanilla , P. Ganesh , Peter B. Littlewood

Strontium titanate (SrTiO$_3$) is a foundational material in the emerging field of complex oxide electronics. While its electronic and optical properties have been studied for decades, SrTiO$_3$ has recently become a renewed materials…

介观与纳米尺度物理 · 物理学 2014-07-11 W. D. Rice , P. Ambwani , M. Bombeck , J. D. Thompson , C. Leighton , S. A. Crooker

We report the optical, electrical transport, and magnetotransport properties of high quality oxygen deficient SrTiO3 (STO) single crystal film fabricated by pulsed laser deposition and reduced in the vacuum chamber. The oxygen vacancy…

In this work, we study the time- and temperature-dependence of optically induced magnetization in bulk crystals of slightly oxygen-deficient SrTiO$_{3-\delta}$ using an optically coupled SQUID magnetometer. We find that a weak…

材料科学 · 物理学 2014-07-17 W. D. Rice , P. Ambwani , J. D. Thompson , C. Leighton , S. A. Crooker

We discuss, based on first principles calculations, the possibility to tune the magnetism of oxygen vacancies at the (001) surface of strontium titanate $(\mathrm{SrTiO_3}\!)$. The magnetic moment of single and clustered vacancies stemming…

介观与纳米尺度物理 · 物理学 2017-09-29 Oleg O. Brovko , Erio Tosatti

Oxygen-deficient TiO$_2$ in the rutile structure as well as the Ti$_3$O$_5$ Magn{\'e}li phase is investigated within the charge self-consistent combination of density functional theory (DFT) with dynamical mean-field theory (DMFT). It is…

材料科学 · 物理学 2017-06-07 Frank Lechermann , Wolfgang Heckel , Oleg Kristanovski , Stefan Müller

SrTiO$_3$ (STO) is the substrate of choice to grow oxide thin-films and oxide heterojunctions, which can form quasi-two-dimensional electronic phases that exhibit a wealth of phenomena, and, thus, a workhorse in the emerging field of…

强关联电子 · 物理学 2016-08-31 Soham S. Ghosh , Efstratios Manousakis

Ferroics based on transition-metal (TM) substituted SrTiO$_{3}$ have called much attention as magnetism and/or ferroelectricity can be tuned by using cations substitution and defects, strain and/or oxygen deficiency. C. A. Ross et al.…

Magnetism in La$_{1-x}$Sr$_x$CoO$_3$ as a function of doping is investigated with X-ray absorption spectroscopy and X-ray magnetic circular dichroism at the O K edge, and corresponding first principles electronic structure calculations. For…

强关联电子 · 物理学 2012-10-15 S. Medling , Y. Lee , H. Zhang , J. F. Mitchell , J. W. Freeland , B. N. Harmon , F. Bridges

We use density functional theory to calculate the structure, band-gap and magnetic properties of oxygen-deficient SrTi$_{1-x-y}$Fe$_x$Co$_y$O$_{3-\delta}$ with x = y = 0.125 and ${\delta}$ = (0,0.125,0.25). The valence and the high or low…

材料科学 · 物理学 2019-10-17 Mariel A. Opazo , Shyue Ping Ong , P. Vargas , C. A. Ross , Juan M. Florez

Mn-doped SrTiO_3.0, when synthesized free of impurities, is a paramagnetic insulator with interesting dielectric properties. Since delocalized charge carriers are known to promote ferromagnetism in a large number of systems via diverse…

材料科学 · 物理学 2013-10-08 D. Choudhury , B. Pal , A. Sharma , S. V. Bhat , D. D. Sarma

We address the long-standing question of the nature of oxygen vacancies in strontium titanate, using a combination of density functional theory and dynamical mean-field theory (DFT+DMFT) to investigate in particular the effect of…

强关联电子 · 物理学 2021-04-14 Jaime Souto-Casares , Nicola A. Spaldin , Claude Ederer

The stoichiometric antiferromagnetic insulator EuTiO$_3$ is proximate to a ferroelectric phase. Whereas cation substitution has been used as a tuning parameter to introduce charge carriers and manipulate the magnetism, the effects of…

SrTiO3 (STO) displays a broad spectrum of physical properties, including superconductivity, ferroelectricity, and photoconductivity, making it a standout semiconductor material. Despite extensive researches, the oxygen partial…

材料科学 · 物理学 2026-04-27 Zenghua Cai , Chunlan Ma

With the motive of unraveling the origin of native vacancy induced magnetization in ferroelectric perovskite oxide systems, here we explore the consequences of electronic structure modification in magnetic ordering of oxygen deficient…

The observation of metallic interface between band insulators LaAlO$_3$ and SrTiO$_3$ has led to massive efforts to understand the origin of the phenomenon as well as to search for other systems hosting such two dimensional electron gases…

The search for oxide-based room-temperature ferromagnetism has been one of the holy grails in condensed matter physics. Room-temperature ferromagnetism observed in Nb-doped SrTiO3 single crystals is reported in this Rapid Communication. The…

材料科学 · 物理学 2013-06-20 Z. Q. Liu , W. M. Lu , S. L. Lim , X. P. Qiu , N. N. Bao , M. Motapothula , J. B. Yi , M. Yang , S. Dhar , T. Venkatesan , Ariando

Motivated by recent spin- and angular-resolved photoemission (SARPES) measurements performed on the two-dimensional electronic states confined near the (001) surface of SrTiO$_3$ in the presence of oxygen vacancies, we explore their spin…

The magneto-optical properties of titanium dioxide systems are related to the presence of impurity states in the band gap due to oxygen vacancies. To understand about the interplay between localized electrons and structural distortions at…

材料科学 · 物理学 2023-05-10 C. Echeverria-Arrondo , H. Raebiger , J. Perez-Conde , C. Gomez-Polo , A. Ayuela

Ferromagnetism and superconductivity are in most cases adverse. However, recent experiments reveal that they coexist at interfaces of LaAlO3 and SrTiO3. We analyze the magnetic state within density functional theory and provide evidence…

强关联电子 · 物理学 2012-01-20 N. Pavlenko , T. Kopp , E. Y. Tsymbal , G. A. Sawatzky , J. Mannhart
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